Two-photon Interferometry Research Articles

Plug-and-Play Measurement of Chromatic Dispersion by Means of Two-Photon Interferometry

Plug-and-Play Measurement of Chromatic Dispersion by Means of Two-Photon Interferometry

Astrometry in two-photon interferometry using an Earth rotation fringe scan

Optical interferometers may not require a phase-stable optical link between the stations if instead sources of quantum-mechanically entangled pairs could be provided to them, enabling long baselines. We developed a new variation of this idea, proposing that photons from two different astronomical sources could be interfered at two decoupled stations. Interference products can then be calculated in post-processing or requiring only a slow, classical connection between stations. In this work, we investigated practical feasibility of this approach. We developed a Bayesian analysis method for the earth rotation fringe scanning technique and showed that in the limit of high signal-to-noise ratio it reproduced the results from a simple Fisher matrix analysis. We identify candidate stair pairs in the northern hemisphere, where this technique could be applied. With two telescopes with an effective collecting area of $\sim 2$ m$^2$, we could detect fringing and measure the astrometric separation of the sources at $\sim 10\,\mu$as precision in a few hours of observations, in agreement with previous estimates.

Attosecond dynamics of multi-channel single photon ionization

Photoionization of atoms and molecules is one of the fastest processes in nature. The understanding of the ultrafast temporal dynamics of this process often requires the characterization of the different angular momentum channels over a broad energy range. Using a two-photon interferometry technique based on extreme ultraviolet and infrared ultrashort pulses, we measure the phase and amplitude of the individual angular momentum channels as a function of kinetic energy in the outer-shell photoionization of neon. This allows us to unravel the influence of channel interference as well as the effect of the short-range, Coulomb and centrifugal potentials, on the dynamics of the photoionization process.

Quantum-clustered two-photon walks

We demonstrate a previously unknown two-photon effect in a discrete-time quantum walk. Two identical bosons with no mutual interactions nonetheless can remain clustered together as they walk on a lattice of directionally-reversible optical four-ports acting as Grover coins; both photons move in the same direction at each step due to a two-photon quantum interference phenomenon reminiscent of the Hong-Ou-Mandel effect. The clustered two-photon amplitude splits into two localized parts, one oscillating near the initial point, and the other moving ballistically without spatial spread, in soliton-like fashion. But the two photons are always clustered in the same part of the superposition, leading to potential applications for transport of entanglement and opportunities for novel two-photon interferometry experiments.

Quantum frequency combs and Hong-Ou-Mandel interferometry: the role of spectral phase coherence.

The Hong-Ou-Mandel interferometer is a versatile tool for analyzing the joint properties of photon pairs, relying on a truly quantum interference effect between two-photon probability amplitudes. While the theory behind this form of two-photon interferometry is well established, the development of advanced photon sources and exotic two-photon states has highlighted the importance of quantifying precisely what information can and cannot be inferred from features in a Hong-Ou-Mandel interference trace. Here we examine Hong-Ou-Mandel interference with regard to a particular class of states, so-called quantum frequency combs, and place special emphasis on the role spectral phase plays in these measurements. We find that this form of two-photon interferometry is insensitive to the relative phase between different comb line pairs. This is true even when different comb line pairs are mutually coherent at the input of a Hong-Ou-Mandel interferometer and the fringe patterns display sharp temporal features. Consequently, Hong-Ou-Mandel interference cannot speak to the presence of high-dimensional frequency-bin entanglement in two-photon quantum frequency combs.

Investigation of third-order dispersion of long-range surface-plasmon-polariton waveguides using a Hong-Ou-Mandel interferometer.

High-order dispersion of long-range surface-plasmon-polariton waveguides (LR-SPP-WGs) have been investigated using a two-photon interferometer. Since linear and even-ordered dispersions in two-photon interferometry are cancelled out by a nonlocal quantum correlation, odd-ordered dispersions of millimeter-long LR-SPP-WGs are revealed. Even under the highly dispersive condition, the indistinguishability between two photons emerged from LR-SPP-WGs was well preserved. In addition, we demonstrated a strong polarization-selection by the LR-SPP-WGs that leads to the polarization-stable and high-fidelity quantum interference.

