Ultracold Neutron Source Research Articles

External Moderation of Reactor Core Neutrons for Optimized Production of Ultra-Cold Neutrons

The ultra-cold neutron (UCN) source being commissioned at North Carolina State University’s PULSTAR reactor is uniquely optimized for UCN production in the former graphite-filled thermal column outside of the reactor pool. The source utilizes a remote moderation design, which is particularly well suited to the PULSTAR reactor because of its high thermal and epithermal neutron leakage from the core face. This large non-equilibrium flux from the core is efficiently transported to the UCN source through the specially designed beam port in order to optimize UCN production at any given reactor power. The increased distance to the source from the core also greatly limits the heat load on the cryogenic system. A MCNP (Monte Carlo N-Particle) model of this system was developed and is in good agreement with gold foil activation measurements using a test configuration as well as with the real UCN source’s heavy water moderator. These results established a firm baseline for estimates of the cold neutron flux available for UCN production and prove that remote moderation in a thermal column port is a valuable option for future designs of cryogenic UCN sources.

τSPECT: a spin-flip loaded magnetic ultracold neutron trap for a determination of the neutron lifetime

The confinement of ultracold neutrons (UCNs) in three-dimensional magnetic field gradient or magneto-gravitational traps allows for a measurement of the free neutron lifetime τ n with superior control over loss channels related to UCNs interacting with material surfaces. The most precise measurement τ n has been achieved using a magneto-gravitational trap, in which UCN are prevented from escaping at the top of their trap by gravity. More compact horizontal confinement geometries with variable energy acceptance ranges can be obtained by using steep magnetic field gradients in all spatial directions, generated by combinations of either permanent or (variable) superconducting magnets. In this paper, we present the first successful implementation of a pulsed spin-flip based loading scheme to fill a three-dimensional magnetic trap with externally produced UCN. The measurements with the τSPECT experiment were performed at the pulsed UCN source of the research reactor TRIGA Mainz. The extracted neutron storage time constant of τ = 859(16) s is compatible with the most precise determinations of τ n . We report on detailed, but statistically limited, investigations of major systematic effects influencing the neutron storage time. The statistical limitations are mitigated by the relocation of the experiment to a stronger UCN source.

ЭКСПЕРИМЕНТ ПО НИЗКОТЕМПЕРАТУРНОМУ ОБЛУЧЕНИЮ ПОРОШКА ФТОРИРОВАННЫХ ДЕТОНАЦИОННЫХ НАНОАЛМАЗОВ В РЕАКТОРЕ ВВР-К: УСЛОВИЯ И ПЕРВИЧНАЯ ХАРАКТЕРИЗАЦИЯ ОБРАЗЦОВ

Fluorine-doped detonation nanodiamond (DND) powders are considered as a new class of neutron reflectors and can significantly improve the performance of very cold and ultracold neutron sources, which in turn will lead to new types of experiments at a qualitative level. These improvements are achieved due to such properties of DNDas high diffusion and quasi-mirror reflection. The high reflectivity improves the neutron delivery efficiency and, consequently, the neutron fluxes at neutron facilities. On this basis, fluorinated DNDs are considered as a potential neutron reflector material for the designed very cold and ultracold neutron source at the WWR-K reactor. However, to date, experimental data on the behaviour of fluorinated DND in the neutron field are insufficient, and therefore, in order to study the radiation resistance of DND at the WWR-K reactor, work has been started on their irradiation and further study. For this purpose, an optimal irradiation capsule design was developed and comprehensive calculations were performed to justify the conditions and limits of reactor irradiation. This paper describes the irradiated samples and reactor experiment, the methodology and conditions for irradiating the samples, and the results of their initial characterisation after irradiation.

Moderator developments in HighNESS and feedback to compact sources design

The main, high-brightness neutron source for ESS is based on the low-dimensional moderator concept, and will serve the initial suite of neutron scattering instruments. In the HighNESS project several design options have been identified and investigated for a second source for ESS, intended to be complementary to the primary one. The emphasis of this project, completed in September 2023, was on the design of high-intensity sources, delivering Cold, Very Cold (VCN), and Ultra-Cold Neutrons (UCN). Remarkable results include: a cold moderator based on liquid deuterium capable of delivering an intensity close to a factor 10 greater than the ESS upper moderator; a VCN moderator based on solid deuterium at 5 K, surrounded by nanodiamond layers, delivering brightness above 40 Å an order of magnitude higher than a conventional cold moderator placed in the same location; and several design options for UCN sources based on the use of superfluid helium and solid deuterium. The use of these new sources would have a major impact on fundamental physics experiments and neutron scattering techniques. We investigate the possible impact that these concepts can have for compact sources, with particular emphasis on VCN.

