XY Antiferromagnet Research Articles

Continuous symmetry breaking in a two-dimensional Rydberg array.

Spontaneous symmetry breaking underlies much of our classification of phases of matter and their associated transitions1-3. The nature of the underlying symmetry being broken determines many of the qualitative properties of the phase; this is illustrated by the case of discrete versus continuous symmetry breaking. Indeed, in contrast to the discrete case, the breaking of a continuous symmetry leads to the emergence of gapless Goldstone modes controlling, for instance, the thermodynamic stability of the ordered phase4,5. Here, we realize a two-dimensional dipolar XY model that shows a continuous spin-rotational symmetry using a programmable Rydberg quantum simulator. We demonstrate the adiabatic preparation of correlated low-temperature states of both the XY ferromagnet and the XY antiferromagnet. In the ferromagnetic case, we characterize the presence of a long-range XY order, a feature prohibited in the absence of long-range dipolar interaction. Our exploration of the many-body physics of XY interactions complements recent works using the Rydberg-blockade mechanism to realize Ising-type interactions showing discrete spin rotation symmetry6-9.

Monte Carlo study of the phase diagram of layered XY antiferromagnet

The three-dimensional XY model is investigated in the presence of a uniform magnetic field applied in the X-direction. The nearest neighbour intraplanar interaction is considered ferromagnetic, and the interplanar nearest neighbour interaction is chosen to be antiferromagnetic. Starting from a high-temperature initial random spin configuration, the equilibrium phase of the system at any finite temperature was achieved by cooling the system using the Monte Carlo single spin-flip Metropolis algorithm with a random updating rule. The components of total magnetization and the sublattice magnetizations were calculated. The variance of the antiferromagnetic order parameter and the susceptibility have been calculated. In a specific range of relative strengths of interactions (antiferromagnetic/ferromagnetic) and the applied magnetic field, the system shows the equilibrium phase transitions at different temperatures. The phase diagrams (in the field-temperature plane) were obtained for different values of the relative interaction strengths. The ordered region bounded by the phase boundary was found to increase as the ratio of relative interaction strength increased. Furthermore, the maximum value of the susceptibility (χaym) was found to increase with the system size (L). For χaym∼Lγν, the exponent γ/ν has been estimated to be 2.10 ±0.11.

The antiferromagnetic xy model on the triangular lattice: topological singularities

We study the discrete-to-continuum variational limit of the antiferromagnetic XY model on the two-dimensional triangular lattice in the vortex regime. Within this regime, the spin system cannot overcome the energetic barrier of chirality transitions, hence one of the two chirality phases is prevalent. We find the order parameter that describes the vortex structure of the spin field in the majority chirality phase and we compute explicitly the $\Gamma$-limit of the scaled energy, showing that it concentrates on finitely many vortex-like singularities of the spin field.

Signatures for Berezinskii-Kosterlitz-Thouless critical behavior in the planar antiferromagnet BaNi2V2O8

We investigate the critical properties of the spin-$1$ honeycomb antiferromagnet BaNi$_2$V$_2$O$_8$, both below and above the ordering temperature $T_N$ using neutron diffraction and muon spin rotation measurements. Our results characterize BaNi$_2$V$_2$O$_8$ as a two-dimensional (2D) antiferromagnet across the entire temperature range, displaying a series of crossovers from 2D Ising-like to 2D XY and then to 2D Heisenberg behavior with increasing temperature. In particular, the extracted critical exponent of the order parameter reveals a narrow temperature regime close to $T_N$, in which the system behaves as a 2D XY antiferromagnet. Above $T_N$, evidence for Berezinsky-Kosterlitz-Thouless behavior driven by vortex excitations is obtained from the scaling of the correlation length. Our experimental results are in accord with classical and quantum Monte Carlo simulations performed for microscopic magnetic model Hamiltonians for BaNi$_2$V$_2$O$_8$.

The antiferromagnetic XY model on the triangular lattice: chirality transitions at the surface scaling

We study the discrete-to-continuum variational limit of the antiferromagnetic XY model on the two-dimensional triangular lattice. The system is fully frustrated and displays two families of ground states distinguished by the chirality of the spin field. We compute the Gamma -limit of the energy in a regime which detects chirality transitions on one-dimensional interfaces between the two admissible chirality phases.

