In Transit-Oriented Development (TOD), the close integration of residential structures with community activities and traffic heightens residents' exposure to traffic-related pollutants. Despite traffic being a primary source of particulate matter (PM), the compact design of TODs, together with the impact of urban heat island (UHI), increases the likelihood of trapping emitted PM from traffic, leading to heightened exposure of TOD residents to PM. Although PM originates from two distinct sources in road traffic, exhaust and non-exhaust emissions (NEE), current legislation addressing traffic-related PM from non-exhaust emissions sources remains limited. This paper focuses on two TOD typologies in Manchester City—Manchester Piccadilly and East Didsbury—to understand the roles of TOD traffic as a PM generator and TOD place design as a PM container and trapper. The investigation aims to establish correlations between street design canyon ratios, vehicular Speed, and PM10/PM2.5, providing design guidance and effective traffic management strategies to control PM emissions within TODs. Through mapping the canyon ratio and utilising the Breezometer API for PM monitoring, the paper revealed elevated PM levels in both TOD areas, exceeding World Health Organization (WHO) recommendations, particularly for PM2.5. Correlation analysis between canyon configuration and PM2.5/PM10 highlighted the importance of considering building heights and avoiding the creation of deep canyons in TOD design to minimise the limited dispersion of PM. Leveraging UK road statistics and the PTV Group API for vehicle speed calculations, the paper studied the average speeds on the TOD roads concerning PM. Contrary to conventional assumption, the correlation analyses have revealed a noteworthy association shift between vehicular speed and PM concentrations. A positive correlation existed between speed increase and PM increases on arterial roads. However, a negative correlation emerged on main, collector, and local streets, indicating that PM levels rise for both PM10 and PM2.5 as Speed decreases. These findings challenge the traditional assumption that higher Speed leads to increased emissions, highlighting the potential impact of NEE on PM concentrations. This paper calls for thorough design considerations and traffic management strategies in TOD, especially in dense areas, considering building height, optimising traffic flow, and enhancing compromised air quality associated with vehicular emissions.