Water Vapor Differential Absorption Lidar Research Articles

Evaluating the representation of Arctic cirrus solar radiative effects in the Integrated Forecasting System with airborne measurements

Abstract. In two case studies, airborne measurements of broadband solar irradiances above and below Arctic cirrus are compared to simulations of the Integrated Forecasting System (IFS) operated by the European Centre for Medium-Range Weather Forecasts (ECMWF) using offline runs of ECMWF's operational radiation scheme, “ecRad”. Furthermore, independent of the solar irradiances, cirrus properties are derived from collocated airborne active remote sensing observations to evaluate the optical and microphysical parameterizations in ecRad. The data were collected in the central Arctic over sea ice (81–90° N) with instrumentation installed aboard the High Altitude LOng range research aircraft (HALO) during a campaign in March and April 2022. Among others, the HALO instrumentation included upward- and downward-looking pyranometers to measure broadband solar irradiances, a cloud radar, and a multi-wavelength water vapour differential absorption lidar. Extended horizontal flight legs above and below single-layer cirrus were performed. The solar radiation measurements are used to evaluate ecRad in two case studies of optically thin and thick cirrus, with an average transmissivity of 0.9 and 0.6, respectively. Different ice optics parameterizations optionally available in ecRad are applied to test the match between simulation and measurements. Furthermore, the IFS-predicted ice water content and ice effective radius are replaced by values retrieved with the radar and lidar. The choice of ice optics parameterizations does not significantly improve the model–measurement agreement. However, introducing the retrieved ice microphysical properties brings measured and modelled irradiances in closer agreement for the optically thin cirrus, while the optically thick cirrus case is simulated as too thick. It is concluded that the ice water content simulated by the IFS is realistic and that the mismatch between observed and simulated solar irradiances mostly originates from the assumed or parameterized ice effective radius.

Sensitivity analysis of space-based water vapor differential absorption lidar at 823 nm

Measurements of water vapor are important for understanding the hydrological cycle, the thermodynamic structure of the lower troposphere, and broader atmospheric circulation. Subsequently, many scientific communities have emphasized a need for high-accuracy and spatial resolution profiles of water vapor within and above the planetary boundary layer (PBL). Advancements in lidar technologies at the NASA Langley Research Center are ongoing to enable the first space-based water vapor differential absorption lidar (DIAL) that can provide high-accuracy and vertical resolution retrievals of moisture in the PBL and through the mid-troposphere. The performance of this space-based DIAL is assessed here for sensitivity throughout the troposphere and globally with representative canonical cases of water vapor and aerosol loading. The specific humidity retrieval sensitivity to systematic and random errors is assessed, and measurement resolutions and capabilities are provided. We show that tunable operation along the side of the 823-nm absorption line allows for the optimization of the lower-tropospheric water vapor retrievals across different meteorological regimes and latitudes and provides the operational flexibility needed to dynamically optimize random errors for different scientific applications. The analysis presented here suggests that baseline and threshold systematic error requirements of <1.5% and <2.5%, respectively, are achievable. Random error is shown to dominate the retrieval, with errors on the order of 5% within the PBL being achievable with 300-m vertical 50-km horizontal resolutions over open ocean and on the order of 10%–15% over high-albedo surfaces. The flexibility of the DIAL method to trade retrieval precision for spatial resolution is shown, highlighting its strengths over passive techniques to tailor retrievals to different scientific applications. Combined, the total error budget demonstrated here indicates a high impact for space-based DIAL, with technologies being advanced for space missions within the next 5–10 years.

Broadband continuous-wave differential absorption lidar for atmospheric remote sensing of water vapor.

What we believe to be a novel low-cost broadband continuous-wave water vapor differential absorption lidar (CW-DIAL) technique has been proposed and implemented by combing the Scheimpflug principle and the differential absorption method. The broadband CW-DIAL technique utilizes an 830-nm high-power multimode laser diode with 3-W output power as a tunable light source and a CMOS image sensor tilted at 45° as the detector. A retrieval algorithm dedicated for the broadband CW-DIAL technique has been developed to obtain range-resolved water vapor concentration from the DIAL signal. Atmospheric remote sensing of water vapor has been carried out on a near-horizontal water vapor path to validate the performance of the broadband CW-DIAL system. The retrieved water vapor concentration showed a good consistency with those measured by an air quality monitoring station, with a correlation coefficient of 0.9669. The fitting error of the water vapor concentration is found to be less than 10%. Numerical simulation studies have revealed that the aerosol-induced error on the water vapor concentration is below 5% with a background water vapor concentration of 5 g/m3 for most atmospheric conditions. The experimental results have successfully demonstrated the feasibility of the present broadband CW-DIAL technique for range-resolved water vapor remote sensing.

