Abstract

this work addresses the methodological challenges of undertaking techno-economic assessments of very early stage (technology readiness level 3–4) CO2 capture technologies. It draws lessons from a case study on CO2 capture from a natural gas combined cycle with exhaust gas recycle and electric swing adsorption technology. The paper shows that also for very early stage technologies it is possible to conduct techno-economic studies that give a sound first indication of feasibility, providing certain conditions are met. These conditions include the availability of initial estimates for the energy use of the capture technology, either from bench scale measurements, or from rigorous process models, and the possibility to draw up a generic (high level) equipment list. The paper shows that for meaningful comparison with incumbent technologies, the performance of very early stage technologies needs to be projected to a future, commercial state. To this end, the state of the art methods have to be adapted to control for the development and improvements that these technologies will undergo during the R&D cycle. We call this a hybrid approach. The paper also shows that CO2 capture technologies always need to be assessed in sympathy with the CO2 source (e.g. power plant) and compression plant, because otherwise unreliable conclusions could be drawn on their feasibility. For the case study, it is concluded that electric swing adsorption is unlikely to become economically competitive with current technologies, even in a highly optimised future state, where 50% of the regeneration duty is provided by LP steam and 50% by electricity: the net efficiency of an NGCC with EGR and optimised ESA (49.3%LHV; min–max 45.8–50.4%LHV) is lower than that of an NGCC with EGR and standard MEA (50.4%LHV). Also, investment and operational costs are higher than MEA, which together with ESA’s lower efficiency leads to an unfavourable levelised cost of electricity: 103€/MWh (min–max 93.89–117.31€/MWh) for NGCC with ESA, versus 91€/MWh for NGCC with MEA.

Highlights

  • Carbon capture and storage (CCS) is a necessary technology towards deep decarbonisation of the energy and industrial sectors, thereby mitigating severe global warming [1]

  • For CCS to succeed as a CO2 mitigation strategy, it is necessary to especially advance the technologies that are most promising in terms of technical, economic and environmental performance

  • The Natural gas combined cycles (NGCC) + electric swing adsorption (ESA) net efficiency increases from 45.9% to 47.5% under an assumption of 25% regeneration with steam (NGCC ESA 25/75), and to 49.3% under an assumption of 50% regeneration with steam (NGCC ESA 50/50)

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Summary

Introduction

Carbon capture and storage (CCS) is a necessary technology towards deep decarbonisation of the energy and industrial sectors, thereby mitigating severe global warming [1]. To reach a commercially ready portfolio of the most promising CCS technologies on time, and in an efficient way, targeted technology selection and investment are required [7]. This selection requires performance assessment of the different technology alternatives, by analysing the performance of the carbon capture technology in an integrated system (CO2 source, carbon capture installation, transport, and storage) already during the early stages of development. These analyses will point out key improvement options, thereby supporting RD & D

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