Top Of Planetary Boundary Layer Research Articles

High organic aerosol in the low layer over a rural site in the North China Plain (NCP): Observations based on large tethered balloon

High mass concentration of organic aerosol (OA) and its fraction in PM2.5 (particle matter with radius <2.5 μm) were observed in the low layer over a rural site of the North China Plain (NCP) in winter 2018. The mass fraction of OA in PM2.5 was 65.5 % at ground level (5 m above ground), and decreased to 37.1 % in layer of 200–1000 m. In addition, there was a sharp decrease of OA at around the top of planetary boundary layer (PBL), which was distinctly different from the vertical distributions of secondary inorganic aerosols (SIA, e.g., nitrate (NO3−), ammonium (NH4+), and sulfate (SO42−)). The altitude with sharp decrease of OA was very low in the morning and evening, e.g., the sharp decrease of OA occurred at a height <50 m at nighttime on Dec. 19, while was elevated in the noon with the PBL development. Furthermore, OA at ground level exhibited a distinct diurnal variation with a night-to-day ratio of 2.3, which was much larger than those of SIA and inactive CO. All the above results indicated the extremely high OA concentration at the rural site was mainly attributed to direct emission from local sources, such as the combustion of coal and biomass for heating. The extremely high OA could be expected in vest rural areas of the NCP in winter because the farmer activities are very similar to the investigated rural site, underscoring the urgency to mitigate OA emission in rural area for improving the local as well as the regional air quality.

Variable Rainfall over Steady SST: The Effect of the Free Troposphere on Surface Pressure in the East Pacific

Abstract Surface winds and precipitation over the tropical oceans are related to sea surface temperature (SST) through multiple mechanisms. Greater SST is associated with greater conditional instability, which in turn is more conducive to deep convection. The associated mass and flow responses can extend to the surface, via associated pressure gradients imprinted on the top of the planetary boundary layer (PBL). SST also influences surface pressure and wind directly through its control over PBL temperature, as explained by Lindzen and Nigam. The authors examine the relative magnitudes of these two influences over the eastern tropical Pacific on subseasonal precipitation variability during northern summer, when and where SST gradients are largest and the direct influence via PBL temperature is expected to be strongest. Geopotential at 1000 hPa is partitioned into two components: the geopotential at the PBL top (the PBL top is chosen to be 850 hPa, supported by an analysis of the vertical structure of geopotential and temperature) and the PBL thickness. These fields are composited on quintiles of daily ITCZ precipitation both with and without a high-pass filter that isolates subseasonal time scales. The PBL thickness varies little between the highest and lowest precipitation quintiles, while the PBL top geopotential varies much more. This supports a view in which the direct contribution of SST to the surface pressure and flow fields, including the associated PBL convergence over sharp SST maxima, can be viewed as a steady forcing on the rest of the column, while free-tropospheric transients contribute most of the variability associated with precipitation on subseasonal time scales.

Structure and variations of global planetary boundary layer top from 2008-2022 multiple GNSS RO observations

The structural changes at the planetary boundary layer (PBL) top are very complex and closely related to climate and environmental changes. With the development of Global Navigation Satellite System Radio Occultation (GNSS RO), it provides a good opportunity to estimate and study PBL variations. In this paper, long-term variations and structures of planetary boundary layer height (PBLH) from 2008 to 2022 are investigated by the Wavelet Covariance Transform (WCT) method based on refractivity profiles from Constellation Observing System for Meteorology, Ionosphere, and Climate (COSMIC) and Korea Multi-purpose Satellite-5 (KOMPSAT-5). Furthermore, the temperature and pressure of PBL top are detected using the temperature and pressure profiles from COSMIC and KOMPSAT-5 occultation data. The results demonstrate the latitudinal distribution of the PBL top height, temperature, and pressure, with the more apparent temperature's latitudinal characteristics. The pressure is more strongly correlated with PBL height than temperature. The PBL height in most land and oceans is high in summer and low in winter, and the PBL pressure is low in summer and high in winter, according to seasonal variation characteristics. The global PBL temperature is high in summer and low in winter, which is more obvious in high latitude region. A positive correlation between latitude and the magnitude of seasonal variation in PBL temperature is observed worldwide. Seasonal variation is less pronounced in the Southern Hemisphere (SH) than in the Northern Hemisphere (NH) due to sea-land differences. The annual average value of the global PBL height, temperature, and pressure do not change significantly over the long term, and also there is no a discernible upward or downward trend.

Incorporating the Effect of Large‐Scale Vertical Motion on Convection Through Convective Mass Flux Adjustment in E3SMv2

AbstractRecent observational studies suggest that the large‐scale dynamical forcing (vertical motion) plays important roles in deep convection development. In this study we propose a convective mass flux adjustment (MAdj) approach to represent the dynamical effects of large‐scale vertical motion on convection in the Department of Energy's Energy Exascale Earth System Model version 2 (E3SMv2). With MAdj, convection is enhanced (suppressed) when there is large‐scale ascending (descending) motion at the planetary boundary layer top. The coupling of convection with large‐scale circulation significantly improves the simulation of climate variability in E3SMv2 across multiple scales from the diurnal cycle, convectively coupled equatorial waves, to the Madden‐Julian Oscillation (MJO). The standard E3SMv2 tends to simulate overly weak diurnal amplitude of precipitation and overly weak variance of convectively coupled equatorial Kelvin and westward inertio‐gravity (WIG) waves. It also fails to simulate the essential characteristics of the MJO: continuous eastward propagation. With MAdj, the amplitude of diurnal cycle of precipitation is systematically increased and its probability density distribution is much closer to observations. The MAdj can also simulate more realistic eastward propagation of the MJO and much stronger convectively coupled Kelvin and WIG waves. Moreover, the MAdj approach slightly improves the climatology simulations in precipitation, cloud, radiation, circulation, temperature, and moisture fields, with overall root‐mean‐square error (RMSE) of major climatological fields reduced by about 2%. The MAdj approach suppresses excessive grid‐scale precipitation, reducing precipitation wet biases over South China Sea, Philippine Sea, Himalayas, and South Pacific Convergence Zone in western Pacific in summer.