Simultaneous Observations of Surface Layer Profiles of Humidity, Temperature, and Wind Using Scanning Lidar Instruments

AbstractWe demonstrate the combination of three Doppler lidars (DLs), a water vapor differential absorption lidar and a temperature rotational Raman lidar for the investigation of the interactions between the land‐surface and the atmospheric boundary layer. This combination of scanning lidars was operated for the first time during the Land‐Atmosphere Feedback Experiment at the Atmospheric Radiation Measurement program's Southern Great Plain site, Oklahoma, USA, in August 2017, and provided simultaneous surface layer profiles of horizontal wind, humidity and temperature. The horizontal wind profiles were determined using the dual‐Doppler method with two DLs. The scans were performed above four towers providing atmospheric variables and fluxes. These combined lidar data allowed for the estimation of the friction velocity as well as the surface latent and sensible heat fluxes. For this purpose, profiles calculated with Monin‐Obukhov similarity theory were fitted with the Levenberg‐Marquardt nonlinear least squares curve‐fitting method to the measured surface‐layer lidar profiles. We present case studies of three 50‐min periods to illustrate the new method. The measurements resulted in friction velocities of 0.31, 0.29, and 0.38 ms−1, sensible surface heat fluxes of 312.1, 234.1, and 183.3 Wm−2 and latent surface heat fluxes of 251.8, 227.3, and 274.4 Wm−2. These values were compared with the in‐situ measurements of the towers. Considering the sampling differences and the error analyses, the results agree within 25.1%, 42.5%, and 28.8%, respectively, demonstrating that this synergy of scanning active remote sensing systems can be used to derive surface fluxes with reasonable accuracy.

Differential absorption lidar measurements of water vapor by the High Altitude Lidar Observatory (HALO): retrieval framework and first results

Abstract. Airborne differential absorption lidar (DIAL) offers a uniquely capable solution to the problem of measuring water vapor (WV) with high precision, accuracy, and resolution throughout the troposphere and lower stratosphere. The High Altitude Lidar Observatory (HALO) airborne WV DIAL was recently developed at NASA Langley Research Center and was first deployed in 2019. It uses four wavelengths near 935 nm to achieve sensitivity over a wide dynamic range and simultaneously employs 1064 nm backscatter and 532 nm high-spectral-resolution lidar (HSRL) measurements for aerosol and cloud profiling. A key component of the WV retrieval framework is flexibly trading resolution for precision to achieve optimal datasets for scientific objectives across scales. An approach to retrieving WV in the lowest few hundred meters of the atmosphere using the strong surface return signal is also presented. The five maiden flights of the HALO WV DIAL spanned the tropics through midlatitudes with a wide range of atmospheric conditions, but opportunities for validation were sparse. Comparisons to dropsonde WV profiles were qualitatively in good agreement, though statistical analysis was impossible due to systematic error in the dropsonde measurements. Comparison of HALO to in situ WV measurements aboard the aircraft showed no substantial bias across 3 orders of magnitude, despite variance (R2=0.66) that may be largely attributed to spatiotemporal variability. Precipitable water vapor measurements from the spaceborne sounders AIRS and IASI compared very well to HALO with R2>0.96 over ocean.

High Energy Parametric Laser Source and Frequency-Comb-Based Wavelength Reference for CO2 and Water Vapor DIAL in the 2 µm Region: Design and Pre-Development Experimentations

We present a differential absorption lidar (DIAL) laser transmitter concept designed around a Nested Cavity Optical Parametric Oscillator (NesCOPO) based Master Oscillator Power Amplifier (MOPA). The spectral bands are located around 2051 nm for CO2 probing and 1982 nm for H216O and HD16O water vapor isotopes. This laser is aimed at being integrated into an airborne lidar, intended to demonstrate future spaceborne instrument characteristics: high-energy (several tens of mJ nanosecond pulses) and high optical frequency stability (less than a few hundreds of kHz long term drift). For integration and efficiency purposes, the proposed design is oriented toward the use of state-of-the-art high aperture periodically poled nonlinear materials. This approach is supported by numerical calculations and preliminary experimental validations, showing that it is possible to achieve energies in the 40–50 mJ range, reaching the requirement levels for spaceborne Integrated Path Differential Absorption (IPDA) measurements. We also propose a frequency referencing technique based on beat note measurement of the laser signal with a self-stabilized optical frequency comb, which is expected to enable frequency measurement precisions better than a few 100 kHz over tens of seconds integration time, and will then be used to feed the cavity locking of the NesCOPO.