Superfluid Helium Nased Ultracold Neutron Source for the PIK Reactor

Superfluid Helium Nased Ultracold Neutron Source for the PIK Reactor

Simulation of the Ultracold Neutron Source at the Reactor PIK

Simulation of the Ultracold Neutron Source at the Reactor PIK

Vertical time-of-flight spectroscopy of ultracold neutrons

This paper describes the mathematical basis for analysis of vertical time-of-flight (TOF) measurements with ultracold neutrons (UCN). In contrast to conventional horizontal TOF, this enables spectroscopy of UCN incident on the chopper with kinetic energies below the neutron optical potential of the detector entrance window. Much of the treatment presented here is general, and may be applied to horizontal and vertical TOF data of stationary and time-dependent spectra. Transformation rules are given for the conversion of vertical TOF spectra into other spectra of interest, and some aspects of detection efficiency are discussed that are common to all vertical TOF measurements using detectors with entrance windows. Throughout the paper, examples are provided using experimental data from measurements at the SUN-2 prototype superthermal UCN source. The technical details of these experiments and a comprehensive characterization of the source will be published by the present authors in a later paper.

Demonstration of sub-micron UCN position resolution using room-temperature CMOS sensor

High spatial resolution of ultracold neutron (UCN) measurement is of growing interest to UCN experiments such as UCN spectrometers, UCN polarimeters, quantum physics of UCNs, and quantum gravity. Here we utilize physics-informed deep learning to enhance the experimental position resolution and to demonstrate sub-micron spatial resolutions for UCN position measurements obtained using a room-temperature CMOS sensor, extending our previous work (Kuk et al., 2021; Yue et al., 2023) that demonstrated a position uncertainty of 1.5μm. We explore the use of the open-source software Allpix Squared to generate experiment-like synthetic hit images with ground-truth position labels. We use physics-informed deep learning by training a fully-connected neural network (FCNN) to learn a mapping from input hit images to output hit position. The automated analysis for sub-micron position resolution in UCN detection combined with the fast data rates of current and next generation UCN sources will enable improved precision for future UCN research and applications.

Time-of-flight spectroscopy of ultracold neutrons at the PSI UCN source

The ultracold neutron (UCN) source at the Paul Scherrer Institute (PSI) provides high intensities of storable neutrons for fundamental physics experiments. The neutron velocity spectrum parallel to the beamline axis was determined by time-of-flight spectroscopy using a neutron chopper. In particular, the temporal evolution of the spectrum during neutron production and UCN storage in the source storage volume was investigated and compared to Monte Carlo simulation results. A softening of the measured spectrum from a mean velocity of 7.7(1)–5.1(1) hbox {m s}^{-1} occurred within the first 30 hbox {s} after the proton beam pulse had impinged on the spallation target. A spectral hardening was observed over longer time scales of one measurement day, consistent with the effect of surface degradation of the solid deuterium moderator.

The HighNESS Project at the European Spallation Source: Current Status and Future Perspectives

The European Spallation Source (ESS), presently under construction in Lund, Sweden, is a multidisciplinary international laboratory that, once completed at full specifications, will operate the world’s most powerful pulsed neutron source. Supported by a 3 M Euro Research and Innovation Action within the European Union Horizon 2020 program, a design study (HighNESS) is now underway to develop a second neutron source located below the spallation target. Compared to the first source, which is located above the spallation target and designed for high cold and thermal brightness, the new source is being optimized to deliver higher intensity and a shift to longer wavelengths in the spectral regions of cold neutrons (CNs) (2 to 20 Å), very cold neutrons (VCNs) (10 to 120 Å), and ultracold neutrons (UCNs) ( > 500 Å). The second source consists of a large liquid deuterium moderator to deliver CNs and serve secondary VCN and UCN sources, for which different options are under study. These new sources will boost several areas of condensed matter research and will provide unique opportunities in fundamental physics. The HighNESS project is now entering its last year, and we are working toward the Conceptual Design Report of the ESS upgrade. In this paper, results obtained in the first 2 years, ongoing developments, and future perspectives are described.

