Abstract
Magnetic cation of Co2+ was incorporated in a monovalent [Ni(dmit)2]- (2-thioxo-1,3-dithiole-4,5-dithiolate) salt by using the supramolecular framework of 15-crown-5. The π-spins of [Ni(dmit)2]- formed a one-dimensional Heisenberg antiferromagnetic linear chain, while the d-spin of Co2+ behaved as a free S = 3/2 spin within the crystal.
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