Creation of charged excitons with two-color excitation method and initialization of electron spin qubit in quantum dots

Abstract

An optical pumping method for creating charged excitons in semiconductor quantum dots is demonstrated using a two-color excitation method. This method employs two laser sources whose energies are in the resonant and barrier excitation conditions, respectively. The photoluminescence (PL) spectra of a single quantum dot clearly vary from exciton-originated PL to charged exciton-originated PL as the excitation conditions are changed. This method is applied to the initialization process of an electron spin qubit without a magnetic field, which provides a simple and effective way of implementing quantum computing with spin qubits.