Characterization of ultracold neutron production in thin solid deuterium films at the PSI Ultracold Neutron source

We determined the ultracold neutron (UCN) production rate by superthermal conversion in the solid deuterium $({\mathrm{sD}}_{2})$ moderator of the UCN source at the Paul Scherrer Institute (PSI). In particular, we considered low amounts of less than 20 mol of ${\mathrm{D}}_{2}$, deposited on the cooled moderator vessel surfaces in thin films of a few mm in thickness. We measured the isotopic $({c}_{\text{HD}}<0.2%)$ and isomeric $({c}_{\text{para}}\ensuremath{\le}2.7%)$ purity of the deuterium to conclude that absorption and up-scattering at 5 K have a negligible effect on the UCN yield from the thin films. We compared the calculated UCN yield based on the previously measured thermal neutron flux from the heavy water thermal moderator with measurements of the UCN count rates at the beamports. We confirmed our results and thus demonstrated an absolute characterization of the UCN production and transport in the source by simulations.

Development of UCN sources at PNPI

This article reviews the development of various sources for ultracold neutrons (UCNs) at the Petersburg Nuclear Physics Institute (PNPI). For 45 years, PNPI has proposed and manufactured cryogenic devices for neutron conversion to low energies. Based on beryllium, hydrogen and deuterium, they can be operated in the intense radiation fields near the core of a nuclear reactor. A more recently launched UCN source development utilizes superfluid helium (He-II) as conversion medium. Initially proposed and designed for PNPI’s old WWR-M reactor, the project has been reshaped to equip the institute’s PIK reactor with a modern UCN source of this type. The projected UCN density in the closed source chamber is 2.2 × 103 cm−3, which, as calculations of neutron transport show, will provide 200 cm−3 in the chambers of a neutron EDM spectrometer connected to the source by a UCN guide. Experiments at PNPI with a full-scale UCN source model have demonstrated that a heat load of 60 W can be removed from the He-II in the converter at a temperature of 1.37 K. This fact confirms the practical possibility to implement low-temperature converters under “in-pile” conditions with large heat inflows. The review concludes with a presentation of various proposed options for a He-II based UCN source at the European Spallation Source.

The source for ultra-cold neutrons at the FRM II

At the Forschungs-Neutronenquelle Heinz Maier-Leibnitz (FRM II) of the Technical University of Munich (TUM) a new source for ultra-cold neutrons (UCN) with a solid deuterium converter is currently under construction. This summary paper shall give an overview of the project and its current status. Research results concerning converter preparation, para-to-ortho conversion, radiation effects and neutron transport, which have been achieved in the last years, are presented and their relevance and transferability for the design of a future UCN source at the European Spallation Source (ESS) are discussed.

Concept and strategy of SuperSUN: A new ultracold neutron converter

A new source of ultracold neutrons (UCNs), developed at the Institut Laue-Langevin (ILL) and named SuperSUN, is currently being commissioned. Its operational principle is the conversion of cold neutrons, delivered by ILL’s existing beam H523, to UCNs in a vessel filled with superfluid helium-4, wherein the neutron’s energy and momentum are transferred by inelastic scattering to phonons in the superfluid. The inverse Boltzmann-suppressed process is negligible at temperatures below 0.6 K, enabling long storage times and high in-situ UCN densities as demonstrated at the ILL for two prototype sources. These two prototypes are installed at secondary beams behind crystal monochromators, whereas a primary beam with a white cold spectrum illuminates the SuperSUN conversion volume. This provides not only higher intensity around the wavelength 0.89 nm where the dominant single-phonon process for UCN production takes place, but also a contribution to UCN production by multi-phonon processes. In the first phase of the project, material walls will trap the UCNs, while in the second phase an octupole magnet will generate a 2.1 T magnetic field at the edge of the conversion volume. For low-field-seeking UCNs, this field increases the trapping potential and reduces wall losses so that the accumulated UCNs are spin-polarized as a result. SuperSUN aims to deliver the highest possible UCN densities to external storage experiments, the first of which will be the PanEDM experiment measuring the neutron’s permanent electric dipole moment.

Very cold and ultra cold neutron sources for ESS

The goal of the “Workshop on Very Cold and Ultra Cold Neutron Sources for ESS” was to discuss scientific cases, ideas and possibilities for the implementation of sources of Very Cold and Ultra Cold neutrons at the European Spallation Source. The ESS facility, presently under construction, offers several possibilities for in-pile UCN or VCN sources, in primis thanks to the available space below the spallation target where additional neutron sources can be placed to complement those above the target. Neutron beams can be extracted over a wide angular range with a grid of forty-two beamports with 6° average angular separation, allowing future instruments to be installed which may view either the upper or lower moderator systems. Of greatest interest for fundamental physics is the so-called Large Beamport foreseen for the NNBAR experiment. This beamport is also particularly well suited to feed a UCN source, for which several ideas were presented that employ either superfluid helium or solid deuterium as established neutron converter materials. Concepts for VCN sources make use of novel materials for VCN production and/or advanced reflectors to increase yields in the coldest part of the neutron spectrum from a cryogenic neutron source. In this paper we discuss these ideas and the possible locations of UCN and VCN sources at ESS.

