Type Ion Source Research Articles

Practical guides for x-ray photoelectron spectroscopy: Use of argon ion beams for sputter depth profiling and cleaning

Ion beams are used in x-ray photoelectron spectroscopy (XPS) to clean samples and perform compositional sputter depth profiles. The purpose of this article is to compile good practice, recommendations, and useful information related to the use of argon ion sources for inexperienced users of XPS instrumentation. The most used type of ion source generates monoatomic argon ions at a range of energies from a fixed direction relative to the instrument. The angle and direction of the ion beam with respect to the surface are normally altered by manipulating the sample, and this may involve tilting the sample to change the angle of incidence or rotating the sample to change the azimuthal incidence angle. Atomic argon ion beams cause damage to the structure of the material surface, which may exhibit itself as a change in stoichiometry or topography as well as the implantation of argon atoms. Therefore, caution is required in the interpretation of XPS depth profiles. Gas cluster ion sources offer new possibilities and choices to XPS users. Gas cluster sources enable the sputtering of organic materials with high yield in comparison to inorganic materials and offer the potential for nearly damage-free depth profiling of delicate organic materials as well as low damage cleaning of inorganic materials. It may be possible to use argon clusters to reduce damage during the depth profiling of inorganic materials, but there is currently insufficient evidence to make any general recommendations.

Ion source developments to supply mono & multi charged ion beams to the new NHa C400 hadrontherapy system.

Normandy Hadrontherapy (NHa) is developing, in collaboration with Ion Beam Applications (IBA), a full hadrontherapy treatment solution based on a new multiparticle cyclotron. 12C6+ and 4He2+ ions will be accelerated up to 400 MeV/u and (H2)+ up to 260 MeV/u. Three different ion sources will be carried out for each accelerated particle: the mono-charged ion source (H2)+ and low charged ion source He2+ are provided by the Polygon Physics (PP) company. The carbon ion source is under development at NHa in collaboration with IBA and PP. The (H2)+ ion source is an industrial Tubular ECR Source (TES) fitted for the needs of the NHa C400 cyclotron (30 µA of (H2)+). The He2+ ion source is a classic 10 GHz ECR type with a new concept because the complete source is set inside a vacuum chamber and it runs under 10−6 mbar of gas residual pressure. The 12C6+ ion source is also an ECR type ion source operating at 14.5 GHz frequency, its design is under progress to produce a beam providing stability and reproducibility levels compatible with clinical use. The article will present the External Injection System of the NHa C400 cyclotron hence it will focus on the experimental results obtained with the (H2)+ ion source and preliminary outputs from the He2+ ECRIS. A presentation of the multicharged ECRIS design dedicated to the 12C6+ production will be done.

Additively manufactured tantalum cathode for FEBIAD type ion sources: production, geometric measurements, and high temperature test

The Laser Powder Bed Fusion (LPBF) is an Additive Manufacturing (AM) technology suitable to produce almost free-form metallic components. At Legnaro National Laboratories (LNL) of the Italian National Institute for Nuclear Physics (INFN), the LPBF process was recently used to produce parts of the Forced Electron Beam Induced Arc Discharge (FEBIAD) ion source for the SPES Isotope Separation On-Line (ISOL) facility. In this work are presented the feasibility assessment and production steps of tantalum cathodes produced via AM; in addition, the results concerning both the dimensional-geometrical measurements and the preliminary high-temperature test are reported.

