Two-photon Wavefunction Research Articles

Quantum vortices of strongly interacting photons

Vortices are topologically nontrivial defects that generally originate from nonlinear field dynamics. All-optical generation of photonic vortices—phase singularities of the electromagnetic field—requires sufficiently strong nonlinearity that is typically achieved in the classical optics regime. We report on the realization of quantum vortices of photons that result from a strong photon-photon interaction in a quantum nonlinear optical medium. The interaction causes faster phase accumulation for copropagating photons, producing a quantum vortex-antivortex pair within the two-photon wave function. For three photons, the formation of vortex lines and a central vortex ring confirms the existence of a genuine three-photon interaction. The wave function topology, governed by two- and three-photon bound states, imposes a conditional phase shift of π per photon, a potential resource for deterministic quantum logic operations.

Characterizing and Tailoring Spatial Correlations in Multimode Parametric Down-Conversion

Photons entangled in their position-momentum degrees of freedom serve as an elegant manifestation of the Einstein-Podolsky-Rosen paradox, while also enhancing quantum technologies for communication, imaging, and computation. The multimode nature of photons generated in parametric down-conversion has inspired a generation of experiments on high-dimensional entanglement, ranging from complete quantum state teleportation to exotic multipartite entanglement. However, precise characterization of the underlying position-momentum state is notoriously difficult due to limitations in detector technology, resulting in a slow and inaccurate reconstruction riddled with noise. Furthermore, theoretical models for the generated two-photon state often forgo the importance of the measurement system, resulting in a discrepancy between theory and experiment. Here we formalize a description of the two-photon wave function in the spatial domain, referred to as the collected joint-transverse momentum amplitude (JTMA), which incorporates both the generation and measurement system involved. We go on to propose and demonstrate a practical and efficient method to accurately reconstruct the collected JTMA using a simple phase-step scan known as the $2D\ensuremath{\pi}$ measurement. Finally, we discuss how precise knowledge of the collected JTMA enables us to generate tailored high-dimensional entangled states that maximize discrete-variable entanglement measures such as entanglement of formation or entanglement dimensionality, and optimize critical experimental parameters such as photon heralding efficiency. By accurately and efficiently characterizing photonic position-momentum entanglement, our results unlock its full potential for discrete-variable quantum information science and lay the groundwork for future quantum technologies based on multimode entanglement.

Semiparametric estimation of the Hong-Ou-Mandel profile

We apply the theory of semiparametric estimation to a Hong-Ou-Mandel interference experiment with a spectrally entangled two-photon state generated by spontaneous parametric downconversion. Thanks to the semiparametric approach we can evaluate the Cram\'er-Rao bound and find an optimal estimator for a particular parameter of interest without assuming perfect knowledge of the two-photon wave function, formally treated as an infinity of nuisance parameters. In particular, we focus on the estimation of the Hermite-Gauss components of the marginal symmetrised wavefunction, whose Fourier transform governs the shape of the temporal coincidence profile. We show that negativity of these components is an entanglement witness of the two-photon state.

Distinguishability and "which pathway" information in multidimensional interferometric spectroscopy with a single entangled photon-pair.

Correlated photons inspire abundance of metrology-related platforms, which benefit from quantum (anti-) correlations and outperform their classical counterparts. While these mainly focus on entanglement, the role of photon exchange phase and degree of distinguishability has not been widely used in quantum applications. Using an interferometric setup, we theoretically show that, when a two-photon wave function is coupled to matter, it is encoded with “which pathway?” information even at low-degree of entanglement. An interferometric protocol, which enables phase-sensitive discrimination between microscopic interaction histories (pathways), is developed. We find that quantum light interferometry facilitates utterly different set of time delay variables, which are unbound by uncertainty to the inverse bandwidth of the wave packet. We illustrate our findings on an exciton model system and demonstrate how to probe intraband dephasing in the time domain without temporally resolved detection. The unusual scaling of multiphoton coincidence signals with the applied pump intensity is discussed.

Unraveling Two-Photon Entanglement via the Squeezing Spectrum of Light Traveling through Nanofiber-Coupled Atoms.

We observe that a weak guided light field transmitted through an ensemble of atoms coupled to an optical nanofiber exhibits quadrature squeezing. From the measured squeezing spectrum we gain direct access to the phase and amplitude of the energy-time entangled part of the two-photon wave function which arises from the strongly correlated transport of photons through the ensemble. For small atomic ensembles we observe a spectrum close to the line shape of the atomic transition, while sidebands are observed for sufficiently large ensembles, in agreement with our theoretical predictions. Furthermore, we vary the detuning of the probe light with respect to the atomic resonance and infer the phase of the entangled two-photon wave function. From the amplitude and the phase of the spectrum, we reconstruct the real and imaginary part of the time-domain wave function. Our characterization of the entangled two-photon component constitutes a diagnostic tool for quantum optics devices.

