Abstract

$Background:$ Previous measurements of $\beta$-delayed neutron emitters comprise around 230 nuclei, spanning from the $^{8}$He up to $^{150}$La. Apart from $^{210}$Tl, with a minuscule branching ratio of 0.007\%, no other neutron emitter is measured yet beyond $A=150$. Therefore new data are needed, particularly in the heavy mass region around N=126, in order to guide theoretical models and to understand the formation of the third r-process peak at $A\sim195$. $Purpose:$ To measure both, $\beta$-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb and Bi isotopes beyond $N=126$. $Method:$ Ions of interest are produced by fragmentation of a $^{238}$U beam, selected and identified via the GSI-FRS fragment separator. A stack of segmented silicon detectors (SIMBA) is used to measure ion-implants and $\beta$-decays. An array of 30 $^3$He tubes embedded in a polyethylene matrix (BELEN) is used to detect neutrons with high efficiency and selectivity. A self-triggered digital system is employed to acquire data and to enable time-correlations. The latter are analyzed with an analytical model and results for the half-lives and neutron-branching ratios are derived using the binned Maximum-Likelihood method. $Results:$ Twenty new $\beta$-decay half-lives are reported for $^{204-206}$Au, $^{208-211}$Hg,$^{211-216}$Tl,$^{215-218}$Pb and $^{218-220}$Bi, nine of them for the first time. Neutron emission probabilities are reported for $^{210,211}$Hg and $^{211-216}$Tl. $Conclusions:$ The new $\beta$-decay half-lives are in good agreement with previous measurements in this region. The measured neutron emission probabilities are comparable or smaller than values predicted by global models like RHB+RQRPA.

Highlights

  • BackgroundThere have been measurements on roughly 230 nuclei that are β-delayed neutron emitters

  • Very-neutron-rich nuclei may emit one or more neutrons when they disintegrate via β decay

  • CABALLERO-FOLCH et al Conclusions: The new β-decay half-lives are in good agreement with previous measurements on nuclei in this region

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Summary

Background

There have been measurements on roughly 230 nuclei that are β-delayed neutron emitters They range from 8He up to 150La. Apart from 210Tl, with a branching ratio of only 0.007%, no other neutron emitter has been measured beyond A = 150. Purpose: To measure both β-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb, and Bi isotopes beyond N = 126. A self-triggered digital system is employed to acquire data and to enable time correlations. The latter were analyzed with an analytical model and results for the half-lives and neutron-branching ratios were derived by using the binned maximum-likelihood method. Results: Twenty new β-decay half-lives are reported for 204−206Au, 208–211Hg,211–216Tl,215–218Pb, and 218–220Bi, nine of them for the first time.

Conclusions
INTRODUCTION
EXPERIMENTAL SETUP AND ION IDENTIFICATION
Implantation and decay-detection system
DETERMINATION OF β-DECAY HALF-LIVES AND P1n VALUES
Reference analysis of 213Tl half-life
Neutron branching ratio for 213Tl
Thallium isotopes
Lead isotopes
Mercury isotopes
Gold isotopes
Bismuth isotopes
12 Background
SUMMARY AND DISCUSSION
Findings
CONCLUSIONS

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