Ultrafast All-optical Modulation Research Articles

All-optical modulator with photonic topological insulator made of metallic quantum wells

Abstract All-optical modulators hold significant prospects for future information processing technologies for they are able to process optical signals without the electro-optical convertor which limits the achievable modulation bandwidth. However, owing to the hardly-controlled optical backscattering in the commonly-used device geometries and the weak optical nonlinearities of the conventional material systems, constructing an all-optical modulator with a large bandwidth and a deep modulation depth in an integration manner is still challenging. Here, we propose an approach to achieving an on-chip ultrafast all-optical modulator with ultra-high modulation efficiency and a small footprint by using photonic topological insulators (PTIs) made of metallic quantum wells (MQWs). Since PTIs have attracted significant attention because of their unidirectional propagating edge states, which mitigate optical backscattering caused by structural imperfections or defects. Meanwhile, MQWs have shown a large Kerr nonlinearity, facilitating the development of minimally sized nonlinear optical devices including all-optical modulators. The proposed photonic topological modulator shows a remarkable modulation depth of 15 dB with a substantial modulation bandwidth above THz in a tiny footprint of only 4 × 10 µm2, which manifests itself as one of the most compact optical modulators compared with the reported ones possessing a bandwidth above 100 GHz. Such a high-performance optical modulator could enable new functionalities in future optical communication and information processing systems.

Si-CMOS compatible epsilon-near-zero metamaterial for two-color ultrafast all-optical switching

Driven by the escalating demands of advanced technologies, developing integration strategies has kept pace with the realization of ultrafast components during the past two decades. Ultrafast all-optical switches enabled by artificial materials are considered at the forefront of the next generation of photonic integration for communications and high-volume data processing. Encouraged by these advancements, applications, and interest have increased toward all-optical switches based on epsilon-near-zero (ENZ) materials. However, some all-optical switches lack CMOS compatibility, require high energy activation, and are limited in switching speed and working wavelength. Here, we propose and demonstrate a multilayered ENZ metamaterial utilizing Si-compatible titanium nitride and indium-tin-oxide materials with two effective working wavelengths in the visible and near-infrared spectrum. This device enables switching time down to a few hundred femtoseconds utilizing minimal energy at the corresponding ENZ regions induced by intraband pumping. Our approach can enhance the adaptability of designing ENZ metamaterials for new hybrid integrated photonic components for low-power ultrafast all-optical terahertz modulation.

Giant Ultrafast All-Optical Modulation Based on Exceptional Points in Exciton-Polariton Perovskite Metasurfaces.

Ultrafast all-optical modulation with optically resonant nanostructures is an essential technology for high-speed signal processing on a compact optical chip. Key challenges that exist in this field are relatively low and slow modulations in the visible range as well as the use of expensive materials. Here we develop an ultrafast all-optical modulator based on MAPbBr3 perovskite metasurface supporting exciton-polariton states with exceptional points. The additional angular and spectral filtering of the modulated light transmitted through the designed metasurface allows us to achieve 2500% optical signal modulation with the shortest modulation time of 440 fs at the pump fluence of ∼40 μJ/cm2. Such a value of the modulation depth is record-high among the existing modulators in the visible range, while the main physical effect behind it is polariton condensation. Scalable and cheap metasurface fabrication via nanoimprint lithography along with the simplicity of perovskite synthesis and deposition make the developed approach promising for real-life applications.

Nonlinear optical response and ultrafast all-optical modulation of Nb4C3.

MXenes exhibit a variety of unique electronic, optical, chemical, and mechanical properties. In this work, the nonlinear optical (NLO) properties of Nb4C3Tx are systematically investigated. The Nb4C3Tx nanosheets exhibit saturable absorption (SA) response from visible region to near-infrared region and better saturability under 6 ns pulse excitation than that under 380 fs excitation. The ultrafast carrier dynamics show a relaxation time of ∼6 ps, which suggests a high optical modulation speed of ∼160 GHz. Consequently, an all-optical modulator is demonstrated by transferring the Nb4C3Tx nanosheets to the microfiber. The signal light can be modulated well by pump pulses with a modulation rate of 5 MHz and an energy consumption of 12.564 nJ. Our study indicates that Nb4C3Tx is a potential material for nonlinear devices.