Finite-temperature dynamics and the role of disorder in nearly critical Ni(Cl1−xBrx)2·4SC(NH2)2

Inelastic neutron scattering is used to investigate the temperature dependence of spin correlations in the 3-dimensional XY antiferromagnet Ni(Cl$_{1-x}$Br$_x$)$_2$$\cdot$4SC(NH$_2$)$_2$, $ x = 0.14(1)$, tuned close to the chemical-composition-induced soft-mode transition. The local dynamic structure factor shows $\hbar\omega/T$ scaling behavior characteristic of a quantum critical point. The deviation of the measured critical exponent from spin wave theoretical expectations are attributed to disorder. Another effect of disorder is local excitations above the magnon band. Their energy, structure factor and temperature dependence are well explained by simple strong-bond dimers associated with Br-impurity sites.

Random-bond disorder in two-dimensional noncollinear XY antiferromagnets: From quasi-long-range order to spin glass

We study effects of quenched bond disorder in frustrated easy-plane antiferromagnets in two space dimensions, using a combination of analytical and numerical techniques. We consider local-moment systems which display non-collinear long-range order at zero temperature, with the antiferromagnetic triangular-lattice XY model as a prime example. We show that (i) weak bond disorder transforms the clean ground state into a state with quasi-long-range order, and (ii) strong bond disorder results in a short-range-ordered glassy ground state. Using extensive Monte Carlo simulations, we also track the fate of the quasi-long-range-ordered phase at finite temperature and the associated Kosterlitz-Thouless-like transition. Making contact with previous studies of disordered XY models, we discuss similarities and differences concerning the interplay of disorder and frustration. Our results are also of relevance to non-collinear Heisenberg magnets in an external magnetic field.

Phase transitions in the frustrated antiferromagnetic XY model on the triangular lattice

Phase transitions and thermodynamics properties of the frustrated antiferromagnetic XY (FAXY) model have been investigated near the two transition temperatures. We found that the Kosterlitz-Thouless (KT) transition corresponding to the rotational U(1) symmetry breaking and the Ising-like (I) transition corresponding to the reflection Z2 symmetry breaking occur at two-separate transition temperatures, Tkt < TI. These temperatures lie close to each other, however in our results the separation is obvious. Our results show the order parameters as a function of temperature and we also estimate the critical exponents, β, α, γ, η and ν. The critical exponent ν indicates that the Ising-like transition is inconsistent with the Ising universality class.

Ising-XY Transition in Three-dimensional Frustrated Antiferromagnets with Collinear Spin Ordering

Using Monte Carlo simulations, we study the critical behavior of two models of frustrated XY antiferromagnets with a collinear spin ordering and with an additional twofold degeneracy of the ground state. We consider a classic antiferromagnet on a body-centered cubic lattice with an additional antiferromagnetic exchange interaction between next-nearest spins, and a ferromagnet with an extra antiferromagnetic intralayer exchange. In both models, a single first-order transition on the discrete and continuous order parameters is found. Observed critical pseudo-exponents are in agreement with exponents of XY magnets with a planar spin ordering like a stacked-triangular antiferromagnet and helimagnets belonging to the same symmetry class.

Frustrated bilayer spin one XY model on the honeycomb lattice

The spin-one honeycomb bilayer XY antiferromagnet has been studied taking into account the effect of the next-near neighbor J2 exchange interactions and single-ion easy plane anisotropy, using a flavor wave theory. We found that, at a critical point αC=13.8, where α=J⊥/J1 is the ratio between the interlayer J⊥ to the intralayer near neighbor J1 exchange interaction, the system shows a quantum phase transition from an Néel ordered phase to a paramagnetic phase. The phase diagram at zero temperature is presented.

Nonequilibrium selection of magnetic order in a driven triangular XY antiferromagnet

We show that a weak periodic drive removes the accidental degeneracy in the ground state of the XY antiferromagnet on the triangular lattice in a uniform static magnetic field. The underlying mechanism involves adding a small periodically modulated component to the magnetic field, which influences finite-frequency modes to generate an effective potential for the accidental pseudo-Goldstone mode. This selection can be arranged to compete with the degeneracy lifting via the thermal order by disorder mechanism. This yields a non-equilibrium phase transition as the relative strength of the two mechanisms is tuned by varying temperature. This proposal may be amenable to experimental realization, in particular as applying the field is noninvasive, and no complex bath engineering is required.

