Traditional piezoelectric energy harvesters cannot adapt to environmental energy with low frequency, wideband, and randomness because of the narrow working bandwidth. The introduction of magnetic coupling can improve the narrow-band characteristics of piezoelectric energy harvesting structures. To explore more efficient broadband methods, this paper designs a piezoelectric and electromagnetic hybrid energy harvester (PEEH) based on two-stage magnetic coupling to realize the expansion of piezoelectric energy harvesting bandwidth. In this paper, the magnetic pole alternating frequency is changed and the output of the structure is tested, and the operating frequency bands under different alternating frequencies are compared according to the test results. It can be seen from the experimental results that the output performance of the structure is obviously improved by increasing the AC frequency of the magnetic pole while reducing the optimal frequency point of the structure. When the number of magnets in the rotor magnet array is 6, increasing the pole alternating frequency can effectively improve the output performance of the electromagnetic unit when the rotor speed is low, and can also increase the maximum output voltage and energy harvest bandwidth of the piezoelectric unit by 189% and 150%, respectively. Therefore, by increasing the alternating frequency of magnetic poles, the output voltage of the structure can be improved, and the bandwidth of the structure can be broadened.