A new method for investigating the impact of temperature on in-situ reservoir properties using high-temperature AFM

Abstract

Accurately evaluating the influence of temperature variations is crucial for geothermal engineering. Existing conventional testing methods are limited in providing detailed characterizations of reservoir micro properties at high temperatures. This study employed variable-temperature AFM testing techniques to examine sandstone and limestone under in-situ temperatures (25-200°C). The study analyzed the mechanisms behind the temperature effects on rock properties and established theoretical models for porosity and permeability variations with elevated temperatures based on these mechanisms. The research revealed that sandstone and limestone exhibit similar temperature effects at high temperatures. The pore fractal dimension of sandstone and limestone does not change with temperature change. As the temperature increases, sandstone and limestone experience mean roughness (Ra) and porosity reductions. The impact of high temperature was more pronounced on sandstone compared to limestone, with sandstone showing a decrease of 2.8 % and 0.59 % in mean roughness (Ra) and AFM porosity, respectively, from 25 °C to 200 °C, while limestone exhibited reductions of 1.4 % and 0.085 %, respectively. With increasing temperature, sandstone transformed some pores with equivalent diameters of 1-2.5 μm to pores smaller than 1μm, while limestone did not show significant changes in pore structure. The temperature effects on sandstone and limestone were attributed to mineral expansion. Sandstone contains a higher proportion of minerals with a high coefficient of thermal expansion, such as quartz. In contrast, limestone primarily comprises minerals with lower thermal expansion coefficients, such as calcite, resulting in a more significant temperature impact on sandstone than on limestone. The theoretical models based on the mechanisms for porosity and permeability at high temperatures exhibited good predictive performance for sandstone and are more suitable for reservoirs predominantly composed of minerals with high coefficients of thermal expansion. The variation of porosity and permeability at high temperatures have different impacts on geothermal reservoirs. Temperature effects on porosity and permeability should be considered in geothermal engineering.