Stokes–anti-Stokes light-scattering process: A photon-wave-function approach

The Photon wave function Formalism provides an alternative description of some quantum optical phenomena in a more intuitive way. We use this formalism to describe the process of correlated Stokes--anti-Stokes Raman scattering. In this process, two photons from a laser beam are inelastically scattered by a phonon created by the first photon (Stokes processes) and annihilated by the second photon (anti-Stokes process), producing a Stokes--anti-Sokes (SaS) photon pair. We arrive at an expression for the two-photon wave function of the scattered SaS photon pair, which is in agreement with a number of experimental results.

Engineering two-photon wavefunction and exchange statistics in a semiconductor chip

High-dimensional entangled states of light provide novel possibilities for quantum information, from fundamental tests of quantum mechanics to enhanced computation and communication protocols. In this context, the frequency degree of freedom combines the assets of robustness to propagation and easy handling with standard telecommunication components. Here, we use an integrated semiconductor chip to engineer the wavefunction and exchange statistics of frequency-entangled photon pairs directly at the generation stage, without post-manipulation. Tailoring the spatial properties of the pump beam allows generating frequency-anticorrelated, correlated and separable states, and to control the symmetry of the spectral wavefunction to induce either bosonic or fermionic behaviors. These results, obtained at room temperature and telecom wavelength, open promising perspectives for the quantum simulation of fermionic problems with photons on an integrated platform, as well as for communication and computation protocols exploiting antisymmetric high-dimensional quantum states.

Measuring the frequency-time two-photon wavefunction of narrowband entangled photons from cold atoms via stimulated emission

Cold atom based narrowband entangled photon sources are important for efficient atom–photon interaction, which is at the heart of long-distance quantum communication and quantum memory protocols. Complete characterization of the narrowband entangled photons requires acquiring the frequency-time two-photon wavefunction, involving both joint temporal intensity (JTI) and joint temporal phase (JTP) measurements. Here, we demonstrate stimulated emission tomography of the frequency-time two-photon wavefunction of narrowband entangled photons from cold atoms. We show more than six orders of magnitude (×106) improvement in the measurement time for obtaining JTI and JTP compared to the conventional direct photon counting method, thus paving the way toward ultrafast high-resolution quantum tomography of photonic quantum states.

Generation of high spectral purity photon-pairs with MgO-doped periodically poled lithium niobate

We study the spectral correlation of photon pairs generated via type-II spontaneous parametric down conversion in periodically poled lithium niobate crystals. By performing Schmidt decomposition on the two-photon wavefunction, we calculate the spectral purity of the two-photon state under various pump laser characteristics and doping concentrations of MgO in lithium niobate crystals. Our results show that periodically poled 5% MgO doped lithium niobate is a good candidate to generate photon-pairs with high spectral purity at telecom wavelength.

Ensemble-Averaged Quantum Correlations between Path-Entangled Photons Undergoing Anderson Localization.

We measure ensemble-averaged quantum correlations of path-entangled photons, propagating in a disordered lattice and undergoing Anderson localization. These result in intriguing patterns, which show that quantum interference leads to unexpected dependencies of the location of one particle on the location of the other. These correlations are shared between localized and nonlocalized components of the two-photon wave function, and, moreover, yield information regarding the nature of the disorder itself. Such effects cannot be reproduced with classical waves, and are undetectable without ensemble averaging.

Dipolar Dephasing of Rydberg D-State Polaritons.

We experimentally study the effects of the anisotropic Rydberg interaction on D-state Rydberg polaritons slowly propagating through a cold atomic sample. We observe the interaction-induced dephasing of Rydberg polaritons at very low photon input rates into the medium. We develop a model combining the propagation of the two-photon wave function through our system with nonperturbative calculations of the anisotropic Rydberg interaction to show that the observed effect can be attributed to pairwise interaction of individual Rydberg polaritons at distances larger than the Rydberg blockade.

Attractive photons in a quantum nonlinear medium

The fundamental properties of light derive from its constituent particles--massless quanta (photons) that do not interact with one another. However, it has long been known that the realization of coherent interactions between individual photons, akin to those associated with conventional massive particles, could enable a wide variety of novel scientific and engineering applications. Here we demonstrate a quantum nonlinear medium inside which individual photons travel as massive particles with strong mutual attraction, such that the propagation of photon pairs is dominated by a two-photon bound state. We achieve this through dispersive coupling of light to strongly interacting atoms in highly excited Rydberg states. We measure the dynamical evolution of the two-photon wavefunction using time-resolved quantum state tomography, and demonstrate a conditional phase shift exceeding one radian, resulting in polarization-entangled photon pairs. Particular applications of this technique include all-optical switching, deterministic photonic quantum logic and the generation of strongly correlated states of light.

Photon blockade induced by atoms with Rydberg coupling

We study the photon blockade of two-photon scattering in a one-dimensional waveguide, which contains two atoms coupled via the Rydberg interaction. We obtain the analytic scattering solution of photonic wave packets with the Laplace transform method. We examine the photon correlation by addressing the two-photon relative wave function and the second-order correlation function in the single- and two-photon resonance cases. It is found that, under the single-photon resonance condition, photon bunching and antibunching can be observed in the two-photon transmission and reflection, respectively. In particular, the bunching and antibunching effects become stronger with the increasing of the Rydberg coupling strength. In addition, we find a phenomenon of bunching-antibunching transition caused by the two-photon resonance.

