X-ray Yield Research Articles

Leveraging Machine Learning for Advanced Nanoscale X-ray Analysis: Unmixing Multicomponent Signals and Enhancing Chemical Quantification.

Energy dispersive X-ray (EDX) spectroscopy in the transmission electron microscope is a key tool for nanomaterials analysis, providing a direct link between spatial and chemical information. However, using it for precisely determining chemical compositions presents challenges of noisy data from low X-ray yields and mixed signals from phases that overlap along the electron beam trajectory. Here, we introduce a novel method, non-negative matrix factorization based pan-sharpening (PSNMF), to address these limitations. Leveraging the Poisson nature of EDX spectral noise and binning operations, PSNMF retrieves high-quality phase spectral and spatial signatures via consecutive factorizations. After validating PSNMF with synthetic data sets of different noise levels, we illustrate its effectiveness on two distinct experimental cases: a nanomineralogical lamella, and supported catalytic nanoparticles. Not only does PSNMF obtain accurate phase signatures, but data sets reconstructed from the outputs have demonstrably lower noise and better fidelity than from the benchmark denoising method of principle component analysis.

Characterization of the SIDDHARTA-2 Setup via the Kaonic Helium Measurement

The aim of the SIDDHARTA-2 experiment is to perform the first measurement ever of the width and shift induced by the strong interaction to the 2p→1s energy transition of kaonic deuterium. This ambitious goal implies a challenging task due to the very low X-ray yield of kaonic deuterium, which is why an accurate and thorough characterization of the experimental apparatus is mandatory before starting the data-taking campaign. Helium-4 is an excellent candidate for this characterization since it exhibits a high yield in particular for the 3d→2p transition, roughly 100 times greater than that of the kaonic deuterium. The ultimate goal of the work reported in this paper is to study the performances of the full experimental setup in view of the kaonic deuterium measurement. This is carried out by measuring the values of the shift and the width for the 3d→2p energy transition of kaonic helium-4, induced by the strong interaction. The values obtained for these quantities, for a total integrated luminosity of ∼31/pb, are ε2p=2.0±1.2(stat)±1.5(syst)eV and Γ2p=1.9±5.7(stat)±0.7(syst)eV. The results, compared to the value of the shift measured by the SIDDHARTA experiment ε2p=0±6(stat)±2(syst)eV, show a net enhancement of the resolution of the apparatus, providing strong evidence of the potential to perform the challenging measurement of the kaonic deuterium.

Impact of electrical aging on x-ray image quality and dose rate with vertically aligned carbon nanotube based cold cathode electron beam (C-beam)

The adoption of vertically aligned carbon nanotubes (VACNTs) as electron emitters in x-ray generation has opened a new path for medical imaging technology advancement. With their outstanding electron emission capabilities, VACNTs provide a distinct advantage in miniaturizing and improving the performance of x-ray devices. This research focuses on the effect of electrical aging on x-ray imaging quality and the dose rate while using VACNTs as the electron source. The study includes a thorough examination of the electrical aging effects on VACNT-based x-ray systems, with an emphasis on changes in emission characteristics, beam stability, and the resulting variations in x-ray output. Experiment results show that electrical aging has a considerable impact on the performance of VACNT-based x-ray sources, with visible changes in electron emission parameters and subsequent consequences on x-ray imaging quality. Furthermore, the study investigates the relationship between electrical aging and the x-ray dose rate, providing vital insights into radiation exposure optimization in medical diagnostics.

Intraoperative radiation therapy with 50kV x-rays: A multi-institutional review.

This report covers clinical implementation of a low kV intraoperative radiation therapy (IORT) program with the INTRABEAM® System (Carl Zeiss Meditec AG, Jena, Germany). Based on collective user experience from eight institutions, we discuss best methods of INTRABEAM quality assurance (QA) tests, commissioning measurements, clinical workflow, treatment planning, and potential avenues for research. The guide provides pertinent background information and clinical justification for IORT. It describes the INTRABEAM system and commissioning measurements along with a TG100 risk management analysis to ensure safety and accuracy of the IORT program. Following safety checks, dosimetry measurements are performed for verification of field flatness and symmetry, x-ray output, and depth dose. Also discussed are dose linearity checks, beam isotropy, ion chamber measurements, calibration protocols, and in-vivo dosimetry with optically stimulated luminescence dosimeters OSLDs, and radiochromic film. Emphasis is placed on the importance of routine QA procedures (daily, monthly, and annual) performed at regular intervals for a successful IORT program. For safe and accurate dose delivery, tests of important components of IORT clinical workflow are emphasized, such as, dose prescription, pre-treatment QA, treatment setup, safety checks, radiation surveys, and independent checks of delivered dose. Challenges associated with in-vivo dose measurements are discussed, along with special treatment procedures and shielding requirements. The importance of treatment planning in IORT is reviewed with reference to a Monte Carlo-based commercial treatment planning system highlighting its main features and limitations. The report concludes with suggested topics for research including CT-based image-guided treatment planning and improved prescription dose accuracy. We hope that this multi-institutional report will serve as a guidance document on the clinical implementation and use of INTRABEAM IORT.