Observation of sensible and latent heat flux profiles with lidar

Abstract. We present the first measurement of the sensible heat flux (H) profile in the convective boundary layer (CBL) derived from the covariance of collocated vertical-pointing temperature rotational Raman lidar and Doppler wind lidar measurements. The uncertainties of the H measurements due to instrumental noise and limited sampling are also derived and discussed. Simultaneous measurements of the latent heat flux profile (L) and other turbulent variables were obtained with the combination of water-vapor differential absorption lidar (WVDIAL) and Doppler lidar. The case study uses a measurement example from the HOPE (HD(CP)2 Observational Prototype Experiment) campaign, which took place in western Germany in 2013 and presents a cloud-free well-developed quasi-stationary CBL. The mean boundary layer height zi was at 1230 m above ground level. The results show – as expected – positive values of H in the middle of the CBL. A maximum of (182±32) W m−2, with the second number for the noise uncertainty, is found at 0.5 zi. At about 0.7 zi, H changes sign to negative values above. The entrainment flux was (-62±27) W m−2. The mean sensible heat flux divergence in the observed part of the CBL above 0.3 zi was −0.28 W m−3, which corresponds to a warming of 0.83 K h−1. The L profile shows a slight positive mean flux divergence of 0.12 W m−3 and an entrainment flux of (214±36) W m−2. The combination of H and L profiles in combination with variance and other turbulent parameters is very valuable for the evaluation of large-eddy simulation (LES) results and the further improvement and validation of turbulence parameterization schemes.

Measurements of Water Vapor Profiles with Compact DIAL in the Tokyo Metropolitan Area

In recent years, the frequency of occurrence of locally heavy rainfall that can cause extensive damages, has been increasing in Japan. For early prediction of heavy rainfall, it is useful to measure the water vapor vertical distribution upwind cumulus convection beforehand. For that purpose, we have been developing compact water vapor differential absorption lidar (DIAL). We show the results of the measurements with lidar in summer when the local heavy rainfall frequently occurs in Japan. We also show the preliminary result of the assimilation of the lidar data to the numerical model and impact on the heavy rainfall prediction.

New laser design for NIR lidar applications

Recently, we quantified the very high spatio-temporal short term variability of tropospheric water vapor in a three dimensional study [1]. From a technical point of view this also depicted the general requirement of short integration times for recording water-vapor profiles with lidar. For this purpose, the only suitable technique is the differential absorption lidar (DIAL) working in the near-infrared (NIR) spectral region. The laser emission of most water vapor DIAL systems is generated by Ti:sapphire or alexandrite lasers. The water vapor absorption band at 817 nm is predominated for the use of Ti:sapphire. We present a new concept of transversely pumping in a Ti:Sapphire amplification stage as well as a compact laser design for the generation of single mode NIR pulses with two different DIAL wavelengths inside a single resonator. This laser concept allows for high output power due to repetitions rates up to 100Hz or even more. It is, because of its compactness, also suitable for mobile applications.

