Abstract

The combination of topology and magnetism has demonstrated great potential in the search of emergent quantum matters. In this study, we report the synthesis, magnetic, and electrical properties of GdAuPb, a rare-earth-based half-Heusler topological antiferromagnet candidate. Magnetization and specific heat studies reveal highly frustrated antiferromagnetic ordering of Gd at TN = 11.5 K. Interestingly, this material possesses a large, unsaturated magnetoresistance up to 800% below TN and anomalous Hall conductivity as large as 750 Ω−1cm−1 in the antiferromagnetic state. Moreover, the electric transports including the SdH quantum oscillation patterns all exhibit a sudden change around 9 T, indicating a field-driven quantum transition related to the Fermi surface reconstruction. These results suggest that GdAuPb is close to a topological critical point, which can be easily tuned via external parameters. Our study demonstrates a strong interplay between band topology and magnetism in GdAuPb and offers clues for material designs for topological antiferromagnets.

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