Abstract

Abstract. The mineralogy of airborne dust affects the impact of dust particles on direct and indirect radiative forcing, on atmospheric chemistry and on biogeochemical cycling. It is determined partly by the mineralogy of the dust-source regions and partly by size-dependent fractionation during erosion and transport. Here we present a data set that characterizes the clay and silt-sized fractions of global soil units in terms of the abundance of 12 minerals that are important for dust–climate interactions: quartz, feldspars, illite, smectite, kaolinite, chlorite, vermiculite, mica, calcite, gypsum, hematite and goethite. The basic mineralogical information is derived from the literature, and is then expanded following explicit rules, in order to characterize as many soil units as possible. We present three alternative realizations of the mineralogical maps, taking the uncertainties in the mineralogical data into account. We examine the implications of the new database for calculations of the single scattering albedo of airborne dust and thus for dust radiative forcing.

Highlights

  • Dust particles, emitted in large quantities by aeolian erosion of arid and semi-arid soils, play an important role on Earth’s climate system

  • Sokolik and Toon (1996), were the first to suggest incorporating the mineralogical composition of dust particles into models and subsequent work has shown the importance of accounting for mineralogy in estimating the direct radiative effect (Claquin et al, 1999; Sokolik and Toon, 1999; Balkanski et al, 2007; Hansell et al, 2008)

  • Mineralogy affects the hygroscopic properties of atmospheric particles and the indirect radiative forcing by dust

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Summary

Introduction

Dust particles, emitted in large quantities by aeolian erosion of arid and semi-arid soils, play an important role on Earth’s climate system. During atmospheric transport, they affect Earth’s radiative budget directly by absorbing or scattering the solar or infrared radiation (Sokolik and Toon, 1996) or indirectly by acting as cloud condensation nuclei (CCN) or ice nuclei (IN) (Rosenfeld et al, 2001; DeMott et al, 2003; Creamean et al, 2013). The mineralogy of airborne dust is linked to the mineralogy of the erodible fraction of the soil source, modified by size fractionation during erosion, suspension and transport. We examine some of the consequences of using this database to specify the properties of airborne dust

Construction of the database
Distribution of minerals by size class
Iron content of the clay-size fraction
Associating mineralogy with soil unit
Database of topsoil mineralogy
Expansion of the database and production of the mean mineralogical tables
Creation of the mineralogical maps
Minerals in the clay fraction: the example of illite
Mineralogy of the silt fraction: the example of mica
Minerals occurring in both silt and clay fractions: the example of calcite
Mineralogical composition over modern dust-source regions
Differences between soil and airborne dust mineralogy
Discussion
19 Yermosols haplic
Implications for dust optical properties: single scattering albedo
Findings
Single scattering albedo of dust computed from iron oxide minerals
Conclusions
Full Text
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