Abstract

Smart actuators have shown great potential for a range of industries, including artificial muscles, sensors, and smart devices. However, traditional actuators often suffer from small deformation and complex materials and manufacturing processes. Graphene oxide (GO) has emerged as an ideal candidate for moisture-responsive actuators due to its excellent moisture sensitivity. In this study, we present the development of a moisture-responsive actuator using a simple and straightforward approach based on a monolayer graphene oxide (GO) paper. By utilizing the different affinity of its two sides for water, the graphene oxide actuator demonstrates excellent performance in response to humidity gradients, achieving a large bending amplitude with a curvature of 3 cm−1. Furthermore, the graphene oxide actuator was used as a humidity-sensitive switch to perform on and off switch movements, demonstrating its capability for autonomous detection for real-time humidity monitoring. This work provides a new avenue for the development of moisture-responsive materials and their potential applications in the design of intelligent control systems, actuators, soft robots, artificial muscles, and switches.

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