水汽差分吸收激光雷达发射机935 nm高功率光参量振荡器

水汽差分吸收激光雷达发射机935 nm高功率光参量振荡器

The HD(CP)<sup>2</sup> Observational Prototype Experiment (HOPE) – an overview

Abstract. The HD(CP)2 Observational Prototype Experiment (HOPE) was performed as a major 2-month field experiment in Jülich, Germany, in April and May 2013, followed by a smaller campaign in Melpitz, Germany, in September 2013. HOPE has been designed to provide an observational dataset for a critical evaluation of the new German community atmospheric icosahedral non-hydrostatic (ICON) model at the scale of the model simulations and further to provide information on land-surface–atmospheric boundary layer exchange, cloud and precipitation processes, as well as sub-grid variability and microphysical properties that are subject to parameterizations. HOPE focuses on the onset of clouds and precipitation in the convective atmospheric boundary layer. This paper summarizes the instrument set-ups, the intensive observation periods, and example results from both campaigns. HOPE-Jülich instrumentation included a radio sounding station, 4 Doppler lidars, 4 Raman lidars (3 of them provide temperature, 3 of them water vapour, and all of them particle backscatter data), 1 water vapour differential absorption lidar, 3 cloud radars, 5 microwave radiometers, 3 rain radars, 6 sky imagers, 99 pyranometers, and 5 sun photometers operated at different sites, some of them in synergy. The HOPE-Melpitz campaign combined ground-based remote sensing of aerosols and clouds with helicopter- and balloon-based in situ observations in the atmospheric column and at the surface. HOPE provided an unprecedented collection of atmospheric dynamical, thermodynamical, and micro- and macrophysical properties of aerosols, clouds, and precipitation with high spatial and temporal resolution within a cube of approximately 10 × 10 × 10 km3. HOPE data will significantly contribute to our understanding of boundary layer dynamics and the formation of clouds and precipitation. The datasets have been made available through a dedicated data portal. First applications of HOPE data for model evaluation have shown a general agreement between observed and modelled boundary layer height, turbulence characteristics, and cloud coverage, but they also point to significant differences that deserve further investigations from both the observational and the modelling perspective.

Advances in Diode-Laser-Based Water Vapor Differential Absorption Lidar

An advanced diode-laser-based water vapor differential absorption lidar (WV-DIAL) has been developed. The next generation design was built on the success of previous diode-laser-based prototypes and enables accurate measurement of water vapor closer to the ground surface, in rapidly changing atmospheric conditions, and in daytime cloudy conditions up to cloud base. The lidar provides up to 1 min resolution, 150 m range resolved measurements of water vapor in a broad range of atmospheric conditions. A description of the instrument and results from its initial field test in 2014 are discussed.

A review of the remote sensing of lower tropospheric thermodynamic profiles and its indispensable role for the understanding and the simulation of water and energy cycles

AbstractA review of remote sensing technology for lower tropospheric thermodynamic (TD) profiling is presented with focus on high accuracy and high temporal‐vertical resolution. The contributions of these instruments to the understanding of the Earth system are assessed with respect to radiative transfer, land surface‐atmosphere feedback, convection initiation, and data assimilation. We demonstrate that for progress in weather and climate research, TD profilers are essential. These observational systems must resolve gradients of humidity and temperature in the stable or unstable atmospheric surface layer close to the ground, in the mixed layer, in the interfacial layer—usually characterized by an inversion—and the lower troposphere. A thorough analysis of the current observing systems is performed revealing significant gaps that must be addressed to fulfill existing needs. We analyze whether current and future passive and active remote sensing systems can close these gaps. A methodological analysis and demonstration of measurement capabilities with respect to bias and precision is executed both for passive and active remote sensing including passive infrared and microwave spectroscopy, the global navigation satellite system, as well as water vapor and temperature Raman lidar and water vapor differential absorption lidar. Whereas passive remote sensing systems are already mature with respect to operational applications, active remote sensing systems require further engineering to become operational in networks. However, active remote sensing systems provide a smaller bias as well as higher temporal and vertical resolutions. For a suitable mesoscale network design, TD profiler system developments should be intensified and dedicated observing system simulation experiments should be performed.

Observations of the 9 June 2002 Dryline During IHOP

Detailed studies of drylines that do not initiate storms are rare but scientifically important. Studying these null cases will improve the understanding of critical factors separating whether convection would be initiated along a dryline. This observational study presents a null case dryline near the Oklahoma/New Mexico border during the International H2O Project (IHOP_2002) on 9 June 2002. High-resolution observations obtained from an airborne Doppler radar (ELDORA), two water-vapor Differential Absorption Lidar (LEANDRE II and LASE), Learjet dropsondes, as well as aircraft in situ measurements were used to describe the dryline environment and mesoscale structures in both along- and cross-line directions. The 9 June dryline was characterized by a rather broad radar reflectivity thinline with a large moisture gradient. Its updrafts were found generally associated with the local maximum of radar reflectivity; however, they were not colocated. The simultaneous observations from ELDORA and LEANDRE II confirmed that the dryline updrafts tend to be located near its moisture gradient, consistent with previous findings using aircraft in situ measurements. The dryline moisture boundary was found to be greatly modified by mesocyclone circulations, which caused the alongline moisture gradient at certain segments of the dryline to become greater than the cross-line moisture gradient. Twodimensional water vapor fields derived from LEANDRE II across the dryline clearly showed the moisture gradient associated with the dryline and moisture variations on the order of ~ 1 g kg-1 on both sides of the dryline. No storms initiated within the IHOP_2002 domain associated with this dryline owing to unfavorable atmospheric instability conditions and only weak upward forcing near the dryline.

