Abstract
A comparison of the electronic structures of the molecules OPF 3 and SPF 3 is performed within the framework of an ab initio SCF LCAO MO study. In complete agreement with the empirical assumptions provided by previous magneto-optical experiments, the (PS) bond in SPF 3 is weaker, endowed with a higher π character and less polar than the (PO) bond in OPF 3.
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