Long-term Reproducibility Evaluation of Fluoroscopy Dose Rate in Angiography Equipment

Diagnostic reference levels (DRLs) are defined as fluoroscopic dose rate measurements that are used for patient dose management in angiography. It is recommended that DRLs be measured at least once a year. This study aimed to evaluate the long-term fluctuations of fluoroscopic dose rate in an angiography system. An unconnected X-ray output analyzer was used to measure the fluoroscopic dose rate (air kerma rate) at the patient's entrance reference point for a specific angiography system. The target period was from 2015 to 2022, and four measurements per year were made. First, the fluoroscopic dose rate was measured, and the average value and standard deviation for the target period were calculated. Next, the uncertainty of the measured values and the coefficient of variation were calculated. Finally, we calculated the fluoroscopic dose rate measurement error. The average±standard deviation of the fluoroscopic dose rate was 353.29±9.11 µGy/s. The maximum uncertainty and coefficient of variation for each year were 5.41 µGy/s and 0.03, respectively. The maximum measurement error was 4.67%, where the mean measured value was taken as the true value. The fluctuation in the measured value of the fluoroscopic dose rate by an angiography system for 8 years is within ±5%, indicating stable X-ray output.

Kaonic atoms with SIDDHARTA-2 at the DAΦNE collider

The most important information still missing in the field of the low-energy antikaon-nucleon inter actions studies is the experimental determination of the hadronic energy shift and width of kaonic deuterium. This measurement will be performed by the SIDDHARTA-2 experiment, installed at the DAΦNE collider and presently in data taking campaign. The precise measurement of the shift and width of the 1s level with respect to the purely electromagnetic calculated values, generated by the presence of the strong interaction, through the measurement of the X-ray transitions to this level, in kaonic hydrogen, was performed by the SIDDHARTA collaboration, the kaonic deuterium is underway by SIDDHARTA-2. These measurement will allow the first precise experimental extraction of the isospin dependent antikaon-nucleon scattering lengths, funda mental quantities for understanding low-energy QCD in the strangeness sector. The experimental challenge of the kaonic deuterium measurement is the very small X-rays yield, the even larger width (compared to kaonic hy drogen), and the difficulty to perform X-rays spectroscopy with weak signals in the high radiation environment of DAΦNE. It was, therefore, crucial to develop a new apparatus involving large-area X-rays detector system, to optimize the signal and to control and by improve the signal-to-background ratio by gaining in solid angle, increasing the timing capability, and as well implementing additional charge particle tracking veto systems.

Flux and estimated spectra from a low-intensity laser-driven X-ray source

Abstract Laser-driven X-rays as probes for high-energy-density physics spans an extremely large parameter space with laser intensities varying by 8 orders of magnitude. We have built and characterized a soft X-ray source driven by a modest intensity laser of 4 × 1013 W/cm2. Emitted X-rays were measured by diamond radiation detectors and a filtered soft X-ray camera. A material-dependence study on Al, Ti, stainless steel alloy 304, Fe, Cu and Sn targets indicated 5-μm-thick Cu foils produced the highest X-ray yield. X-ray emission in the laser direction and emission in the reverse direction depend strongly on the foil material and the thickness due to the opacity and hydrodynamic disassembly time. The time-varying X-ray signals are used to measure the material thinning rate and is found to be ∼1.5 μm/ns for the materials tested implying thermal temperature around 0.6 eV. The X-ray spectra from Cu targets peaks at ∼2 keV with no emission >4 keV and was estimated using images with eight different foil filters. One-dimensional hydrodynamic and spectral calculations using HELIOS-CR provide qualitative agreement with experimental results. Modest intensity lasers can be an excellent source for nanosecond bursts of soft X-rays.

