Abstract
AbstractCephalosporolide B (I) is efficiently synthesized and exploited for the first time as a versatile biomimetic synthetic precursor for the chemical syntheses of not only cephalosporolides C (II) and G (V) via a challenging diastereoselective oxa‐Michael addition but also the structurally unprecedented cephalosporolides E (III) and F (IV) via a novel biomimetic ring‐contraction rearrangement.
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