Unraveling mechanical properties from fundamental is far from complete despite their vital role in determining applicability and longevity for a given material. Here, we perform a comprehensive study related to mechanical properties of 60 pure elements in bcc, fcc, hcp, and/or diamond structures by means of pure alias shear and pure tensile deformations via density functional theory (DFT) based calculations alongside a broad review of existing literature. The present data compilation enables a detailed correlation analysis of mechanical properties, focusing on DFT-based ideal shear and tensile strengths ( and ), stable and unstable stacking fault energies ( and ), surface energy (), and vacancy activation energy (); and experimental hardness (), ultimate tensile strength (), fracture toughness (), and elongation (). The present work examines models, identifies outliers, and provides insights into mechanical properties, for example, (i) is correlated by , by or , and by ; (ii) data outliers are identified for Cr (related to , , , and ), Be (, , , and ), Hf ( and ), Yb (all properties), and Pt ( vs. ); and (iii) , , , , , , and are highly correlated to elemental attributes, while , , and especially are less correlated due mainly to experimental uncertainty. In particular, the present data compilation provides a solid foundation to model properties such as and of multicomponent alloys and of unstable structures like bcc Ti, Zr, and Hf.