Abstract
Reaction of the phosphine adduct [ButSi(CH2PMe2)3]CrCl3 with alkyl-lithium reagents gives the first octahedral chromium(III) trialkyls [ButSi(CH2PMe2)3]CrR3(R = Me, Bun); both compounds have been crystallographically characterized and the n-butyl compound is found to be remarkably resistant to β-elimination.
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