Abstract

The high anisotropy in RO1−aFaBiS2 (R denotes a rare-earth element) superconductors demonstrates their potential use as intrinsic Josephson junctions, considering the weak coupling among BiS2–PrO(F)–BiS2 (superconducting–normal–superconducting) layers along the c-axis. We grew PrO1−aFaBiS2 single crystals using CsCl/KCl flux. The superconducting anisotropies of the grown single crystals were estimated to be approximately 40–50 from the effective mass model. The c-axis transport properties were characterized using single-crystal s-shaped intrinsic Josephson junctions with a focused ion beam. Along the c-axis, the crystals showed zero resistivity at 2.7 K and a critical current density of 1.33 × 103 A/cm2 at 2.0 K. The current–voltage curve along the c-axis displayed hysteresis. The c-axis transport measurements under a magnetic field parallel to the ab-plane revealed a “lock-in” state due to the Josephson vortex flow, indicating that BiS2 superconductors are promising candidates for intrinsic Josephson junctions.

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