Case study of Er- and Dy-doped boron-aluminosilicate glasses on radiation shielding performance in the energy range 0.015–10 MeV with MCNP6.2

Abstract

The use of radiation-shielding materials has significantly increased with the advancement of new technologies. The present work aims to demonstrate that the nuclear shielding properties of boron-aluminosilicate glasses can be enhanced by doping with rare earth elements (REEs) such as erbium (Er) and dysprosium (Dy). Testing was performed by mixing different ratios of dopants into the glass system. This procedure was implemented on 13Al2O3–21B2O3-35.4SiO2-(30.6-X) Er2O3-X(Dy2O3) glass, where X = 0, 15.3, 22.1, and 30.6. MCNP6.2, SRIM, PSD, ROOT software, and XCOM databases were used as tools. MCNP6.2 software and XCOM databases were used to calculate, simulate, and validate the mass attenuation cross-sections for 15 selected gamma energies ranging from 0.01 MeV to 10 MeV. On the other hand, SRIM was used to obtain information about the mass stopping power (MSP) and stopping distance, the so-called projected range (PR), for charged particles of H+1 and He+2. Likewise, the PSD was only used to obtain a fast neutron removal cross-section (FNRCS) per density value for each element. This is referred to as the macroscopic neutron cross-section for fast neutron removal in the literature. Finally, the data analysis framework ROOT was used for calculations and graphical representations. To validate this study, the radiation-shielding properties of the material were compared with the globally accepted mass attenuation coefficient database of XCOM using MCNP6.2 simulation results. The proximity between these two is promising. The accuracy of the study was determined by examining the relative error values. The results indicate a strong correlation between the database and theoretical data. Radiation shielding properties such as mass and linear attenuation coefficients (MAC and LAC), half and tenth value layers (HVL and TVL), mean free path (MFP), effective atomic number (Zeff), effective electron density (Neff), effective conductivity (Ceff), and fast neutron removal cross-sections (FNRCS) against gamma rays suggested that the lowest X ratio indicated the highest protection. However, the MSP and PR values for the charged particles at most energies indicate the lowest protection with the lowest X ratio in the glass mixture. Finally, the glass shield with the lowest X ratio provided the highest neutron protection, similar to gamma rays. In summary, dysprosium and erbium doping in boron-aluminosilicate glasses can be tailored to specify different requirements for gamma-ray and particle attenuation, as well as neutron absorption. This study aims to fill a gap in the literature by providing a basis for future research on shielding materials based on doped boron-aluminosilicate glasses using high-atomic-number particles, such as REEs, as a radiation protection medium.