Ultrafast Laser Oscillators Research Articles

Ultrafast 550-W average-power thin-disk laser oscillator

SESAM modelocked oscillators are interesting for applications in strong-field physics such as high-harmonic generation and attosecond science at high repetition rates or frequency combs in the ultraviolet. Here we present a SESAM modelocked ultrafast thin-disk laser oscillator providing 550W of average output power with 852fs pulses at 5.5MHz repetition rate. To reach this significant power scaling, a replicating cavity design for modelocked oscillators is utilized. The oscillator delivers 103 MW of peak power with a pulse energy of 100 µJ at a beam quality of M2<1.2, with a high optical-to-optical efficiency of 35%. The advances in SESAM design and manufacturing that enabled this result are discussed, as well as practical challenges when scaling oscillators to the kW-class. When combined with established pulse compression technologies, this oscillator can enable simpler systems by avoiding the complexity of chirped pulse amplifier chains. Additionally, high power oscillators support a much lower noise floor due to the reduced influence of shot noise, which may provide a route to more sensitive pump-probe measurements.

All-polarization-maintaining Nd-doped ultrafast fiber laser oscillator at 929 nm mode-locked via a 3x3 nonlinear amplifying loop mirror: erratum

All-polarization-maintaining Nd-doped ultrafast fiber laser oscillator at 929 nm mode-locked via a 3x3 nonlinear amplifying loop mirror: erratum

Six-orders-of-magnitude-spanning dispersion measurement via Kalman filtering-aided white-light interferometry.

Dispersion plays a great role in ultrafast laser oscillators, ultrashort pulse amplifiers, and many other nonlinear optical dynamics. Therefore, dispersion measurement is crucial for device characterization, system design and nonlinear dynamics investigation therein. In this work, we demonstrate a versatile approach, i.e., Kalman filtering-aided white-light interferometry, for group delay dispersion (GDD) characterization. Extended Kalman filter is adopted to track the cosine-like interferogram, and to eliminate the unintended bias and the envelope, providing a nearly ideal phase retrieval and GDD estimation. The measurement range could span from tens of fs2 to tens of ps2, with an uncertainty of about 0.1%, enabling precise GDD measurement for diverse optical components, ranging from a millimeter-thick glass slide to highly dispersive chirped fiber Bragg gratings. Benefited by the simplicity, convenient setup, and easy operation as well as relatively low cost, this approach would help photonic device characterization, dispersion management and nonlinear dynamics investigation in the laboratory and work plant.

Modelocked Thin-Disk Laser Oscillator with 550 W of Average Output Power

We present an ultrafast thin-disk laser oscillator providing a record power of 550 W with 100-µJ, 852-fs pulses at a repetition rate of 5.5 MHz. This is enabled by a six-pass replicating-cavity multipass scheme and ion-implanted sapphire-bonded SESAMs.

A Decade of Sub‐100‐fs Thin‐Disk Laser Oscillators

AbstractThin‐disk lasers (TDLs) are best known for their high‐power continuous‐wave industrial applications. Nonetheless, the thin‐disk geometry is also highly attractive for ultrafast laser oscillators. The short propagation distance and large beam diameter inside the gain crystal allows for very low induced nonlinearity, low dispersion, and extreme peak powers inside the laser cavity. The path toward TDL oscillators directly delivering high average power at ultrafast pulse duration required for many scientific applications has, however, been tangled and is still ongoing. A decade ago, the first sub‐100‐fs laser oscillator is demonstrated, initiating the pursuit of even shorter pulses. Since then, many gain materials have been investigated in the thin‐disk geometry as well as various mode‐locking mechanisms for their suitability for efficient short‐pulse operation. In this review, the fast‐evolving development trends of TDL oscillators, as well as their scientific applications and prospects will be discussed.

