Abstract
By considering the condition for lowest order decoupling of the vibrations of local atomic configurations of continuous bonded covalent systems, we arrive at an approximation which we call a decoupled network (DCN). The DCN them serves as a basis for a method of relating vibrational and configurational data in low symmetry systems. This method applied to amorphous, crystalline and molten As 2S 3 yields significant insight into the relationship between the features of the vibrational spectra and the local order.
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