Abstract

Island chains off western Kyushu are the surface exposure in the northern margin of the Taiwan–Sinzi Folded Zone that spreads along the arc–trench system in the back-arc side from SW Japan to Taiwan. Intermittent igneous activity between the Middle Miocene and Holocene occurred on these islands and widely covered or intruded sedimentary rocks of Early–Middle Miocene. Geochemistry of the volcanic rocks from the Hirado, Ikitsuki and Takushima islands believed to relate to the back-arc opening along the East China and Japan Seas shows a temporal change in source material. Submarine to sub-aerial volcanism occurred on Hirado Island at 15 Ma during the final opening stage of the East China Sea producing tholeiitic basalt and associated andesite–dacite. These eruptives show low incompatible element contents and high FeO*/MgO ratios and reflect a tholeiitic differentiation trend. High Sr and Pb and low Nd isotopic ratios suggest the involvement of EM2-like lithospheric mantle and crustal material in the formation of these syn-opening volcanic rocks. Post-opening alkali basalt volcanism occurred at 9–6 Ma on the islands is characterized by OIB-like higher large ionic lithophile elements (LILE) and high field strength elements (HFSE) compared to 15 Ma basalts in this region and Quaternary basalts along the volcanic front. They have variable range of incompatible element concentrations and ratios along with variable Sr, Pb and Nd isotopic ratios suggesting the involvement of both lithospheric and asthenospheric sources at variable melting degrees (from 4% to less than 15%). The observation that the isotopic compositions of Quaternary alkali basalts south of the studied area are even more depleted suggests an increase in the involvement of asthenospheric source with time.

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