Coercivity analysis in sputtered Sm–Co thin films

Abstract

Hard nanocrystalline Sm–Co thin films having a thickness of 500 nm have been prepared by heat-treating magnetron sputtered amorphous samples deposited over a 300 nm Cr buffer layer onto room temperature water cooled Si substrates. The thermal treatments resulted in the nanocrystallization of the precursor films and in the development of room temperature coercivities covering a range going from a few kOe, measured in the samples treated at low temperature, up to some tens of kOe, observed in the case of the films annealed at high temperatures (the room temperature coercivity of the sample treated at 825 K was 26 kOe). Our analysis of the influence of the thermal treatments on the particularities of the reversal process was based on the measurement of the temperature dependence of the coercive force. It was carried out in the framework of the micromagnetic model, which allowed us to evaluate two parameters accounting for the local anisotropy reduction and the magnitude of the local dipolar fields, respectively. Our results show that the high temperature treatments result in a better degree of crystallization (lower local anisotropy deterioration). That crystallinity improvement is associated to an increase of the local dipolar interactions.