Multistart spiral electron vortices in ionization by circularly polarized UV pulses

Multistart spiral vortex patterns are predicted for the electron momentum distributions in the polarization plane following ionization of the helium atom by two time-delayed circularly polarized ultrashort laser pulses. For two ultraviolet (UV) pulses having the same frequency (such that two photons are required for ionization), single-color two-photon interferometry with corotating or counter-rotating time-delayed pulses is found to lead respectively to zero-start or four-start spiral vortex patterns in the ionized electron momentum distributions in the polarization plane. In contrast, two-color one-photon plus two-photon interferometry with time-delayed corotating or counter-rotating UV pulses is found to lead respectively to one-start or three-start spiral vortex patterns. These predicted multistart electron vortex patterns are found to be sensitive to the carrier frequencies, handedness, time delay, and relative phase of the two pulses. Our numerical predictions are obtained by solving the six-dimensional two-electron time-dependent Schr\odinger equation (TDSE). They are explained analytically using perturbation theory (PT). Comparison of our TDSE and PT results for single-color two-photon processes probes the role played by the time-delay-dependent ionization cross channels in which one photon is absorbed from each pulse. Control of these cross channels by means of the parameters of the fields and the ionized electron detection geometries is discussed.

Entanglement measurement of a coupled silicon microring photon pair source.

Using two-photon (Franson) interferometry, we measure the entanglement of photon pairs generated from an optically-pumped silicon photonic device consisting of a few coupled microring resonators. The pair-source chip operates at room temperature, and the InGaAs single-photon avalanche detectors (SPADs) are thermo-electrically cooled to 234K. Such a device can be integrated with other components for practical entangled photon-pair generation at telecommunications wavelengths.

Generalized quantum interference of correlated photon pairs.

Superposition and indistinguishablility between probability amplitudes have played an essential role in observing quantum interference effects of correlated photons. The Hong-Ou-Mandel interference and interferences of the path-entangled photon number state are of special interest in the field of quantum information technologies. However, a fully generalized two-photon quantum interferometric scheme accounting for the Hong-Ou-Mandel scheme and path-entangled photon number states has not yet been proposed. Here we report the experimental demonstrations of the generalized two-photon interferometry with both the interferometric properties of the Hong-Ou-Mandel effect and the fully unfolded version of the path-entangled photon number state using photon-pair sources, which are independently generated by spontaneous parametric down-conversion. Our experimental scheme explains two-photon interference fringes revealing single- and two-photon coherence properties in a single interferometer setup. Using the proposed interferometric measurement, it is possible to directly estimate the joint spectral intensity of a photon pair source.

Time-reversed two-photon interferometry for phase superresolution

We observed two-photon phase super-resolution in an unbalanced Michelson interferometer with classical Gaussian laser pulses. Our work is a time-reversed version of a two-photon interference experiment using an unbalanced Michelson interferometer. A measured interferogram exhibits two-photon phase super-resolution with a high visibility of 97.9% \pm 0.4%. Its coherence length is about 22 times longer than that of the input laser pulses. It is a classical analogue to the large difference between the one- and two-photon coherence lengths of entangled photon pairs.

Two-photon interferometry and quantum state collapse

The quantum measurement problem still finds no consensus. Nonlocal interferometry provides an unprecedented experimental probe by entangling two photons in the ``measurement state'' (MS). The experiments show that each photon measures the other; the resulting entanglement decoheres both photons; decoherence collapses both photons to unpredictable but definite outcomes; and the two-photon MS continues evolving coherently. Thus, when a two-part system is in the MS, the outcomes actually observed at both subsystems are definite. Although standard quantum physics postulates definite outcomes, two-photon interferometry verifies them to be not only consistent with, but also actually a prediction of, the other principles. Nonlocality is the key to understanding this. As a consequence of nonlocality, the states we actually observe are the local states. These actually observed local states collapse, whereas the global MS, which can be ``observed'' only after the fact by collecting coincidence data from both subsystems, continues its unitary evolution. This conclusion implies a refined understanding of the eigenstate principle: Following a measurement, the actually observed local state instantly jumps into the observed eigenstate. We also discuss and rebut objections to this.

Two-photon-counting interferometry

Two-photon-counting interferometry has been realized by measuring the electrical current due to two-photon absorption in the space-charge layer of a semiconductor detector located at the output port of an interferometer. We apply this technique to study the correlation properties of twin beams issued from parametric fluorescence. We describe in detail how the different second-order correlation functions (interbeam, intrabeam) can be extracted at the femtosecond time scale from raw data. The values of these correlation functions determined by our experiments are in excellent agreement with theory. More precisely, extrabunching in twin beams is unambiguously demonstrated and theoretically described using two models: a comprehensive multimode quantum optics model and a simpler classical stochastic approach. Given the high brightness of our twin-beam source, both theories yield similar results. Finally, convenient analytical expressions of the correlation functions were derived from both theories, expressions in which we have been able to relate specific terms to accidental and exact coincidences between photons. Two-photon interferometry thus determines to which extent twin photons are twin. This technique should become a useful tool for future quantum optics developments.