X-ray-induced scintillation properties of Nd-doped calcium niobium gallium garnet single crystals

0.1, 0.5, and 1 % Nd-doped Ca3Nb1.6875Ga3.1875O12 (CNGG) single crystals were successfully synthesized by the Floating Zone method. The optical and scintillation characteristics in ultraviolet–near-infrared (NIR) regions were investigated. All the CNGG crystals showed emissions at 900, 1060, and 1350 nm, which correspond to the typical electronic transitions of Nd3+. The decay times of 200–220 μs were obtained by an approximation of decay curves. The values were valid as the 4f–4f transitions of Nd3+. When relationships between X-ray irradiation dose-rate and output signals in NIR ranges were evaluated, all the prepared samples exhibited good linear responses. The lowest detectable dose-rate in prepared samples was observed by measuring with the 0.5 % Nd-doped sample, and the value was 0.006 Gy/h.

Simulation of x-ray bremsstrahlung generation under vacuum heating of solid target electrons

An extended Brunel model of hot electron generation in nonrelativistic laser-plasma interactions is considered. The model takes into account the permittivity of the surface plasma and the energy absorbed by electrons accelerated by the electric field components perpendicular and parallel to the target. A model for the generation of x-ray bremsstrahlung in the case of a Gaussian laser beam is presented. It is shown that the influence of electron motion parallel to the plasma surface on the absorbed intensity becomes distinguishable only at relatively low absolute values of the permittivity. Calculations of the dependences of the yield of hard bremsstrahlung x-rays on the angle of incidence of laser radiation and on the energy interval in which the yield of bremsstrahlung is measured are in qualitative agreement with the experimental data, if we assume that the electron concentration in the skin layer is relatively low (approximately 5–7 times the critical concentration).

Population synthesis of Be X-ray binaries: metallicity dependence of total X-ray outputs

ABSTRACT X-ray binaries (XRBs) are thought to regulate cosmic thermal and ionization histories during the Epoch of Reionization and Cosmic Dawn (z ∼ 5–30). Theoretical predictions of the X-ray emission from XRBs are important for modelling such early cosmic evolution. Nevertheless, the contribution from Be-XRBs, powered by accretion of compact objects from decretion discs around rapidly rotating O/B stars, has not been investigated systematically. Be-XRBs are the largest class of high-mass XRBs (HMXBs) identified in local observations and are expected to play even more important roles in metal-poor environments at high redshifts. In light of this, we build a physically motivated model for Be-XRBs based on recent hydrodynamic simulations and observations of decretion discs. Our model is able to reproduce the observed population of Be-XRBs in the Small Magellanic Cloud with appropriate initial conditions and binary stellar evolution parameters. We derive the X-ray output from Be-XRBs as a function of metallicity in the (absolute) metallicity range Z ∈ [10−4, 0.03] with a large suite of binary population synthesis (BPS) simulations. The simulated Be-XRBs can explain a non-negligible fraction ($\gtrsim 30{{\ \rm per\ cent}}$) of the total X-ray output from HMXBs observed in nearby galaxies for Z ∼ 0.0003–0.02. The X-ray luminosity per unit star formation rate from Be-XRBs in our fiducial model increases by a factor of ∼8 from Z = 0.02 to Z = 0.0003, which is similar to the trend seen in observations of all types of HMXBs. We conclude that Be-XRBs are potentially important X-ray sources that deserve greater attention in BPS of XRBs.

Prediction on X-ray output of free electron laser based on artificial neural networks

Knowledge of x-ray free electron lasers’ (XFELs) pulse characteristics delivered to a sample is crucial for ensuring high-quality x-rays for scientific experiments. XFELs’ self-amplified spontaneous emission process causes spatial and spectral variations in x-ray pulses entering a sample, which leads to measurement uncertainties for experiments relying on multiple XFEL pulses. Accurate in-situ measurements of x-ray wavefront and energy spectrum incident upon a sample poses challenges. Here we address this by developing a virtual diagnostics framework using an artificial neural network (ANN) to predict x-ray photon beam properties from electron beam properties. We recorded XFEL electron parameters while adjusting the accelerator’s configurations and measured the resulting x-ray wavefront and energy spectrum shot-to-shot. Training the ANN with this data enables effective prediction of single-shot or average x-ray beam output based on XFEL undulator and electron parameters. This demonstrates the potential of utilizing ANNs for virtual diagnostics linking XFEL electron and photon beam properties.