In-beam superfluid-helium ultracold neutron source for the ESS

This paper discusses design principles and possible performances of an “in-beam” ultracold neutron (UCN) source for the European Spallation Source (ESS). The key components of the proposed neutron delivery system are nested-mirror optics (NMO), which image the bright neutron emission surface of the large liquid-deuterium moderator, studied within the HighNESS project, onto a remotely located superfluid-helium converter. Bandpass supermirrors, with optional polarization capability, enable the selective transport of those neutrons that are most effective for UCN production, exploiting the single-phonon conversion process that is possible for neutrons having wavelengths within a narrow range centered on 8.9 A ˚. NMO are capable of extracting and refocusing neutrons with small transport losses under the large solid angle available at the ESS Large Beam Port (LBP), allowing the converter to be placed far away from the high-radiation area in the ESS shielding bunker, where the source stays accessible for trouble-shooting while facilitating a low-background environment for nearby UCN experiments. Various configurations of the beam and converter are possible, including a large-volume converter – with or without a magnetic reflector – for a large total UCN production rate, or a beam focused onto a small converter for highest possible UCN density. The source performances estimated by first simulations of a baseline version presented in this paper, including a saturated UCN density on the order of 10 5 cm − 3 , motivate further study and the development of NMO beyond the first prototypes that have been recently investigated experimentally.

Workshop on very cold and ultra cold neutron sources for ESS

Workshop on very cold and ultra cold neutron sources for ESS

Why very cold neutrons could be useful for neutron-antineutron oscillation searches

This note is based on a talk given at the “Workshop on Very Cold and Ultra Cold Neutron Sources for ESS”. It presents several arguments in favor of using very cold neutrons (VCN) for neutron – antineutron ( n − n ‾) searches. It also proposes a scheme for the implementation of a solid-deuterium VCN converter with a fluorinated detonation nanodiamond (F-DND) reflector that is optimized for an ( n − n ‾) experiment with VCN. An analysis of the feasibility of such a source, as well as its effect on the ( n − n ‾) experiment are beyond the scope of this short note. They will, however, be pursued in the near future in a collaborative manner.

Production of ultracold neutrons in a decelerating trap

This note proposes a new concept for the production of ultracold neutrons (UCNs) in a decelerating trap. UCNs are widely used in the physics of elementary particles and fundamental interactions, and can potentially be used in studies of condensed matter. However, most of these studies are limited by the available UCN densities and fluxes. One of the ways to increase them is to extract more neutrons from the full phase space of a source and better exploit peak fluxes in pulsed neutron sources, orders of magnitude larger than the mean values. For instance, at ESS, the pulsed flux will be a factor of ∼25 larger than the mean flux of ILL at nominal power. Here, a concept of UCN sources is proposed, which allows to implement this idea. We propose to produce very cold neutrons (VCNs) in converters located in a neutron source, extract and slow them down to UCNs by a decelerating magnetic or material trap. As shown in this paper, for both pulsed and continuous neutron sources, this method could provide a high conversion efficiency of VCNs to UCNs with low losses of density in the phase space. More detailed calculations and the proposals for concrete technical designs are going to be developed in future publications.

Design of the 590 MeV proton beamline for the proposed TATTOOS isotope production target at PSI

IMPACT (Isotope and Muon Production with Advanced Cyclotron and Target Technologies) is a proposed initiative envisaged for the high-intensity proton accelerator facility (HIPA) at the Paul Scherrer Institute (PSI). As part of IMPACT, a radioisotope target station, TATTOOS (Targeted Alpha Tumour Therapy and Other Oncological Solutions) will allow the production of terbium radionuclides for therapeutic and diagnostic purposes. The proposed TATTOOS beamline and target will be located near the UCN (Ultra Cold Neutron source) target area, branching off from the main UCN beamline. In particular, the beamline is intended to operate at a beam intensity of 100 μA, requiring a continuous splitting of the main beam via an electrostatic splitter. Realistic beam loss simulations to verify safe operation have been performed and optimised using Beam Delivery Simulation (BDSIM), a Geant4 based tool enabling the simulation of beam transportation through magnets and particle passage through the accelerator. In this study, beam profiles, beam transmission and power deposits are generated and studied.