Abstract

Anomalous positive magnetoresistance (MR) in high temperature organic-based magnet V(TCNE)x (TCNE=tetracynoethylene) thin films is reported. MR increases linearly with applied magnetic field and shows a maximum at the ferrimagnetic ordering temperature. The suggested roles of oppositely spin polarized π* electronic subbands and magnetization fluctuations due to the disordered nature of V(TCNE)x films are discussed.

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