ОГЛЯД РЕЗУЛЬТАТІВ ДОСЛІДЖЕНЬ ЗАБРУДНЕННЯ КАХОВСЬКОГО ВОДОСХОВИЩА ЦЕЗІЄМ-137 І СТРОНЦІЄМ-90, ЯКІ ПРОВОДИЛИСЬ ПІСЛЯ АВАРІЇ НА ЧОРНОБИЛЬСЬКІЙ АЕС (1986-1921 РР.)

Abstract

The available data on the state of radioactive contamination of water and bottom sediments of the Kakhovka Reservoir were analyzed in order to assess the possible deterioration of the quality of the environment based on the indicators of radioactive contamination in the zone of influence of the emergency discharge of water due to destruction of the Kakhovka NPP dam by the Russian military. Contamination of the Kakhovka Reservoir with 137Cs occurred mainly through the fallouts of this radionuclide with aerosols on the water surface in May 1986. A much smaller part of this radionuclide transported by water runoff directly from the headwaters of the Dnieper basin. Strontium-90 entered the reservoir exclusively by water pathway starting from October 1986. The steady trends of decreasing activity of both radionuclides in water has been observed since 1987. Approximately to 1996 137Cs activity concentrations had decreased to pre-accident level, 90Sr activity demonstrated a slow decrease and by 2022 remained slightly higher than pre-accidental level. The average levels of contamination of the Kakhovka reservoir bottom with 137Cs and 90Sr turned out to be the lowest compared to the other reservoirs of the Dnieper cascade. It was shown that in 1994 137Cs activity levels were 0.06 Ci/km2(2,2 kBq/m2) on 80% of the bottom surface (submerged former floodplain of the Dnieper) and were lower than on the territory adjacent to the reservoir. In the areas of silt accumulation (former channel of the Dnieper) 137Cs activity was on average three times higher. Balance calculations based on the data of radiation monitoring of water showed that the amount of 137Cs activity in the bottom sediments in the period 1987-2022 halved due to natural radioactive decay, the amount of 90Sr activity decreased by approximately 20%, since activity losses due to natural radioactive decay were partially compensated by the constant supply of this radionuclide with water runoff from the contaminated part of the catchment. After a catastrophic water leak from the reservoir, the Dnieper floodplain had exposed. According to the calculations, the average density of soil contamination of the ехposed areas with 137Cs does not exceed 0.03 Ci/km2 (1,1 kBq/m2), with 90Sr – less than 0.1 Ci/km2 (3,7 kBq/m2). Silt deposits of the former Dnieper channel, which had an increased level of 137Cs contamination, were re-suspended, probably, and carried out into the Dnipro-Bug estuary and further into the Black Sea. However, according to our assumptions, this should not have a negative effect on the radioecological state of the sea, because the 137Cs activity concentrations in the water of north-western part of the Black Sea were always 20-30 times higher than in the Dnieper water.