Abstract
Hydrogarnets are vital intermediate products in the calcification- carbonation method, which is designed for Bayer red mud treatment. Their carbonation performance greatly depends on SiO2 substitution. In this study, different SiO2-substituted hydrogarnets were synthesized and characterized. Then, batch experiments were performed to evaluate the potential effects of important parameters such as CO2 pressure, and SiO2 substitution degree (x) on the carbonation process. The SiO2 substitution degrees of the hydrogarnets synthesized at 60, 120, 180, and 240°C were 0.27, 0.36, 0.70, and 0.73, respectively. As the SiO2 substitution degree increased, the hydrogarnet carbonation extents gradually declined. With an increase in CO2 pressure, the hydrogarnet carbonation percentages increased gradually and rose from 80.33% to 98.19% within 120min. The phases detected in the carbonized products were strip-like aragonite as well as some calcite; the Al-rich and Si-rich phases in the carbonized products were amorphous.
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