Abstract
Primary yields of radiolysis products of water and nitrate in concentrated nitric acid solutions for low LET radiation were evaluated from the previous studies on radiolysis while those for high LET radiation by using a diffusion kinetics model for the intra-track processes. Radiolytic reactions of NO x and uranium ions in the solutions were proposed mainly from the reported data, and then applied together with the yields to the radiolytic formation of HNO 2 and oxidation of U 4+ to demonstrate the reaction model.
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