Optimization of two-photon wave function in parametric down conversion by adaptive optics control of the pump radiation

We present an efficient method for optimizing the spatial profile of entangled-photon wave function produced in a spontaneous parametric down conversion process. A deformable mirror that modifies a wavefront of a 404nm CW diode laser pump interacting with a nonlinear β-barium borate type-I crystal effectively controls the profile of the joint biphoton function. The use of a feedback signal extracted from the biphoton coincidence rate is used to achieve the optimal wavefront shape. The optimization of the two-photon coupling into two, single spatial modes for correlated detection is used for a practical demonstration of this physical principle.

Analysis of the time-energy entanglement of down-converted photon pairs by correlated single-photon interference

The time-energy entanglement of down-converted photon pairs is particularly difficult to characterize because direct measurements of photon arrival times are limited by the temporal resolution of photon detection. Here, we explore an alternative possibility of characterizing the temporal coherence of two-photon wavefunctions using single photon interference with weak coherent light. Specifically, this method makes use of the fact that down-conversion generates a coherent superposition of vacuum and two-photon states, so that the coincidence count rates for photon pairs after interference with weak coherent light are given by a superposition of the two-photon wavefunction from the down-conversion with the product wavefunction defined by the weak coherent references. By observing the frequency dependent interference pattern, it is possible to reconstruct the amplitudes and the phases of the two-photon wavefunction within the bandwidth of the reference pulses used in the single photon interferences. The correlated single photon interferences therefore provide a direct map of the entangled two-photon wavefunction generated in the down-conversion process.

Amplitude and phase modulation of time-energy entangled two-photon states

We experimentally demonstrate amplitude and phase modulation of a time-energy entangled two-photon wave function. The entangled photons are produced by spontaneous parametric down-conversion, spectrally dispersed in an prism compressor, modulated in amplitude and/or phase, and detected in coincidence by sum-frequency generation. First, we present a Fourier optical analysis of the optical setup yielding an analytic expression for the resulting field distribution at the exit plane of the shaping apparatus. We then introduce amplitude and/or phase shaping and present results which can only be obtained through a combination of the two. Specifically, we use a shaper-based interferometer to measure the two-photon interference of an almost bandwidth-limited two-photon wave function.

Two-photon wave mechanics

The position-representation wave function for multiphoton states and its equation of motion are introduced. A major strength of the theory is that it describes the complete evolution (including polarization and entanglement) of multiphoton states propagating through inhomogeneous media. As a demonstration of the two-photon wave function's use, we show how two photons in an orbital-angular-momentum entangled state decohere upon propagation through a turbulent atmosphere.

TWO-PHOTON NONLINEAR INTERACTION MEDIATED BY CAVITY QUANTUM ELECTRODYNAMICS SYSTEMS

Exploiting the field-amplification effect of a cavity, the possibility of optical nonlinearity by only two photons was indicated experimentally. In the present article, we review our recent analysis of the two-photon dynamics in a cavity quantum electrodynamics (QED) system. Since a cavity-QED system is highly dispersive around its resonances, the shapes of photonic pulses are significantly deformed through interaction with the system. Thus, the present analysis is based on a formalism beyond single-mode approximations. The external photon field is treated rigorously as a continuum, which enables us to handle the two-photon wavefunction in the space representation. The degree of optical nonlinearity in a two-photon state is quantified by comparing the output wavefunction with the linear output wavefunction. It is revealed that the semiclassical optical response theory can be applied for evaluation of the two-photon optical nonlinearity. The two-photon nonlinearity appears not purely as a phase shift in the output wavefunction. The degradation of the fidelity between the output wavefunction and the linear output wavefunction always occurs, which hinders the application of this nonlinear effect as a quantum phase gate. The optimum condition for maximizing the two-photon nonlinearity is clarified, suggesting that pulse shape control is more essential than the Q-value control of the cavity QED system.

Phase-modulated shaping of narrowband type-I parametric down-converted photons

We present a general theoretical description of the temporal shaping of narrowband noncollinear type-I down-converted photons using a spectral phase filter with a symmetric phase distribution. By manipulating the spectral phase of the signal or idler photon, we demonstrate control of the correlation time and shape of the two-photon wavefunction with modulation frequency and modulation depth of the phase distribution.

Temporal Shaping of Entangled Photons

We experimentally demonstrate shaping of the two-photon wave function of entangled-photon pairs, utilizing coherent pulse-shaping techniques. By performing spectral-phase manipulations we tailor the second-order correlation function of the photons exactly like a coherent ultrashort pulse. To observe the shaping we perform sum-frequency generation with an ultrahigh flux of entangled photons. At the appropriate conditions, sum-frequency generation performs as a coincidence detector with an ultrashort response time (approximately 100 fs), enabling a direct observation of the two-photon wave function. This property also enables us to demonstrate background-free, high-visibility two-photon interference oscillations.