Polarization-resolved ultrafast all-optical terahertz micro-grating array modulator based on Weyl semimetallic microfilm towards 6G technology

The 6th generation (6G) of communication technology, defines 0.1–1 THz as the communication band. As a result, ultrafast modulation and multi-dimensional resolution coding technologies in the terahertz band pose a big challenge.In this work, a polarization-resolved ultrafast optical controlled terahertz modulator has been realized by combining tungsten ditelluride (WTe2) thin film with subwavelength metallic gratings.In the frequency range of 0.1–1.2 THz, which covers the 6G frequency band, the modulation depth of the device reaches up to 36.8% with a centimeter-scale effective area. An ultrafast response time of 0.95 ps is obtained due to the limitations of the grating for carrier degrees of freedom. In addition, the polarization sensitivity of terahertz waves polarized in the x- and y-direction is up to 0.77 due to the sub-wavelength grating structure. The results give a chance to develop the large-area, high-performance polarization-resolved ultrafast THz modulators based on Weyl semimetal, which could provide a reliable alternative for 6G communications equipment.

Polaritons in Van der Waals Heterostructures.

2D monolayers supporting a wide variety of highly confined plasmons, phonon polaritons, and exciton polaritons can be vertically stacked in van der Waals heterostructures (vdWHs) with controlled constituent layers, stacking sequence, and even twist angles. vdWHs combine advantages of 2D material polaritons, rich optical structure design, and atomic scale integration, which have greatly extended the performance and functions of polaritons, such as wide frequency range, long lifetime, ultrafast all-optical modulation, and photonic crystals for nanoscale light. Here, the state of the art of 2D material polaritons in vdWHs from the perspective of design principles and potential applications is reviewed. Some fundamental properties of polaritons in vdWHs are initially discussed, followed by recent discoveries of plasmons, phonon polaritons, exciton polaritons, and their hybrid modes in vdWHs. The review concludes with a perspective discussion on potential applications of these polaritons such as nanophotonic integrated circuits, which will benefit from the intersection between nanophotonics and materials science.

Ultrafast hot electron dynamics in plasmonic nanostructures: experiments, modelling, design

Abstract Metallic nanostructures exhibit localized surface plasmons (LSPs), which offer unprecedented opportunities for advanced photonic materials and devices. Following resonant photoexcitation, LSPs quickly dephase, giving rise to a distribution of energetic ‘hot’ electrons in the metal. These out-of-equilibrium carriers undergo ultrafast internal relaxation processes, nowadays pivotal in a variety of applications, from photodetection and sensing to the driving of photochemical reactions and ultrafast all-optical modulation of light. Despite the intense research activity, exploitation of hot carriers for real-world nanophotonic devices remains extremely challenging. This is due to the complexity inherent to hot carrier relaxation phenomena at the nanoscale, involving short-lived out-of-equilibrium electronic states over a very broad range of energies, in interaction with thermal electronic and phononic baths. These issues call for a comprehensive understanding of ultrafast hot electron dynamics in plasmonic nanostructures. This paper aims to review our contribution to the field: starting from the fundamental physics of plasmonic nanostructures, we first describe the experimental techniques used to probe hot electrons; we then introduce a numerical model of ultrafast nanoscale relaxation processes, and present examples in which experiments and modelling are combined, with the aim of designing novel optical functionalities enabled by ultrafast hot-electron dynamics.