Targets and ion sources at CERN-ISOLDE — Facilities and developments

At the CERN-ISOLDE radioactive ion beam facility, thick targets are irradiated using a beam of 1.4-GeV protons. One of ISOLDE’s key features is the large choice of ion source types and target materials available, enabling us to select the ideal combination for optimal intensity and purity of the isotopes requested by ISOLDE users. The ever-increasing demands in terms of isotope production yield, beam purity, and overall reliability of the employed systems are driving the continuous development efforts.Over the past few years, CERN has invested heavily in facilities and infrastructure that facilitate ongoing developments required for ISOLDE. A dedicated offline laboratory (Offline 2) has been recently equipped with high repetition rate nanosecond tunable lasers required for scheme development and developments of specialized laser ion source types such as VADLIS, LIST and PI-LIST. Moreover, it hosts a twin setup of the ISOLDE RFQ cooler and buncher (ISCOOL), which is envisaged to be used for studies of molecular beam creation and breakup, as well as the development of improved RFQ services and operational modes. For material development, particularly for nanostructured materials, the new nano laboratory has just been commissioned and will enable the production and development of nano actinide targets for ISOLDE. In this contribution we describe the infrastructure required for target and ion source developments, highlight recent efforts and experimental results on both target material development and ion source development, and provide an outlook on what to expect in the near future.

3D computational fluid dynamics analysis of PINI ion source back plate under high heat flux condition

Neutral Beam Injection (NBI) plays an essential role in Tokamak plasma heating and current drive. A positive ion-based NBI (PNBI) system is adopted in Steady State Superconducting Tokamak- 1 (SST-1). This PNBI system is capable of generating neutral hydrogen beam power of 1.7 MW at 55 keV. This system has a JET PINI (Positive Ion Neutral Injector) type of ion source. The Back Plate (BP) is a component of the PINI ion source. It consists of an SS 304 L magnet positioning & cover plate, and an OFE copper cooling plate. The back plate plays a vital role in removing the high heat load intercepted during beam operation. The present study describes 3D Computational Fluid Dynamics (CFD) analysis of the actual size back plate using the ANSYS version of R121. The 3D CFD analysis has been done under a 2.5 MW/m2 steady heat load incident on the OFE copper plate. Cooling water is provided in the Inlet header of the back plate with a mass flow rate of 1 kg/s at 34 °C. The analysis gives the surface temperature distribution over the OFE copper cooling plate with a maximum surface temperature of 174 °C and the average temperature is 122 °C. This result is in good agreement with High Heat Flux experimental results.

Recent progresses on ion beam irradiation induced structure and performance modulation of two-dimensional materials.

Two-dimensional (2D) materials are receiving significant attention for both fundamental research and industrial applications due to their unparalleled properties and wide application potential. In this case, the controllable modulation of their structures and properties is essential for the realization and further expansion of their applications. Accordingly, ion beam irradiation techniques, with large scope to adjust parameters, high manufacturing resolution, and a series of advanced equipment being developed, have been demonstrated to have obvious advantages in manipulating the structure and performance of 2D materials. In recent years, many research efforts have been devoted to uncovering the underlying mechanism and control rules regarding ion irradiation induced phenomena in 2D materials, aiming at fulfilling their application potential as soon as possible. Herein, we review the research progress in the interaction between energetic ions and 2D materials based on the energy transfer model, type of ion source, structural modulation, performance modification of 2D materials, and then their application status, aiming to provide useful information for researchers in this field and stimulating more research advances.

Tungsten Electron Emitter (TE2) with direct heated cathode by plasma stream

At Goethe-University, a novel concept of heating metallic cathodes is currently under investigation. In the scope of the ARIES collaboration WP16, an RF-modulated electron gun was developed and manufactured for application in electron lenses for space charge compensation. The goal of this project is to increase the intensity of primary beams, especially in low energy booster synchrotrons like the SIS18 and SIS100 at GSI/FAIR or the SPS at CERN. The gun was designed to produce electron currents of 10 A at extraction voltages of 30 kV. The tungsten electron emitter (TE2) and the grid electrode were designed and manufactured to be integrated in the extractor of the original volume type ion source. Significant effort was put into a robust and flexible design with highly reliable key components. The cathode is heated by a plasma stream generated in the plasma chamber of the source. Different heating options of the cathode are currently being studied. This contribution presents the working principles of the electron gun and first measurements results of cathode heating.

