Coexistence of Superconductivity and Charge Density Waves in Tantalum Disulfide: Experiment and Theory

Y Kvashnin,O Karis,R Thiyagarajan,M Abdel-Hafiez,A N Vasiliev,M Mito,O Eriksson,S A Medvedev,D Vangennep

doi:10.1103/physrevlett.125.186401

Abstract

The coexistence of charge density wave (CDW) and superconductivity in tantalum disulfide (2H-TaS_{2}) at low temperature is boosted by applying hydrostatic pressures to study both vibrational and magnetic transport properties. Around P_{c}, we observe a superconducting dome with a maximum superconducting transition temperature T_{c}=9.1 K. First-principles calculations of the electronic structure predict that, under ambient conditions, the undistorted structure is characterized by a phonon instability at finite momentum close to the experimental CDW wave vector. Upon compression, this instability is found to disappear, indicating the suppression of CDW order. The calculations reveal an electronic topological transition (ETT), which occurs before the suppression of the phonon instability, suggesting that the ETT alone is not directly causing the structural change in the system. The temperature dependence of the first vortex penetration field has been experimentally obtained by two independent methods. While a d wave and single-gap BCS prediction cannot describe the lower critical field H_{c1} data, the temperature dependence of the H_{c1} can be well described by a single-gap anisotropic s-wave order parameter.

Highlights

The coexistence of charge density wave (CDW) and superconductivity in tantalum disulfide (2H-TaS2) at low temperature is boosted by applying hydrostatic pressures to study both vibrational and magnetic transport properties
The calculations reveal an electronic topological transition (ETT), which occurs before the suppression of the phonon instability, suggesting that the ETT alone is not directly causing the structural change in the system
We explore external pressure as a tool to tune the phonon dispersions and the stability of the CDW phase

Summary

Introduction

The coexistence of charge density wave (CDW) and superconductivity in tantalum disulfide (2H-TaS2) at low temperature is boosted by applying hydrostatic pressures to study both vibrational and magnetic transport properties. First-principles calculations of the electronic structure predict that, under ambient conditions, the undistorted structure is characterized by a phonon instability at finite momentum close to the experimental CDW wave vector.

Results

Conclusion