Wildfires in western US forests increased over the last two decades, resulting in elevated solid and nutrient loadings to streams, and occasionally threatening drinking water supplies. We demonstrated that a linked LANDIS (LANDscape DIsturbance and Succession)-VELMA (Visualizing Ecosystem Land Management Assessments) modeling approach can simulate wildland fire effects on water quality using the 2002 Colorado Hayman Fire. Utilizing LANDIS-II's forest landscape model to simulate forest composition and VELMA's eco-hydrologic model to simulate pre- and post-fire water quantity and quality, the best calibration performance yielded a Nash-Sutcliffe Efficiency (NSE) of 0.621 during 2000–2006 (most optimal annual - 0.921) in comparison to North American Land Data Assimilation System (NLDAS) runoff. Pre-fire modeled runoff, nitrate, and surface water temperature (SWT) correlated with observations. Simulated post-fire runoff (229%) and SWT (20.6%) were elevated relative to pre-fire, with nitrate concentrations 34 times greater than the aquatic life threshold (0.01 mg N/L).