Ultrafast thin-disk laser oscillators as driving sources for high harmonic generation

Thin-disk laser oscillators can nowadays reach few tens of femtosecond pulses at gigawatt-level intracavity powers and megahertz-repetition rates becoming increasingly more powerful sources for intra-oscillator high harmonic generation (HHG). Currently, we can generate high harmonics in neon reaching photon energies of 70 eV, which we expect to increase toward 100 eV in the near future. In parallel, the achievable average and peak output powers of these oscillators in the range of 100 W and 100 MW, respectively, make these sources very promising to drive HHG in single-pass configuration after nonlinear pulse compression. Starting from transform-limited 30 to 50-fs soliton output soliton pulses of TDL oscillators, we will likely see these lasers approaching a single-cycle regime becoming highly attractive sources for attosecond science.

All-PM Fiber Mamyshev Oscillator Delivers Hundred-Nanojoule and Multi-Watt Sub-100 fs Pulses

An all-fiber Mamyshev oscillator with a single amplification arm is experimentally demonstrated to achieve high-energy and high-average-power ultrafast pulse output, with the initiating of an external seed pulse. In the high-energy operation, a maximum single-pulse energy of 153 nJ is achieved at a repetition rate of 9.77 MHz. After compression with a pair of diffraction gratings, a measured pulse width of 73 fs with a record energy of 122.1 nJ and a peak power of 1.7 MW is obtained. In the high-average-power operation, up to 5th harmonic mode locking of the oscillator is realized via slightly adjusting the output coupling ratio and the cavity length. The achieved maximum output power is 3.4 W at a repetition rate of 44.08 MHz, while the corresponding pulse width is compressed to around ~100 fs. Meanwhile, the system is verified to be operated reliability in both high-energy and -average-power operation regimes through assessing its short- and long-term stabilities. To the best of our knowledge, these are the highest records in pulse energy and average power delivered from a single all-fiber ultrafast laser oscillator with picosecond/femtosecond pulse duration. It is believed that even higher-energy and -average-power ultrafast laser can be realized with the proposed laser scheme through further increasing the core diameter of the all-fiber cavity, providing promising sources for advanced fabrication, biomedical imaging, laser micromachining, and other practical applications, as well as an unprecedented platform for exploring undiscovered nonlinear dynamics.

High-power 55-fs Yb:YAG thin-disk oscillator at 200 MHz repetition rate

High-repetition-rate ultrafast laser oscillators with high average power and short pulse duration provide excellent sources for generating optical frequency combs. Here we report a Kerr-lens mode locked Yb:YAG thin-disk oscillator delivering 203-MHz pulses at an average power of 9.4 W. A single additional nonlinear plate was inserted inside the cavity to enhance the Kerr lens effect, which leads to a substantial broadening of the mode-locked spectrum. The resultant pulse duration is 55 fs. The demonstrated oscillator combines a high repetition rate, a high average power and short pulse duration within one resonator, offering an ideal prerequisite for the optical-frequency metrology and frequency-comb spectroscopy with high signal-to-noise ratio.

Efficient XUV-light out-coupling of intra-cavity high harmonics by a coated grazing-incidence plate.

We experimentally demonstrate an efficient and broadband extreme-ultraviolet light (XUV) out-coupling mechanism of intra-cavity generated high harmonics. The mechanism is based on a coated grazing-incidence plate (GIP), which utilizes the enhanced reflectivity of s-polarized light in comparison to p-polarized light for large angles of incidence (AoI). We design and produce a 60°-AoI coated GIP, tailored specifically for the high demands inside a sub-50-fs Kerr-lens mode-locked Yb:YAG thin-disk laser oscillator in which high harmonic generation (HHG) is driven at ∼450 MW peak power and 17 MHz repetition rate. The coated GIP features an XUV out-coupling efficiency of >25% for photon energies ranging from 10 eV to 60 eV while being anti-reflective for the driving laser field. The XUV spectra reach up to 52 eV in argon and 30 eV in xenon. In a single harmonic, we out-couple 1.3 µW of XUV average power at 37 eV in argon and 5.4 µW at 25 eV in xenon. The combination of an improved HHG driving laser performance and the out-coupling via the coated GIP enabled us to increase the out-coupled XUV average power in a single harmonic by a factor of 20 compared to previous HHG inside ultrafast laser oscillators. Our source approaches the state-of-the-art out-coupled XUV power levels per harmonic of femtosecond enhancement cavities operating at comparable photon energies.

