Abstract

Single-wall carbon nanotube (SWCNT) thin films are promising for sensitive uncooled infrared detection based on the photothermoelectric effect. The SWCNT film is usually shaped into a belt and diversely doped to form a p-n junction at the center. Under the illumination of a focused incident light, the temperature gradient from the junction to the contacts leads to photoresponse. When the SWCNTs are aligned in one direction, the photoresponse becomes polarization selective. Although a typical bowtie antenna can improve the responsivity and polarization extinction ratio by deep-subwavelength light focusing, the absolute absorptance of the junction region is only 0.6%. In this work, the antenna was engineered for a higher light coupling efficiency. By integrating a bottom metal plane at a specific distance from the SWCNT film and optimizing the antenna geometries, we achieved ultra-efficient impedance matching between the antenna and the SWCNTs, thus the absorptance of the junction region was further enhanced by 21.3 times and reached 13.5%, which is more than 3 orders of magnitude higher than that of the device without the engineered antenna. The peak responsivity was further enhanced by 19.9 times and responsivity reached 1500 V/W at 1 THz. The resonant frequency can be tuned by changing the size of the antenna. Over the frequency range of 0.5 THz to 1.5 THz, the peak responsivity was further enhanced by 8.1 to 19.9 times, and the polarization extinction ratio was enhanced by 2.7 to 22.3 times. The highest polarization extinction ratio reached 3.04 × 105 at 0.5 THz. The results are based on the numerical simulations of the light and the thermal fields.

Highlights

  • Single-wall carbon nanotube (SWCNT) thin films are promising for sensitive uncooled infrared detection based on the photothermoelectric effect

  • We propose to significantly enhance the absorptance of the junction region in an aligned SWCNT film by engineering the optical antenna

  • SWCNT film is considered as an effective uniaxial medium [18,19] because the diameter of each SWCNT and the inter-distances between them are within the deep subwavelength scale

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Summary

Introduction

Single-wall carbon nanotube (SWCNT) thin films are promising for sensitive uncooled infrared detection based on the photothermoelectric effect. Thermal detectors have an advantage as they can operate in an uncooled mode, they are generally less sensitive and slower than photonic detectors [4] In this situation, new materials with a prominent thermoelectric effect, low specific heat capacity, and high thermal stability become promising candidates for future infrared thermal detectors [5,6,7,8,9,10,11,12]. New materials with a prominent thermoelectric effect, low specific heat capacity, and high thermal stability become promising candidates for future infrared thermal detectors [5,6,7,8,9,10,11,12] Among those materials, single-wall carbon nanotubes (SWCNT) have attracted great attention due to their unique electrical, optical and thermal properties [4,8,9,10,11,12,13,14]. They are compatible published maps and institutional affiliations

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