The promotion of multimodal coordination is of great significance for the joint development of diverse urban transportation systems. Focusing on a comprehensive urban passenger transport hub that converges both intercity modes and multiple inner-city modes, our study aims to incorporate intercity railway and Metrorail coordination into train scheduling optimization to enhance transfer efficiency and provide a seamless service for passengers in urban railway networks. By considering the variety of passenger demands in different transport modes (e.g., rail transit and traditional mainline railway), train loading capacity, and potential disruption scenarios, we specifically developed a mixed-integer nonlinear programming (MINLP) model to simultaneously generate the coordination strategies, arrival/departure times of trains at each station, and the number of carriages in service in the network. To enhance computational efficiency, we proposed several improvement strategies involving the model linearization to reformulate the MINLP model into a mixed-integer linear programming (MILP) model and the determination of appropriate big- M values. Finally, numerical experiments based on historical passenger data from a realistic urban railway network in China were implemented to verify the effectiveness of our approach. The results demonstrate that our intercity railway and Metrorail coordination strategies could, in practice, significantly improve passenger transfer efficiency by over 35% compared with the train schedule without coordination.