Finite Correlation Length Scaling in Lorentz-Invariant Gapless iPEPS Wave Functions

It is an open question how well tensor network states in the form of an infinite projected entangled pair states (iPEPS) tensor network can approximate gapless quantum states of matter. Here we address this issue for two different physical scenarios: i) a conformally invariant $(2+1)d$ quantum critical point in the incarnation of the transverse field Ising model on the square lattice and ii) spontaneously broken continuous symmetries with gapless Goldstone modes exemplified by the $S=1/2$ antiferromagnetic Heisenberg and XY models on the square lattice. We find that the energetically best wave functions display {\em finite} correlation lengths and we introduce a powerful finite correlation length scaling framework for the analysis of such finite-$D$ iPEPS states. The framework is important i) to understand the mild limitations of the finite-$D$ iPEPS manifold in representing Lorentz-invariant, gapless many body quantum states and ii) to put forward a practical scheme in which the finite correlation length $\xi(D)$ combined with field theory inspired formulae can be used to extrapolate the data to infinite correlation length, i.e. to the thermodynamic limit. The finite correlation length scaling framework opens the way for further exploration of quantum matter with an (expected) Lorentz-invariant, massless low-energy description, with many applications ranging from condensed matter to high-energy physics.

Cluster-Glass Phase in Pyrochlore XY Antiferromagnets with Quenched Disorder.

We study the impact of quenched disorder (random exchange couplings or site dilution) on easy-plane pyrochlore antiferromagnets. In the clean system, order by disorder selects a magnetically ordered state from a classically degenerate manifold. In the presence of randomness, however, different orders can be chosen locally depending on details of the disorder configuration. Using a combination of analytical considerations and classical MonteCarlo simulations, we argue that any long-range-ordered magnetic state is destroyed beyond a critical level of randomness where the system breaks into magnetic domains due to random exchange anisotropies, becoming, therefore, a glass of spin clusters, in accordance with the available experimental data. These random anisotropies originate from off-diagonal exchange couplings in the microscopic Hamiltonian, establishing their relevance to other magnets with strong spin-orbit coupling.

Phase transitions of the frustrated bilayer spin one XY model

In this paper we use the SU(3) Schwinger boson representation, followed by a mean field decoupling, to study the disordered phases of the bilayer spin one quantum XY antiferromagnet on a square lattice with next near neighbor and a single ion anisotropy. The phase diagram at zero temperature is obtained. The ratio η=J⊥/J1 between the interlayer J⊥ to the intralayer near neighbor J1 exchange interactions exhibits a quantum phase transition at a critical ratio ηc=21.725 that separates the small- η Nèel phase from the large η quantum disordered paramagnet. The effect of next near neighbor interactions is discussed. The Neel phase is studied using a self consistent harmonic approximation that takes into account topological effects.

Control of the Effective Free-Energy Landscape in a Frustrated Magnet by a Field Pulse.

Thermal fluctuations can lift the degeneracy of a ground state manifold, producing a free-energy landscape without accidentally degenerate minima. In a process known as order by disorder, a subset of states incorporating symmetry breaking may be selected. Here, we show that such a free-energy landscape can be controlled in a nonequilibrium setting as the slow motion within the ground state manifold is governed by the fast modes out of it. For the paradigmatic case of the classical pyrochlore XY antiferromagnet, we show that a uniform magnetic field pulse can excite these fast modes to generate a tunable effective free-energy landscape with minima at thermodynamically unstable portions of the ground state manifold.

The complexity of antiferromagnetic interactions and 2D lattices

Estimation of the minimum eigenvalue of a quantum Hamiltonian can be formalised as the Local Hamiltonian problem. We study the natural special case of the Local Hamiltonian problem where the same 2-local interaction, with differing weights, is applied across each pair of qubits. First we consider antiferromagnetic/ferromagnetic interactions, where the weights of the terms in the Hamiltonian are restricted to all be of the same sign. We show that for symmetric 2-local interactions with no 1-local part, the problem is either QMA-complete or in StoqMA. In particular the antiferromagnetic Heisenberg and antiferromagnetic XY interactions are shown to be QMA-complete. We also prove StoqMA-completeness of the antiferromagnetic transverse field Ising model. Second, we study the Local Hamiltonian problem under the restriction that the interaction terms can only be chosen to lie on a particular graph. We prove that nearly all of the QMA-complete 2-local interactions remain QMA-complete when restricted to a 2D square lattice. Finally we consider both restrictions at the same time and discover that, with the exception of the antiferromagnetic Heisenberg interaction, all of the interactions which are QMA-complete with positive coefficients remain QMA-complete when restricted to a 2D triangular lattice.