Ultrafast low-pump fluence all-optical modulation based on graphene-metal hybrid metasurfaces

Graphene is an attractive material for all-optical modulation because of its ultrafast optical response and broad spectral coverage. However, all-optical graphene modulators reported so far require high pump fluence due to the ultrashort photo-carrier lifetime and limited absorption in graphene. We present modulator designs based on graphene-metal hybrid plasmonic metasurfaces with highly enhanced light-graphene interaction in the nanoscale hot spots at pump and probe (signal) wavelengths. Based on this design concept, we have demonstrated high-speed all-optical modulators at near and mid-infrared wavelengths (1.56 μm and above 6 μm) with significantly reduced pump fluence (1–2 orders of magnitude) and enhanced optical modulation. Ultrafast near-infrared pump-probe measurement results suggest that the modulators’ response times are ultimately determined by graphene’s ultrafast photocarrier relaxation times on the picosecond scale. The proposed designs hold the promise to address the challenges in the realization of ultrafast all-optical modulators for mid-and far-infrared wavelengths.

Ultrafast, All Optically Reconfigurable, Nonlinear Nanoantenna.

The enhancement of nonlinear optical effects via nanoscale engineering is a hot topic of research. Optical nanoantennas increase light–matter interaction and provide, simultaneously, a high throughput of the generated harmonics in the scattered light. However, nanoscale nonlinear optics has dealt so far with static or quasi-static configurations, whereas advanced applications would strongly benefit from high-speed reconfigurable nonlinear nanophotonic devices. Here we propose and experimentally demonstrate ultrafast all-optical modulation of the second harmonic (SH) from a single nanoantenna. Our design is based on a subwavelength AlGaAs nanopillar driven by a control femtosecond light pulse in the visible range. The control pulse photoinjects free carriers in the nanostructure, which in turn induce dramatic permittivity changes at the band edge of the semiconductor. This results in an efficient modulation of the SH signal generated at 775 nm by a second femtosecond pulse at the 1.55 μm telecommunications (telecom) wavelength. Our results can lead to the development of ultrafast, all optically reconfigurable, nonlinear nanophotonic devices for a broad class of telecom and sensing applications.

Ultrafast all-optical terahertz modulation based on an inverse-designed metasurface

Metasurface plays a key role in various terahertz metadevices, while the designed terahertz metasurface still lacks flexibility and variety. On the other hand, inverse design has drawn plenty of attention due to its flexibility and robustness in the application of photonics. This provides an excellent opportunity for metasurface design as well as the development of multifunctional, high-performance terahertz devices. In this work, we demonstrate that, for the first time, a terahertz metasurface supported by the electromagnetically induced transparency (EIT) effect can be constructed by inverse design, which combines the particle swarm optimization algorithm with the finite-difference time-domain method. Incorporating germanium (Ge) film with inverse-designed metasurface, an ultrafast EIT modulation on the picosecond scale has been experimentally verified. The experimental results suggest a feasibility to build the terahertz EIT effect in the metasurface through an optimization algorithm of inverse design. Furthermore, this method can be further utilized to design multifunctional and high-performance terahertz devices, which is hard to accomplish in a traditional metamaterial structure. In a word, our method not only provides a novel way to design an ultrafast all-optical terahertz modulator based on artificial metamaterials but also shows the potential applications of inverse design on the terahertz devices.

Ultrafast Magneto-Optics in Nickel Magnetoplasmonic Crystals.

Here, we report on ultrafast all-optical modulation of the surface-plasmon (SP)-assisted transverse magneto-optical Kerr effect (TMOKE) and the reflectance in a one-dimensional nickel magnetoplasmonic crystal (MPC). A 50 fs nonresonant laser pump pulse with 7 mJ/cm2 fluence reduces the magnetization by 65%, which results in the suppression of TMOKE in the SP-resonant probe from 1.15% to 0.4%. The differential reflectance of SP-resonant probe achieves 5.5%. Besides this, it is shown that electron thermalization and relaxation in MPC are several times slower than those in the plane nickel.

Efficient ultrafast all-optical modulation in a nonlinear crystalline gallium phosphide nanodisk at the anapole excitation.