Particle orbit optimization in the beam extraction region of a cold cathode PIG negative ion source for electrostatic tandem accelerators

When using a PIG (Penning Ion Gauge) type ion source for production of negative ions, these ions must be extracted from a hole on the side of the anode cylinder, perpendicularly to the magnetic field for plasma confinement. As a result, unnecessary deflection force works on the extracted beam. This study aims to improve the ion extraction efficiency of a cold-cathode PIG negative-ion source. The idea is to reduce the beam loss by cancelling the stray magnetic field from the source by placing small dipole magnets in the extraction electrode. Through the measurement of the magnetic field distribution and beam trajectory calculation, it was numerically confirmed that the beam trajectory can be corrected by this small dipole magnet with a peak magnetic field of about 50 mT under the present experimental condition.

Effects of axial magnetic field in a magnetic multipole line cusp ion source

Experiments have been performed to study the effects of axial magnetic field on plasma and ion beam parameters in a magnetic multipole line cusp ion source. Studies performed on ring cusp and Kaufmann type ion sources suggest that the axial component of magnetic field may help in improving the ion extraction current at a low discharge power. The line cusps ion sources have been used since long to produced uniform beams, however, they lack axial component of the magnetic field. These ion sources generally suffer from low efficiency possibly due the absence of axial magnetic field. In this work, an additional magnetic coil is added at various axial positions between the back-plate and the plasma grid of the multipole line cusp ion source. We have investigated the effects of axial magnetic field on the discharge efficiency and source parameters like beam current and uniformity in the multipole line cusp ion source. The beam profiles are obtained using an eleven-channel faraday cup array to estimate the effects of the axial magnetic field on beam uniformity and divergence. Initial studies suggest a reduction of beam divergence with increasing axial magnetic field. A significant rise in the beam current and the discharge current is also observed when the axial magnetic field is increased. Particle trajectory simulation using the CST-Studio suite is utilised in understanding the role of confinement of primary electrons behind the improved performance of the ion source.

Design and first operations of a ECR based He source at INFN-LNS

A new source for the TANDEM accelerator of LNS has been designed and installed. It is called NESTOR (Noble Elements Source for acceleraTORs) and consists of an ultra-compact ECR microwave discharge type ion source [1] operating around 6 GHz and up to 40 W of RF power, provided by a solid state power amplifier, coupled to a Li-Charge Exchange Cell (Li-CEC). It is engineered for the production of a wide range of 1+ and/or 1- ion beams from gaseous elements, in particular for noble gases. This work presents the characterization of the primary source and first operations of the whole setup on the HV platform (injector) of the Tandem. The He+ beams have been formerly characterized in terms of current, beam shape (by BaF2 beam viewers) and emittance (by the three-gradients method). Measurements have been carried out varying pressure, microwave frequency and RF power. Then, the source has been moved to the HV platform, coupled to the Li-CEC for first operations running in gas-exchange mode. Activities are ongoing to optimize beam transport towards the Tandem.

High-current H2 + beams from a filament-driven multicusp ion source.

We report the results from a new multicusp ion source (MIST-1) that produces record steady-state currents of H2 + (1 mA) from this type of ion source with high purity (80% H2 +). We built MIST-1 to fulfill the stringent beam purity and beam quality requirements for IsoDAR, a proposed discovery-level neutrino experiment, requiring a 10 mA, 60 MeV/amu continuous wave (cw) proton beam on the target. IsoDAR will use a cyclotron accelerating H2 + ions and using a novel radio frequency quadrupole (RFQ) direct injection method. Systematic measurements, varying discharge voltage, discharge current, and gas pressure, indicate that the ideal operating regime is at low pressure, high discharge current, and high discharge voltage. We have measured the combined species emittance after the source extraction to be <0.05 π-mm-mrad (rms, normalized) for a 0.95 mA beam. Beyond showing high currents and high H2 + fraction, our measurements agree well with high fidelity simulations. These results show the feasibility of using a multicusp ion source for IsoDAR and the RFQ direct injection prototype and paves the way to record breaking cw beam currents of 5 mA H2 + (equivalent to 10 mA protons) from compact cyclotrons, ideal for underground installation.