Efficient high-power sub-50-fs gigahertz repetition rate diode-pumped solid-state laser.

In this article we present a directly diode-pumped high-power Kerr-lens mode-locked Yb:CALGO bulk laser oscillator operating at 1-GHz repetition rate. We report on two laser configurations optimized for either highest average power or shortest pulse duration. In the first configuration optimized for high average power, the oscillator delivers up to 6.9 W of average power, which is the highest average power of any ultrafast laser oscillator operating at gigahertz repetition rate. The 93-fs pulses have a peak power of 64 kW, and the optical-to-optical efficiency amounts to 37%. In the second configuration optimized for short pulse duration, we demonstrate 48-fs pulses at 4.1 W of average power corresponding to a higher peak power of 74kW with 21% optical-to-optical efficiency. This is the shortest pulse duration and the highest peak power demonstrated by any GHz-class Yb-based laser oscillator. The compact laser setup is directly pumped by a low-cost multimode fiber-coupled laser diode and has a high potential as an economical yet powerful source for various applications.

High-power low-noise 2-GHz femtosecond laser oscillator at 2.4 µm.

Femtosecond lasers with high repetition rates are attractive for spectroscopic applications with high sampling rates, high power per comb line, and resolvable lines. However, at long wavelengths beyond 2 µm, current laser sources are either limited to low output power or repetition rates below 1 GHz. Here we present an ultrafast laser oscillator operating with high output power at multi-GHz repetition rate. The laser produces transform-limited 155-fs pulses at a repetition rate of 2 GHz, and an average power of 0.8 W, reaching up to 0.7 mW per comb line at the center wavelength of 2.38 µm. We have achieved this milestone via a Cr2+-doped ZnS solid-state laser modelocked with an InGaSb/GaSb SESAM. The laser is stable over several hours of operation. The integrated relative intensity noise is 0.15% rms for [10 Hz, 100 MHz], and the laser becomes shot noise limited (-160 dBc/Hz) at frequencies above 10 MHz. Our timing jitter measurements reveal contributions from pump laser noise and relaxation oscillations, with a timing jitter of 100 fs integrated over [3 kHz, 100 MHz]. These results open up a path towards fast and sensitive spectroscopy directly above 2 µm.

Efficient few-cycle Yb-doped laser oscillator with Watt-level average power.

So far, the operation of ultrafast bulk laser oscillators based on Yb-doped gain materials and directly emitting few-cycle pulses have been restricted to low optical-to-optical efficiencies and average output powers of only a few milliwatt. This performance limitation can be attributed to the commonly-applied standard collinear pumping scheme in which the optical pump is transmitted through a dichroic mirror whose spectral transmission and dispersion properties severely perturb the oscillating pulse when its optical spectrum extends towards the pump wavelength. In this study, we report on a novel pumping scheme relying on cross polarization that overcomes this challenge. In our concept, the pump transmitting mirror is highly transmissive for the pump light in p-polarization, while it is highly reflective for the laser light in s-polarization over a broad wavelength range, even covering the pump wavelength and beyond. In contrast to a standard thin-film polarizer featuring similar polarization dependent properties, it provides a low and flat dispersion profile over a broad spectral range for the s-polarization. Implementing this pumping scheme in a soft-aperture Kerr-lens mode-locked bulk laser oscillator based on the gain material Yb:CALGO, we achieve clean 22-fs soliton pulses at 729 mW of average output power and an optical-to-optical efficiency of 25%. In a second configuration optimized for the highest average output power, we demonstrate a high optical-to-optical efficiency of 36.6%, which was obtained for 31-fs pulses at 1.63 W of average output power. In a third configuration we experimentally confirm the limiting effect of a dichroic mirror commonly used in the standard collinear pumping scheme. All the results presented here and obtained in the first and second configuration generate pulses with a center wavelength ranging from 1030 nm to 1056 nm, well within the spectral region of high gain cross sections of Yb:CALGO. While this initial demonstration was realized using a commercial diffraction-limited fiber laser as pump source, the pump geometry appears also well suited for pumping with laser diodes coupled into multimode fibers. This novel approach opens up new opportunities for compact and cost-efficient high-power few-cycle bulk laser oscillators based on Yb-doped gain materials and can be applied to any gain material with small quantum defect.