Dry and moist convection in the boundary layer over the Black Forest - a combined analysis of in situ and remote sensing data

During the COPS experiment performed in south-western Germany and eastern France in 2007, several insitu and remote sensing systems were operated at Hornisgrinde - the highest summit of the northern Black Forest mountains. For this case study, data from a surface flux station, radiosondes, cloud camera, cloud radar, wind lidar, water vapour differential absorption lidar, and microwave profiler were used to investigate turbulence characteristics in cloud-free and cloud-topped convective boundary layers (CBLs). Short time intervals were analysed, during which dry and moist convective cells occurred, in order to obtain insight of the processes that determine the turbulent characteristic in the CBL. The frequently-used aerosol concentration was used to calculate the CBL height, zi. It was found that active CBL clouds penetrated deeper into the free troposphere than dry convective cells. In the cloud-free CBL the normalised variance of the vertical velocity, rw 2 , decreased to zero approximately at zi, while rw 2 was nearly constant between 0.5 and 1 z/zi in the cloud-topped CBL. The higher normalised rw 2 values in the cloud layer could be attributed to the additional elevated heat source due to condensation. In the cloud-free CBL the latent heat flux showed a strong decrease between 0.7 and 1.1 z/zi, i.e., it considerably moistened the upper part of the CBL and entrainment zone. In the cloud-topped CBL the latent heat flux decreased significantly above the CBL top only and became zero at about 1.4 z/zi. CBL height calculations, which took measures of the turbulence into account, resulted in normalised rw 2 and E profiles, which became zero at the CBL top and appeared more appropriate for CBL height scaling over complex terrain. The case studies demonstrated that only the combined use of different monitoring systems allowed for the recording of the entire structure of the convective cells and that synergetic measurements in cloud-topped CBLs were indispensable to capture the latters’ turbulent characteristics. Also, significant differences between turbulent characteristics in cloud-free and cloud-topped CBLs became evident.

Online/offline injection seeding system with high frequency-stability and low crosstalk for water vapor DIAL

A compact and rugged distributed feedback (DFB) laser system has been developed as online–offline injection seeder for the laser transmitter of a ground-based water vapor differential absorption lidar (WV DIAL) near 820nm. The frequency stability of this injection seeder system shows a standard deviation of only 6.3MHz and a linewidth of less than 4.6MHz during continuous operation of more than 14h. These values by far exceed the requirements for WV DIAL. By use of a novel technique based on an electro-optic deflector (EOD), alternating online–offline wavelength switching is achieved for each shot of the seeded laser with 250Hz with a response time of less than 10µs and very low crosstalk between the channels of only 33dB. As a result, a spectral purity of 99.95% is reached by the WV DIAL transmitter which again fulfills the requirements for WV DIAL measurements with high accuracy. Because moveable parts are not present in the seeding system, this setup is significantly less sensitive to acoustic vibrations and ambient temperature drifts during field experiments than other seeding systems which use external cavity diode lasers (ECDL) and mechanical switches. By our new seeding system not only the requirements for ground-based water-vapor DIAL are met but also for space-borne WV DIAL applications that pose even higher demands to the frequency stability and spectral purity of the laser transmitters.

Detection and Analysis of Water Vapor Transport by Airborne Lidars

Water vapor, a minor constituent of the earth's atmosphere, plays a major role in the radiation budget and the water cycle with important implications for weather and climate. Due to the heterogeneous distribution of its sources, evaporation, and sinks, condensation and precipitation, and due to the complexity of atmospheric motion and mixing, its distribution in the atmosphere is highly variable. Despite the high relevance of this trace gas, its variability challenges accurate measurements of its concentration. Advanced airborne lidar instruments aid to better observe water vapor and its transport in the atmosphere, in view of an improved understanding of atmospheric processes that are key to weather and climate research. The combination of a water vapor differential absorption lidar and a heterodyne detection Doppler wind lidar on an aircraft is new and allows to measure vertical profiles of the latent heat flux in a convective boundary layer and to portray the small- to large-scale humidity transport and variability along the aircraft flight track with high accuracy and spatial resolution.