Highly Efficient Small Anode Ion Source

We describe some modifications to a Bernas-type ion source that improve the ion beam production efficiency and source operating lifetime. The ionization efficiency of a Bernas type ion source has been improved by using a small anode that is a thin rod, oriented along the magnetic field. The transverse electric field of the small anode causes the plasma to drift in the crossed ExB field to the emission slit. The cathode material recycling was optimized to increase the operating lifetime, and the wall potential optimized to suppress deposition of material and subsequent flake formation. A three-electrode extraction system was optimized for low energy ion beam production and efficient space charge neutralization. An ion beam with emission current density up to 60 mA/cm2 has been extracted from the modified source running on BF3 gas. Space charge neutralization of positive ion beams was improved by injecting electronegative gases.

DISCHARGE CHARACTERISTICS OF COMBINED LOW ENERGY ION SOURCE – MAGNETRON SPUTTERING SYSTEM

The discharge characteristics of a new combined low energy magnetron-ion-source sputtering system are presented. The ignition curves, current-voltage characteristics of the system in dependence on gas pressure, magnitude and topology of magnetic field have been researched both for autonomous operation of the planar magnetron discharge and Hall type ion source in plasma mode and for their combination. Spatial distributions of ion current are also presented.

Hydrochemistry Differences and Causes of Tectonic Lakes and Glacial Lakes in Tibetan Plateau

The Tibetan Plateau has the largest lake cluster in China and in the world. In order to clarify the differences of lake hydrochemistry of Tibetan Plateau, water samples were collected from 32 lakes, including 22 tectonic lakes and 11 glacial lakes, along the Tibetan Plateau road, from September to October 2016. We detected and analyzed the major ion concentrations and characteristics of samples, and discuss the hydrochemistry type, controlling factors, and major ion sources of lake water. The results showed that, firstly, tectonic lake samples on the Tibetan Plateau have much higher physicochemical parameters and ion contents than glacial lakes, and Total Dissolved Solids (TDS) contents fluctuate from high to low latitudes. The variations of ion concentrations in the northern part of the Qiagui Co were more fluctuating and have two obvious peaks, while the variations in the southern part were moderate. The TDS of glacial lakes were low and leveling off in the upper and middle reaches of the basin, while higher and more variable in the lower reaches. Secondly, the tectonic lakes were mainly chloride saline lakes, with Na+ as the major cation, and SO42−, Cl− as the major anions. Glacial lakes were mainly carbonate and sulfate type lakes, Ca2+ and Mg2+ were the major cations, HCO3− was the major anion, and SO42− was the second. Thirdly, the hydrochemistry processes of the tectonic lakes were mainly controlled by evaporation-crystallization, and the ions mainly came from the evaporites of basin. Glacial lake water samples were mainly influenced by the weathering of basin rocks, with ion sources strongly influenced by the weathering of basin carbonates than evaporites, with calcite and dolomite being important sources of Ca2+, Mg2+, and HCO3−.

A new Collinear Apparatus for Laser Spectroscopy and Applied Science (COALA).

We present a new collinear laser spectroscopy setup that has been designed to overcome systematic uncertainty limits arising from high-voltage and frequency measurements, beam superposition, and collisions with residual gas that are present in other installations utilizing this technique. The applied methods and experimental realizations are described, including an active stabilization of the ion-source potential, new types of ion sources that have not been used for collinear laser spectroscopy so far, dedicated installations for pump-and-probe measurements, and a versatile laser system referenced to a frequency comb. The advanced setup enables us to routinely determine transition frequencies, which was so far demonstrated only for a few cases and with lower accuracy at other facilities. It has also been designed to perform accurate high-voltage measurements for metrological applications. Demonstration and performance measurements were carried out with Ca+ and In+ ions.