High-refractive index nanostructured dielectrics have the ability to locally enhance electromagnetic fields with low losses while presenting high third-order nonlinearities. In this work, we exploit these characteristics to achieve efficient ultrafast all-optical modulation in a crystalline gallium phosphide (GaP) nanoantenna through the optical Kerr effect (OKE) and two-photon absorption (TPA) in the visible/near-infrared range. We show that an individual GaP nanodisk can yield differential reflectivity modulations of up to ~40%, with characteristic modulation times between 14 and 66 fs, when probed at the anapole excitation (AE). Numerical simulations reveal that the AE represents a unique condition where both the OKE and TPA contribute with the same modulation sign, maximizing the response. These findings highly outperform previous reports on sub-100-fs all-optical switching from resonant nanoscale dielectrics, which have demonstrated modulation depths no larger than 0.5%, placing GaP nanoantennas as a promising choice for ultrafast all-optical modulation at the nanometer scale.

CMOS-compatible all-optical modulator based on the saturable absorption of graphene

Graphene resting on a silicon-on-insulator platform offers great potential for optoelectronic devices. In the paper, we demonstrate all-optical modulation on the graphene–silicon hybrid waveguides (GSHWs) with tens of micrometers in length. Owing to strong interaction between graphene and silicon strip waveguides with compact light confinement, the modulation depth reaches 22.7% with a saturation threshold down to 1.38 pJ per pulse and a 30-μm-long graphene pad. A response time of 1.65 ps is verified by a pump–probe measurement with an energy consumption of 2.1 pJ. The complementary metal-oxide semiconductor compatible GSHWs with the strip configuration exhibit great potential for ultrafast and broadband all-optical modulation, indicating that employing two-dimensional materials has become a complementary technology to promote the silicon photonic platform.

非线性超构表面：谐波产生与超快调控

Metasurfaces refer to the optical nanoantenna arrays composed of subwavelength structures. Nanoantennas can have resonances under appropriate excitation conditions, to achieve near-field enhancement, and thus enhancing nonlinear optical effects. Compared with conventional nonlinear optical crystals, metasurfaces are more compact, with the possibility for on-chip integration. Due to the subwavelength light-matter interaction length, for applications such as nonlinear harmonic generation, metasurfaces does not suffer from the limitation of phase-matching. In addition, metasurfaces own the subwavelength spatial resolution. By designing and arranging the meta-atoms, metasurfaces can realize flexible control of the phase, polarization, and amplitude of the harmonic wave. Recent works on nonlinear metasurfaces for applications in optical frequency conversion, nonlinear wavefront control and ultrafast all-optical modulation were reviewed, the challenges and perspectives for the practical application of metasurfaces were presented.

Ultrafast All-Optical Signal Modulation Induced by Optical Kerr Effect in a Tellurite Photonic Bandgap Fiber

Ultrafast all-optical signal modulation induced by optical Kerr effect (OKE) was demonstrated in an all-solid tellurite photonic bandgap fiber (PBGF) which was designed and fabricated based on TeO2-Li2O-WO3-MoO3-Nb2O5 (TLWMN, high-index rods), TeO2-ZnO-Na2O-La2O3 (TZNL, background), and TeO2-ZnO-Li2O-K2O-Al2O3-P2O5 (TZLKAP, cladding) glasses. At the input of a control pulse with high intensity, OKE occurred in the tellurite PBGF and the transmission bands of the tellurite PBGF shifted. The signal at 1.57 μm transmitting in the fiber core can be ultrafast all-optically modulated by the ultrafast single pulse (200 kW, 200 fs) under OKE, where the modulation speed can reach 50 GHz, faster than some commercial LiNbO3 modulators. The results in this paper can be applied to multi-monitors, local area network, detectors, multi-sources, etc.

Ultrafast All-Optical Light Control with Tamm Plasmons in Photonic Nanostructures

Ultrafast all-optical modulators are crucial parts of prospective photonic devices. A number of plasmonic and dielectric nanostructures were nominated as candidates for integrated all-optical circuits. The key principle in the design of such devices is to engineer artificial optical resonances to increase the magnitude of modulation or to change the characteristic switching time. The major drawback is that the manufacturing becomes rather sophisticated. Here, we propose a method to tailor the ultrafast response of photonic crystal–metal nanostructures by employing a spectral shift of the Tamm-plasmon resonance. We show that for the absorbed pump fluence of 6 pJ reflectance of the sample at the near-infrared probe wavelength in the vicinity of the Tamm-plasmon resonance changes 25× stronger as compared with a bare metal film. Additionally, we show that by choosing a proper wavelength around the resonance a background-free reflectance modulation can be achieved. The characteristic pulse-limited switching time, in this case, is 150 fs.

