In this study, the ballistic performance of the composite structure was investigated and studied by experiment and finite element analysis in order to study the anti-penetration performance of a polyurethane elastomer-coated honeycomb sandwich construction. Six kinds of target plate structures with different configurations were prepared by changing the hard segment content and coating position of polyurethane elastomer. The first-stage light gas gun device is used to conduct impact experiments at various speeds, and the finite element simulation computation is performed using LS-DYNA. Based on the experimental and finite element results, the ballistic limit velocity and specific energy absorption of different target configurations were analyzed, and the failure forms, damage areas, and failure mechanisms were discussed. The findings demonstrate that the polyurethane elastomer coating enhances the honeycomb sandwich structure’s ballistic limit performance by 40.6% to 51% and that the honeycomb core of the target plate with the coating on the front panel has a larger area of collapse. This fully exploits the benefits of the honeycomb structure in the energy absorption process and makes up for the weaknesses of the honeycomb sandwich structure’s subpar energy absorption effect under local impact loads. Therefore, the front panel coating has better ballistic limit performance. The coated polyurethane with medium hardness demonstrated the best ballistic limit performance for the various polyurethane hardness. The ballistic limit speeds of the front panel and back panel coatings increased by 51% and 48.8% respectively, in comparison to the uncoated target plate. After comparing the structure of polyurea coating, it is found that the ballistic limit performance of polyurethane coating with medium hardness is higher than that of polyurea coating structure, and the negative growth of the ballistic limit performance of the whole structure caused by the coating of rigid polyurea on the back panel is effectively avoided.
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