The SIDDHARTA-2 Veto-2 system for X-ray spectroscopy of kaonic atoms at DAΦNE

The Veto-2 is a fundamental component of a multiple-stage veto system for the SIDDHARTA-2 experiment installed at the DAΦNE collider at INFN-LNF in Italy. It was developed to improve the signal-to-background ratio for the challenging measurement of X-ray transitions to the fundamental level in kaonic deuterium. Its purpose is the suppression of hadronic background in the form of Minimum Ionizing Particles by using the topological correlation between signals in the X-ray and Veto-2 detectors. The Veto-2 system consists of a barrel of plastic scintillators read out by Silicon Photomultipliers. The system performed its first successful test run within the apparatus with a helium-4 target in 2022. The efficiency of the Veto-2 was determined and found to be 0.62 ± 0.01. The Veto-2 improved the signal-to-background ratio for the kaonic helium-4 Lα measurement by ∼ 16%, which is crucial due to the low expected X-ray yield of kaonic deuterium.

Study on chemical forms of aluminum in tea leaves using micro-PIXE method

Elemental analysis of the epidermis of tea leaves was performed using the micro-beam particle-induced X-ray emission (micro-PIXE) method. The ratios of the X-ray yields of silicon (Si), potassium (K), calcium (Ca), and manganese (Mn) to that of aluminum (Al) in the cell wall of epidermal cells of tea leaves were determined. The ratio of Si to Al X-ray yields agreed within a range of 11% in the four samples measured in this study. On the other hand, the ratio of the X-ray yields of K, Ca, and Mn to Al varied from 41% to 87%. This result suggests that Al forms compounds with Si in tea leaves.

Self-Adjusting Optical Systems Based on Reinforcement Learning

Progress in the field of machine learning has enhanced the development of self-adjusting optical systems capable of autonomously adapting to changing environmental conditions. This study demonstrates the concept of self-adjusting optical systems and presents a new approach based on reinforcement learning methods. We integrated reinforcement learning algorithms into the setup for tuning the laser radiation into the fiber, as well as into the complex for controlling the laser-plasma source. That reduced the dispersion of the generated X-ray signal by 2–3 times through automatic adjustment of the position of the rotating copper target and completely eliminated the linear trend arising from the ablation of the target surface. The adjustment of the system was performed based on feedback signals obtained from the spectrometer, and the movement of the target was achieved using a neural network-controlled stepper motor. As feedback, the second harmonic of femtosecond laser radiation was used, the intensity of which has a square root dependence on the X-ray yield. The developed machine learning methodology allows the considered systems to optimize their performance and adapt in real time, leading to increased efficiency, accuracy, and reliability.

Effect of shape of automatic dose rate control and wedge compensation filter on radiation dose in an angiography system with a flat-panel detector.

The purpose was to investigate air-kerma area product (PKA) and entrance surface air-kerma rate ([Formula: see text]a,e) on the effect of the shape of automatic dose rate control (ADRC) in the presence of a wedge compensation filter. We compared and evaluated the variability of the X-ray output using a combination of wedge compensation filters and the ADRC. Two ADRC shapes (round and square) and three poly-methyl-methacrylate thicknesses (15, 20, and 25cm) were used. A wedge compensation filter was inserted 2cm at a time, up to 6cm. When the wedge compensation filter was inserted to 6 cm for 20cm of poly-methyl-methacrylate, the X-ray output fluctuated significantly. The PKA was reduced by 39% when the wedge compensation filter was inserted to 6 cm and by 59% when it was inserted to 4cm under round-type for 20cm poly-methyl-methacrylate. The shape of the ADRC affects [Formula: see text]a,e and PKA.

Neural-network–based algorithm for the inverse problem of measuring K-shell ionization cross-sections of Si induced by 3–25 keV electrons and 4.5–9 keV positrons using the thick-target method

In this study, a neural network method is proposed for solving the inverse problem in the measurement of inner-shell ionization cross-sections using the thick-target method. It was applied to calculate the K-shell ionization cross-section of silicon (Si) from positron impacts in the energy range from 4.5 to 9 keV, using a Monte Carlo simulation program called PENELOPE to construct a comprehensive characteristic X-ray yield and cross-section database, serving as a foundation for training the neural network. The experimental values are compared with those obtained using regularization, yield differential, and distorted-wave Born approximation (DWBA) theoretical models. Our findings reveal that the cross-section results obtained from all three algorithms are in good agreement with the theoretical DWBA values within the error range. Moreover, our study highlights the superiority of the neural network algorithm in solving ill-posed problems, compared with traditional regularization algorithms and the yield differential method. Furthermore, we re-analyse the experimental data of electron-induced ionization cross-sections on a pure thick Si target in the energy range from 3 to 25 keV, which were originally obtained by Zhu et al. who used a regularization method. The reprocessed cross-sections obtained in this study exhibit good agreement with the reported results within the error range. To the best of our knowledge, this is the first experimental report of the K-shell ionization cross-sections of Si from positron impact.