Ultrafast all-optical plasmonic graphene modulator.

By utilizing the ultrafast dynamics of the photo-excited electrons in graphene, we theoretically present an ultrafast all-optical plasmonic modulator. With the help of an external pump, the femtosecond thermodynamics of the hot carriers can tune the Fermi level of the graphene sheet in less than 1ps, which is the dependence of the support for the surface plasmonic wave. This device shows the ability to operate from the near-infrared regime to the far-infrared spectrum with the extinction ratio over 10dB and the pump fluence of 0.41 mJ/cm2. Such an ultrafast modulator may pave the way for designing the ultrahigh speed integrated photonics circuits.

Concave Rectangle Photonic Crystal Ring Resonator for Ultra-Fast All-Optical Modulation

Abstract In this paper, an ultra-fast all-optical modulator, based on a new shape of nonlinear photonic crystal ring resonator, is designed and studied. Numerical methods such as plane wave expansion (PWE) and finite-difference time domain (FDTD) are used to perform simulations. The modulation technique consists of carrier light controlling by means of input light signal and Kerr effect. The investigation of extinction ratio and insertion loss within the carrier input power shows that the choice of 0.7 W is the optimal value of that power to ensure the tradeoff between both characteristics. The suggested modulator demonstrates an excellent extinction ratio about 20.8018, a very low insertion loss of −13.98 and a short switching time about 13.4 ps. According to the obtained results, the modulator can be considered as an ultra-fast and ultra-compact optical component.

All-optical retro-modulation for free-space optical communication.

This work presents device and system architectures for free-space optical and optical wireless communication at high data rates over multidirectional links. This is particularly important for all-optical networks, with high data rates, low latencies, and network protocol transparency, and for asymmetrical networks, with multidirectional links from one transceiver to multiple distributed transceivers. These two goals can be met by implementing a passive uplink via all-optical retro-modulation (AORM), which harnesses the optical power from an active downlink to form a passive uplink through retroreflection. The retroreflected optical power is modulated all-optically to ideally achieve terabit-per-second data rates. The proposed AORM architecture, for passive uplinks, uses high-refractive-index S-LAH79 hemispheres to realize effective retroreflection and an interior semiconductor thin film of CuO nanocrystals to realize ultrafast all-optical modulation on a timescale of approximately 770 fs. The AORM architecture is fabricated and tested, and ultimately shown to be capable of enabling multidirectional free-space optical communication with terabit-per-second aggregate data rates.

Hot-Electron-Assisted Femtosecond All-Optical Modulation in Plasmonics.

The optical Kerr nonlinearity of plasmonic metals provides enticing prospects for developing reconfigurable and ultracompact all-optical modulators. In nanostructured metals, the coherent coupling of light energy to plasmon resonances creates a nonequilibrium electron distribution at an elevated electron temperature that gives rise to significant Kerr optical nonlinearities. Although enhanced nonlinear responses of metals facilitate the realization of efficient modulation devices, the intrinsically slow relaxation dynamics of the photoexcited carriers, primarily governed by electron-phonon interactions, impedes ultrafast all-optical modulation. Here, femtosecond (≈190 fs) all-optical modulation in plasmonic systems via the activation of relaxation pathways for hot electrons at the interface of metals and electron acceptor materials, following an on-resonance excitation of subradiant lattice plasmon modes, is demonstrated. Both the relaxation kinetics and the optical nonlinearity can be actively tuned by leveraging the spectral response of the plasmonic design in the linear regime. The findings offer an opportunity to exploit hot-electron-induced nonlinearities for design of self-contained, ultrafast, and low-power all-optical modulators based on plasmonic platforms.