Single-ion properties of theSeff=12XY antiferromagnetic pyrochloresNaA′Co2F7(A′=Ca2+, Sr2+)

The antiferromagnetic pyrochlore material NaCaCo$_2$F$_7$ is a thermal spin liquid over a broad temperature range (~ 140 K down to $T_F = 2.4 $K), in which magnetic correlations between Co$^{2+}$ dipole moments explore a continuous manifold of antiferromagnetic XY states. The thermal spin liquid is interrupted by spin freezing at a temperature that is ~ 2 % of the mean field interaction strength, leading to short range static XY clusters with distinctive relaxation dynamics. Here we report the low energy inelastic neutron scattering response from the related compound NaSrCo$_2$F$_7$, confirming that it hosts the same static and dynamic spin correlations as NaCaCo$_2$F$_7$. We then present the single-ion levels of Co$^{2+}$ in these materials as measured by inelastic neutron scattering. An intermediate spin orbit coupling model applied to an ensemble of trigonally distorted octahedral crystal fields accounts for the observed transitions. The single-ion ground state of Co$^{2+}$ is a Kramers doublet with a strongly XY-like $g$-tensor ($g_{xy}/g_{z}$ ~ 3). The local disorder inherent from the mixed pyrochlore $A$ sites (Na$^{+}$/Ca$^{2+}$ and Na$^{+}$/Sr$^{2+}$) is evident in these measurements as exaggerated broadening of some of the levels. A simple model that reproduces the salient features of the single-ion spectrum produces approximately 8.4 % and 4.1 % variation in the $z$ and $xy$ components of the $g$-tensor, respectively. This study confirms that an $S_{eff} =1/2$ model with XY antiferromagnetic exchange and weak exchange disorder serves as a basic starting point in understanding the low temperature magnetic behavior of these strongly frustrated magnets.

Anisotropic XY antiferromagnets in a field

Classical anisotropic XY antiferromagnets in a field on square and simple cubic lattices are studied using mainly Monte Carlo simulations. While in two dimensions the ordered antiferromagnetic and spin--flop phases are observed to be separated by a narrow disordered phase, a line of direct transitions of first order between the two phases and a bicritical point are found in three dimensions. Results are compared to previous findings.

Order by virtual crystal field fluctuations in pyrochlore XY antiferromagnets

Conclusive evidence of order by disorder is scarce in real materials. Perhaps one of the strongest cases presented has been for the pyrochlore XY antiferromagnet Er2Ti2O7, with the ground state selection proceeding by order by disorder induced through the effects of quantum fluctuations. This identification assumes the smallness of the effect of virtual crystal field fluctuations that could provide an alternative route to picking the ground state. Here we show that this order by virtual crystal field fluctuations is not only significant, but competitive with the effects of quantum fluctuations. Further, we argue that higher-multipolar interactions that are generically present in rare-earth magnets can dramatically enhance this effect. From a simplified bilinear-biquadratic model of these multipolar interactions, we show how the virtual crystal field fluctuations manifest in Er2Ti2O7 using a combination of strong coupling perturbation theory and the random phase approximation. We find that the experimentally observed psi2 state is indeed selected and the experimentally measured excitation gap can be reproduced when the bilinear and biquadratic couplings are comparable while maintaining agreement with the entire experimental spin-wave excitation spectrum. Finally, we comments on possible tests of this scenario and discuss implications for other order-by-disorder candidates in rare-earth magnets.

Complexity of the XY antiferromagnet at fixed magnetization

We prove that approximating the ground energy of the antiferromagnetic XY model on a simple graph at fixed magnetization (given as part of the instance specification) is QMA-complete. To show this, we strengthen a previous result by establishing QMAcompleteness for approximating the ground energy of the Bose-Hubbard model on simple graphs. Using a connection between the XY and Bose-Hubbard models that we exploited in previous work, this establishes QMA-completeness of the XY model.