Comparison of round and knife-edge-like cathodes on gas-puff implosions.

Preionization is believed to play an important role on the implosion of gas-puff Z pinches. Some experiments have used an external preionization source, e.g., UV light or electron beam. In contrast, other experiments rely completely on over voltage breakdown by the own generator's voltage pulse. However, this approach lacks shot-to-shot reproducibility since self-breakdown is mainly a stochastic process. In this work, we performed a systematic study on self-breakdown using two different cathode geometries: (i) a smooth, round cathode to provide a homogeneous electric field, (ii) a sharp, knife-edge-like geometry to enhance the electric field locally and eventually electron emission. The experiments were carried out on the Llampudken current generator, which provides a current pulse of ∼400kA amplitude and 200ns rise time (10%-90%). We implemented gated XUV imaging, filtered diodes and time-integrated x-ray imaging to obtain information about the implosion as well as the stagnation phase for the two cathode geometries. We found that erosion of the knife-edge cathode might be a serious problem, and we had to replace it every 15 shots. On the other hand, the round cathode lasted for the whole series of experiments. We also measured a more reproducible and larger peak current for the knife cathode. From the photo-conductive detectors we observed that even if the round cathode might present shots with higher x-ray yield compared to the knife cathode, dispersion is almost twice as large. Moreover, after a statistic analysis, it is demonstrated that the dispersion in the yield is due solely to differences imposed by the cathodes and not to variations in the driver, as no correlation was found between them. We found that in order to fit the experimental data with the snowplow model, only ∼60% of the total mass is compressed in the knife cathode while ∼20% for the round one, highlighting the importance of the cathode and preionization. Therefore, we conclude that the use of the knife cathode increases the reproducibility of the experiment in comparison with the round cathode.

Simulations of collisional effects in an inner-shell solid-density Mg X-ray laser.

Inner-shell [Formula: see text] X-ray lasers have been created by pumping gaseous, solid, and liquid targets with the intense X-ray output of free-electron lasers (FELs). For gaseous targets lasing relies on the creation of [Formula: see text]-shell core holes on a time-scale short compared with filling via Auger decay. In the case of solid and liquid density systems, collisional effects will also be important, affecting not only populations but also line-widths, both of which impact the degree of overall gain, and its duration. However, to date, such collisional effects have not been extensively studied. We present here initial simulations using the CCFLY code of inner-shell lasing in solid-density Mg, where we self-consistently treat the effects of the incoming FEL radiation and the atomic kinetics of the Mg system, including radiative, Auger and collisional effects. We find that the combination of collisional population of the lower states of the lasing transitions and broadening of the lines precludes lasing on all but the [Formula: see text] of the initially cold system. Even assuming instantaneous turning on of the FEL pump, we find the duration of the gain in the solid system to be sub-femtosecond. This article is part of the theme issue 'Dynamic and transient processes in warm dense matter'.

Increase in the Yield of X-rays and Terahertz Radiation from a Thin Foil Irradiated by Femtosecond Laser Pulses

Increase in the Yield of X-rays and Terahertz Radiation from a Thin Foil Irradiated by Femtosecond Laser Pulses

Correlation between the Surface Undulation and Luminescence Characteristics in Semi-Polar 112¯2 InGaN/GaN Multi-Quantum Wells

Surface undulation was formed while growing InGaN/GaN multi-quantum wells on a semi-polar m-plane (1–100) sapphire substrate. Two distinct facets, parallel to 112¯2 and 011¯1, were formed in the embedded multi-quantum wells (MQWs). The structural and luminescence characteristics of the two facets were investigated using transmission electron microscopy equipped with cathodoluminescence. Those well-defined quantum wells, parallel and slanted to the growth plane, showed distinct differences in indium incorporation from both the X-ray yield and the contrast difference in annular darkfield images. Quantitative measurements of concentration in 011¯1 MQWs show an approximately 4 at% higher indium incorporation compared to the corresponding 112¯2 when the MQWs were formed under the same growth condition.