Assessment of the coronavirus disease 2019 (COVID-19) pandemic imposed lockdown and unlock effects on black carbon aerosol, its source apportionment, and aerosol radiative forcing over an urban city in India

Abstract

A nationwide lockdown was imposed in India due to the Coronavirus Disease 2019 (COVID-19) pandemic which significantly reduced the anthropogenic emissions. We examined the characteristics of equivalent black carbon (eBC) mass concentration and its source apportionment using a multiwavelength aethalometer over an urban site (Ahmedabad) in India during the pandemic induced lockdown period of year 2020. For the first time, we estimate the changes in BC, its contribution from fossil (eBCff) and wood (eBCwf) fuels during lockdown (LD) and unlock (UL) periods in 2020 with respect to 2017 to 2019 (normal period). The eBC mass concentration continuously decreased throughout lockdown periods (LD1 to LD4) due to enforced and stringent restrictions which substantially reduced the anthropogenic emissions. The eBC mass concentration increased gradually during unlock phases (UL1 to UL7) due to the phase wise relaxations after lockdown. During lockdown period eBC mass concentration decreased by 35%, whereas during the unlock period eBC decreased by 30% as compared to normal period. The eBCwf concentrations were higher by 40% during lockdown period than normal period due to significant increase in the biomass burning emissions from the several community kitchens which were operational in the city during the lockdown period. The average contributions of eBCff and eBCwf to total eBC mass concentrations were 70% and 30% respectively during lockdown (LD1 to LD4) period, whereas these values were 87% and 13% respectively during the normal period. The reductions in BC concentrations were commensurate with the reductions in emissions from transportation and industrial activities. The aerosol radiative forcing reduced significantly due to the reduction in anthropogenic emissions associated with COVID-19 pandemic induced lockdown leading to a cooling of the atmosphere. The findings in the present study on eBC obtained during the unprecedented COVID-19 induced lockdown can provide a comprehensive understanding of the BC sources and current emission control strategies, and thus can serve as baseline anthropogenic emissions scenario for future emission control strategies aimed to improve air quality and climate.