Distributed Kerr Lens Mode-Locked Yb:YAG Thin-Disk Oscillator

Ultrafast laser oscillators are indispensable tools for diverse applications in scientific research and industry. When the phases of the longitudinal laser cavity modes are locked, pulses as short as a few femtoseconds can be generated. As most high-power oscillators are based on narrow-bandwidth materials, the achievable duration for high-power output is usually limited. Here, we present a distributed Kerr lens mode-locked Yb:YAG thin-disk oscillator which generates sub-50 fs pulses with spectral widths far broader than the emission bandwidth of the gain medium at full width at half maximum. Simulations were also carried out, indicating good qualitative agreement with the experimental results. Our proof-of-concept study shows that this new mode-locking technique is pulse energy and average power scalable and applicable to other types of gain media, which may lead to new records in the generation of ultrashort pulses.

Efficient 100-MW, 100-W, 50-fs-class Yb:YAG thin-disk laser oscillator

We demonstrate an efficient 102-MW peak power, 103-W average power, Kerr-lens mode-locked thin-disk laser (TDL) oscillator generating 52-fs pulses at 17.1-MHz repetition rate. The TDL is based on an Yb:YAG disk and operates in the strongly self-phase-modulation (SPM) broadened regime. In this regime, the spectral bandwidth of the oscillating pulse exceeds the available gain bandwidth by generating additional frequency components via SPM in the Kerr medium inside the laser cavity. At an optical-to-optical efficiency of 26%, our oscillator delivers a more than six times higher average power compared to any 50-fs-class laser oscillator. Compared to previous 100-W-class high-power laser oscillators, we reach this performance in a more than two times shorter pulse duration at a comparable optical-to-optical efficiency. Our TDL delivers the highest peak power of any ultrafast laser oscillator. The short pulse duration combined with high average power and peak power makes the presented TDL oscillator an attractive source for high field science and nonlinear optics.

Intra-oscillator broadband THz generation in a compact ultrafast diode-pumped solid-state laser.

We demonstrate broadband and powerful terahertz (THz) generation at megahertz repetition rate based on intra-oscillator optical rectification (OR) in gallium phosphide (GaP). By placing the nonlinear crystal directly inside the cavity of a Kerr-lens mode-locked ultrafast diode-pumped solid-state laser (DPSSL) oscillator, we demonstrate a compact and single-stage THz source. Using only 7 W of diode-pump power, we drive OR in a GaP crystal with 22 W of average power at ∼80 MHz repetition rate. In a first configuration, using a 0.3-mm-thick GaP and 105 fs driving pulses, we generate up to 150 µW of THz radiation with a spectrum extending to 5.5 THz. In a second configuration allowing for sub-50-fs pulse duration, we generate up to 7 THz inside a 0.1-mm-thick GaP crystal. This performance is well suited for THz time-domain spectroscopy and THz imaging. Intra-oscillator THz generation in sub-100-fs DPSSLs is a promising way to scale down footprint, complexity and cost of powerful broadband THz sources.

An in-band diode-end-pumped high-power and high-efficiency ultrashort pulse Nd:YVO4 bulk laser mode-locked by a frequency doubling LBO crystal

Nonlinear mirror (NLM) mode locking has also been verified to be an efficient technology for high-power ultrashort pulse laser generation. In this paper, we report on high-power and high-efficiency NLM mode-locked Nd:YVO4 laser with a 880-nm diode laser for in-band pumping, which has very rarely been investigated in the past. The achieved maximum average output power reached 6.76 W at an absorbed power of 13.82 W corresponding to a slope efficiency of 54.5%. Thanks to the used type I LBO crystal with small group velocity mismatch, the achieved pulse duration was as short as 6.5 ps. The results represent one of the best performances that ever achieved for NLM mode-locked Nd:YVO4 laser. NLM mode locking could be very promising for high-power ultrashort pulse generation in visible and middle infrared wavelengths, at which SESAMs are still not mature and the average output powers of ultrafast laser oscillators are also still limited to great extent.