Deuterium experiment with large-scale negative ion source for large helical device

The deuterium experiment with various source plasma diagnostics was conducted at the research and development negative ion source at National Institute for Fusion Science, which is a cesium-seeded large-scale negative hydrogen-ion source with half discharge volume and the same type of ion source for large helical device. A change of filling gas from hydrogen to deuterium increased line-averaged negative ion density by a factor of 1.3 in beam extraction region as a result of flattened profile with keeping central density. Positive ion and electron densities increased threefold. This was influenced by the increase of plasma density in the plasma generation region. The plasma space potential varied as equivalent of the collisionless sheath theory in electro-positive plasma expected by the hydrogen isotope gas species, although the negative ion could affect sheath formation. Higher atomic cesium density was observed because of higher sputtering yield due to higher momentum of deuterium.

A Cost-Effective Microwave Ion Source Test Stand

Turkish Accelerator Center (TAC) Proton Accelerator Facility (PAF) is a project proposal that aims to build a megawatt (MW) power proton accelerator in Turkey. The proton source of this project was chosen as a microwave discharge ion source due to its long life time, its high current, and its lower maintenance requirements when compared with other ion source types. A microwave discharge ion source test stand was built to gain experience for TAC PAF and for similar projects requiring high beam current in Turkey. A magnetron with 2.45-GHz frequency, 50-Hz repetition rate, and 150-W fixed power was used to create the hydrogen plasma. Two different electrode systems were experimented: the first design consists of 2-mm radius plasma electrode that extracts beam currents up to 0.75 mA and the second design consists of 4-mm radius plasma electrode that extracts beam currents up to 5.2 mA.

Overview of high intensity ion source development in the past 20 years at IMP.

Ion source development over the last 20 years at the IMP is reviewed. For versatile purposes, several types of ion sources have been involved in the research and development work at the IMP, i.e., the highly charged ECR (Electron Cyclotron Resonance) ion source, intense microwave ion source or the 2.45 GHz intense beam ECR ion source, and laser ion source (LIS). In the development of ECR ion sources, SECRAL (Superconducting ECR ion source with Advanced design in Lanzhou), Lanzhou ECR ion source, and Lanzhou all permanent magnet ECR ion source series have been made, which can cover the operation microwave frequency range of 10-28 GHz. The LIS with an Nd:YAG laser with a maximum output energy of 8 J in 8 ns pulse duration has been developed for very intense short pulse ion beams from solid materials such as C, Ti, Ni, Ag, and so on. Microwave ion sources have been built to produce intense pulsed or direct current beams from several mA to 100 mA for either high intensity accelerators or applications. This paper will give an overview of the high intensity ion source development at the IMP, especially on the recent progress and new results, such as the status of the fourth generation ECR ion source (first fourth generation ECR ion source), the production of recorded highly charged ion beams with SECRAL sources, key technology research studies, and so on.

Effect of focused ion beam process parameter on Tin-Nickel-Copper micropillars microfabrication

ABSTRACTIn this work, the mechanism of focused ion beam (FIB) milling as an advanced manufacturing technique is studied to pattern micropillars at different diameter sizes of 5, 10 and 20 μm. Under the same type of ion source which is Ga ion, the main ion beam parameters that influenced the FIB machining to produce micropillars are the ion beam scanning, dose, profile, and incident angle. The mathematical modeling is presented to describe the micropillars’ production by crater sputtering of the FIB milling. The effect of sputtering and redeposition on the final geometrical micropillars suggest the arrangement of the multilayer sample (Sn/Ni/Cu) that close to the ion irradiation gets highly sputtered and redeposited despite the surface binding energy and sputtering yield, ϒ of each element is known. Results show that the highest aspect ratio values are derived from the lowest diameter size of the micropillars produced from the FIB machining.

Considerations for the nano aperture ion source: Geometrical design and electrical control.

A new type of ion source is being developed for proton beam writing and other focused ion beam applications. The potential of this source as well as achieved performance of the nano aperture ion source will be evaluated. Based on the ideal source parameters, critical geometrical parameters constraining chromatic aberrations and a possible pathway to achieve this performance will be presented. Finally, an electronic control system to minimize chromatic and spherical aberrations to an acceptable level will be demonstrated.