High-power Ti:sapphire laser at 820 nm for scanning ground-based water–vapor differential absorption lidar

The Ti:sapphire (TISA) laser transmitter of the mobile, three-dimensional-scanning water-vapor differential absorption lidar (DIAL) of the University of Hohenheim is described in detail. The dynamically-stable, unidirectional ring resonator contains a single Brewster-cut TISA crystal, which is pumped from both sides with 250 Hz using a diode-pumped frequency-doubled Nd:YAG laser. The resonator is injection seeded and actively frequency-stabilized using a phase-sensitive technique. The TISA laser is operating near 820 nm, which is optimum for ground-based water-vapor DIAL measurements. An average output power of up to 6.75 W with a beam quality factor of M2<2 is reached. The pointing stability is <13 μrad (rms), the depolarization <1%. The overall optical-optical conversion efficiency is up to 19%. The pulse length is 40 ns with a pulse linewidth of <157 MHz. The short- and long-term frequency stabilities are 10 MHz (rms). A spectral purity of 99.9% was determined by pointing to a stratus cloud in low-elevation scanning mode with a cloud bottom height of ≈2.4 km.

Micropulse water vapor differential absorption lidar: transmitter design and performance

An all diode-laser-based micropulse differential absorption lidar (DIAL) laser transmitter for tropospheric water vapor and aerosol profiling is presented. The micropulse DIAL (MPD) transmitter utilizes two continuous wave (cw) external cavity diode lasers (ECDL) to seed an actively pulsed, overdriven tapered semiconductor optical amplifier (TSOA). The MPD laser produces up to 7 watts of peak power over a 1 µs pulse duration (7 µJ) and a 10 kHz pulse repetition frequency. Spectral switching between the online and offline seed lasers is achieved on a 1Hz basis using a fiber optic switch to allow for more accurate sampling of the atmospheric volume between the online and offline laser shots. The high laser spectral purity of greater than 0.9996 coupled with the broad tunability of the laser transmitter will allow for accurate measurements of tropospheric water vapor in a wide range of geographic locations under varying atmospheric conditions. This paper describes the design and performance characteristics of a third generation MPD laser transmitter with enhanced laser performance over the previous generation DIAL system.

Optical characterization of continental and biomass-burning aerosols over Bozeman, Montana: A case study of the aerosol direct effect

[1] Atmospheric aerosol optical properties were observed from 21 to 27 September 2009 over Bozeman, Montana, during a transitional period in which background polluted rural continental aerosols and well-aged biomass-burning aerosols were the dominant aerosol types of extremely fresh biomass-burning aerosols resulting from forest fires burning in the northwestern United States and Canada. Aerosol optical properties and relative humidity profiles were retrieved using an eye-safe micropulse water vapor differential absorption lidar (DIAL) (MP-DIAL), a single-channel backscatter lidar, a CIMEL solar radiometer as part of the Aerosol Robotic Network (AERONET), a ground-based integrating nephelometer, and aerosol products from Moderate Resolution Imaging Spectroradiometer (MODIS) Terra and Aqua. Aerosol optical depths (AODs) measured during the case study ranged between 0.03 and 0.17 (0.015 and 0.075) at 532 nm (830 nm) as episodic combinations of fresh and aged biomass-burning aerosols dominated the optical depth of the pristinely clean background air. Here, a pristinely clean background refers to very low AOD conditions, not that the aerosol scattering and absorption properties are necessarily representative of a clean aerosol type. Diurnal variability in the aerosol extinction to backscatter ratio (Sa) of the background atmosphere derived from the two lidars, which ranged between 55 and 95 sr (50 and 90 sr) at 532 nm (830 nm), showed good agreement with retrievals from AERONET sun and sky measurements over the same time period but were consistently higher than some aerosol models had predicted. Sa measured during the episodic smoke events ranged on average from 60 to 80 sr (50 to 70 sr) at 532 nm (830 nm) while the very fresh biomass-burning aerosols were shown to exhibit significantly lower Sa ranging between 20 and 40 sr. The shortwave direct radiative forcing that was due to the intrusion of biomass-burning aerosols was calculated to be on average −10 W/m2 and was shown to compare favorably with regional-scale forcing calculations using MODIS-Terra and AERONET data in an effort to assess the accuracy of estimating the regional-scale aerosol direct radiative forcing effect using aerosol optical properties measured from a single rural site such as Bozeman, Montana.