Attosecond Two-Photon Interferometry for Doubly Excited States of Helium

We show that the correlation dynamics in coherently excited doubly excited resonances of helium can be followed in real time by two-photon interferometry. This approach promises to map the evolution of the two-electron wave packet onto experimentally easily accessible noncoincident single-electron spectra. We analyze the interferometric signal in terms of a semianalytical model which is validated by a numerical solution of the time-dependent two-electron Schrödinger equation in its full dimensionality.

Role of pump coherence in two-photon interferometry

We use a parametric down-conversion source pumped by a short coherence-length continuous-wave (CW) diode laser to perform two-photon interferometry in an intermediate regime between the more familiar Franson-type experiments with a long coherence-length pump laser, and the short pulsed pump "time-bin" experiments pioneered by Gisin's group. The use of a time-bin-like Mach-Zehnder interferometer in the CW pumping beam induces coherence between certain two-photon amplitudes, while the CW nature of the experiment prevents the elimination of remaining incoherent ones. The experimental results highlight the role of pump coherence in two-photon interferometry.

Nonlocal Pancharatnam phase in two-photon interferometry

We propose a polarized intensity interferometry experiment, which measures the nonlocal Pancharatnam phase acquired by a pair of Hanbury-Brown--Twiss photons. The setup involves two polarized thermal sources illuminating two polarized detectors. Varying the relative polarization angle of the detectors introduces a two-photon geometric phase. Local measurements at either detector do not reveal the effects of the phase, which is an optical analog of the multiparticle Aharonov-Bohm effect. The geometric phase sheds light on the three-slit experiment and suggests ways of tuning entanglement.

Nonclassical nature of dispersion cancellation and nonlocal interferometry

Several recent papers have shown that some forms of dispersion cancellation have classical analogs and that some aspects of nonlocal two-photon interferometry are consistent with local realistic models. It is noted here that the classical analogs only apply to local dispersion cancellation experiments [A.M. Steinberg et al., Phys. Rev. Lett. 68, 2421 (1992)] and that nonlocal dispersion cancellation [J.D. Franson, Phys. Rev. A 45, 3126 (1992)] is inconsistent with any classical field theory and has no classical analog. The local models that have been suggested for two-photon interferometry are shown to be local but not realistic if the spatial extent of the interferometers is taken into account. It is the inability of classical models to describe all of the relevant aspects of these experiments that distinguishes between quantum and classical physics, which is also the case in Bell's inequality.

Lepton interferometry in relativistic heavy ion collisions: A case study

We propose intensity interferometry with identical lepton pairs as an efficient tool for the estimation of the source size of the expanding hot zone produced in relativistic heavy ion collisions (RHIC). This can act as a complementary method to two-photon interferometry. The correlation function of two electrons with the same helicity has been evaluated for RHIC energies. The thermal shift of the $\ensuremath{\rho}$ meson mass has negligible effects on the Hanbury Brown--Twiss radii.

Quantum entanglement with acousto-optic modulators: Two-photon beats and Bell experiments with moving beam splitters

We present an experiment testing quantum correlations with frequency shifted photons. We test Bell inequality with two-photon interferometry where we replace the beam splitters with acousto-optic modulators, which are equivalent to moving beam splitters. We measure the two-photon beats induced by the frequency shifts, and we propose a cryptographic scheme in relation. Finally, setting the experiment in a relativistic configuration, we demonstrate that the quantum correlations are not only independent of the distance but also of the time ordering between the two single-photon measurements.

Off-diagonal geometric phase for mixed states.

We extend the off-diagonal geometric phase [Phys. Rev. Lett. 85, 3067 (2000)]] to mixed quantal states. The nodal structure of this phase in the qubit (two-level) case is compared with that of the diagonal mixed state geometric phase [Phys. Rev. Lett. 85, 2845 (2000)]]. Extension to higher dimensional Hilbert spaces is delineated. A physical scenario for the off-diagonal mixed state geometric phase in polarization-entangled two-photon interferometry is proposed.

Two-photon interferometry for high-resolution imaging

This paper discusses the advantages of using non-classical states of light for two aspects of optical imaging: the creation of microscopic images on photosensitive substrates, which constitutes the foundation for optical lithography, and the imaging of microscopic objects. In both cases, the classical resolution limit given by the Rayleigh criterion is approximately half of the optical wavelength. It has been shown, however, that by using multi-photon quantum states of the light field, and a multi-photon sensitive material or detector, this limit can be surpassed. A rigorous quantum mechanical treatment of this problem is given, some particularly widespread misconceptions are addressed, and turning quantum imaging into a practical technology is discussed.