Mamyshev Oscillator With a Widely Tunable Repetition Rate

Controlling an ultrafast laser oscillator repetition rate is crucial for the emerging laser burst micromachining. The efficiency of a material surface treatment process as well as the quality of live tissue ablation depends, to a considerable extent, on the number of laser pulses in a burst window. In the following article, we present an all-PM fiber harmonically mode-locked Mamyshev ring oscillator capable of producing laser pulses with a tunable period. The oscillator can be operated at any frequency, being a multiple of the fundamental repetition rate up to 305 MHz at 19th harmonic. We found that the operation frequency is limited by the available pump power only. What is worth noting is that the energy of the emitted pulses is independent of the operating frequency. The essential laser parameters are excellent: an amplitude noise of 0.1% and fundamental frequency suppression levels of 70 dB at every repetition rate. Additionally, the mechanism of harmonic mode-locking is discussed in detail and is found to be caused by gain depletion and recovery effect.

Optical rectification of ultrafast Yb lasers: pushing power and bandwidth of terahertz generation in GaP

We demonstrate broadband high-power terahertz (THz) generation at megahertz repetition rates by optical rectification in GaP driven by an ultrafast Yb-based thin-disk laser (TDL) oscillator. We investigate the influence of pulse duration in the range of 50–220 fs and thickness of the GaP crystal on the THz generation. Optimization of these parameters with respect to the broadest spectral bandwidth yields a gap-less THz spectrum extending to nearly 7 THz. We further tailor the driving laser and the THz generation parameters for the highest average power, demonstrating 0.3 mW THz radiation with a spectrum extending to 5 THz. This was achieved using a 0.5 mm thick GaP crystal pumped with a 95 fs, 20 W TDL, operating at 48 MHz repetition rate. We also provide a simple method to estimate the THz spectrum, which can be used for design and optimization of similar THz systems.

Self-phase modulation cancellation in a high-power ultrafast thin-disk laser oscillator

Ultrafast high-power lasers are employed in a wide variety of applications in science and industry. Thin-disk oscillators can offer compelling performance for these applications. However, because of the high intracavity peak power, a large amount of self-phase modulation (SPM) is picked up in the intracavity air environment. Consequently, the highest performance oscillators have been operated in a vacuum environment. Here, we introduce a new concept to overcome this hurdle. We cancel the SPM picked up in air by introducing an intracavity phase-mismatched second-harmonic-generation crystal. The resulting cascaded χ(2) processes provide a large SPM with a sign opposite the one originating from the air. This enables laser operation in air at 210 W average output power with 780 fs, 19 μJ pulses, the highest output power of any semiconductor saturable absorber mirror (SESAM) modelocked laser operated in air to date, to the best of our knowledge. This result paves the way to a novel approach for nonlinearity management in high-power lasers.

Broadband terahertz pulse generation driven by an ultrafast thin-disk laser oscillator.

We demonstrate broadband THz generation driven by an ultrafast thin-disk laser (TDL) oscillator. By optical rectification of 50-fs pulses at 61 MHz repetition rate in a collinear geometry in crystalline GaP, THz radiation with a central frequency at around 3.4 THz and a spectrum extending from below 1 THz to nearly 7 THz are generated. We realized a spectroscopic characterization of a GaP crystal and a benchmark measurement of the water-vapor absorption spectrum in the THz range. Sub-50-GHz resolution is achieved within a 5 THz bandwidth. Our experiments show the potential of ultrafast TDL oscillators for driving MHz-repetition-rate broadband THz systems.