Dust-planetary boundary layer interactions amplified by entrainment and advections

Mineral dust contributes to more than half of the global aerosol loading. However, the radiative impacts of dust aerosols on planetary boundary layer (PBL) structure have not been explored sufficiently. During a typical dust storm event over Tarim Basin, dust aerosols exhibit a well-mixed distribution during the daytime in spite of a shallow layer of dust particles accumulated at higher altitudes. By contrast, nocturnal dust plumes are located near the surface due to stable stratification. We demonstrate that these differentiated vertical distributions determine the spatial heterogeneity of dust loading, radiative fluxes and PBL height variations. Dust aerosols cause daytime PBL suppression and nighttime PBL promotion through modulating surface and atmospheric radiative budgets. Specifically, dust-induced cooling effect within PBL directly inhibits the daytime PBL development. PBL suppression effect is then amplified by entrainment processes resulting in excessively low PBL height, especially for dust particles below but near the PBL top. Dust plumes weaken updrafts from PBL and downdrafts of the free atmosphere, which further reduce the entrainment mixing through attenuating horizontal and vertical advection, and eventually amplify PBL suppression. At night, near-surface dust aerosols stimulate a warm and unstable lower atmosphere, generate warm advection heating and promote the PBL development. Our study highlights the importance of specifying entrainment parameters and nighttime advection activities in quantifying the dust-PBL interactions.

COSMIC-2 RO Profile Ending at PBL Top with Strong Vertical Gradient of Refractivity

The Formosa Satellite-7/Constellation Observing System for Meteorology, Ionosphere, and Climate-2 (Satellite-7/COSMIC-2), which was successfully launched on 25 June 2019, provides dense radio occultation (RO) observations over the tropics and subtropics. This study examines the RO-observed lowest altitude and its possible relationship to refractivity gradients and planetary boundary layer (PBL) heights. COSMIC-2 RO data over the Southeast Pacific region (SEP) and the South-Central Pacific (SCP) from August 2020 are employed to determine their RO-observed lowest altitudes, and the European Centre for Medium-Range Weather Forecasts (ECMWF) ERA5 reanalysis data are used to obtain the gradients of refractivity. Results show that there are no ray perigees below the PBL top when the vertical gradient of N−N(r) is strong (&lt;−65 N-unit km−1), where N(r) represents the vertical profile of the spherically symmetric refractivity. Significantly strong local vertical gradients due to atmospheric ducting occur more frequently over the SEP than the SCP areas. For some cases, a strong local horizontal gradient of refractivity in the tangent direction of a ray near its perigee point can also limit the RO profile from going further below even when the vertical gradient of N−N(r) is relatively weak. Fortunately, only about 0.6% COSMIC-2 RO profiles are unaffected by the above factors but cannot observe below 2-km altitude.

Impact of lidar data assimilation on planetary boundary layer wind and PM2.5 prediction in Taiwan

Accurate simulations of planetary boundary layer (PBL) processes in numerical weather models are vital for air quality predictions. Advanced remote sensing techniques, such as lidar detection and ranging (lidar), can provide aerosol information with high temporal and vertical resolutions in the PBL. In this study, a lidar data assimilation system was developed based on the Weather Research and Forecasting-Local Ensemble Transform Kalman Filter (WRF-LETKF) framework coupled with the Community Multiscale Air Quality (CMAQ) model. The objective was to investigate the impact of lidar data assimilation on PBL prediction and the subsequent influence on PM2.5 prediction for a high-air-pollution event.The fine particulate matter (PM2.5) profiles retrieved from two micropulse lidar observations in northern and central Taiwan were assimilated in the WRF-LETKF system. Three numerical experiments, BASE (with a nudging strategy), CTRL (with an ensemble framework), and LDA (with assimilation of lidar-retrieved PM2.5 profiles), were conducted for a high-air-pollution episode. The BASE simulation overestimates the wind speed, which also leads to PM2.5 underestimation. The CTRL and LDA simulations are able to improve the wind fields and enhance the PM2.5 accumulation. With a strong error correlation between the lidar-retrieved PM2.5 concentration and the wind fields, the LDA simulation effectively corrects the wind flow from the surface to the PBL top, which further adjusts the PM2.5 transport processes and leads to results that agree well with observations.

Observation system simulation experiments (OSSEs) for assimilation of the planetary boundary‐layer height (PBLH) using the EnSRF technique

AbstractThe planetary boundary‐layer height (PBLH) is a key parameter that is very important in numerical weather and air quality predictions. The current LiDAR networks make it possible to provide potential PBLH observations, and assimilating the parameter will be helpful to improve the forecast of variables within the planetary boundary layer (PBL). This study first carried out idealized experiments on PBLH assimilation through observation system simulation experiments (OSSEs). The ensemble square root filter (EnSRF) is applied to assimilate the simulated PBLH based on the Weather Research and Forecast (WRF) model. This study mainly focused on two issues: which variables can be effectively improved by assimilating the PBLH, and whether there are differences in the assimilation effects above and within the PBL in the vertical direction. The results show that during the daytime within the PBL, PBLH assimilation could effectively improve the simulation and forecasting of model variables, including perturbation potential temperature (pt), water vapour mixing ratio (qv) and perturbation geopotential (ph); meanwhile, PBLH assimilation could strengthen turbulence mixing and result in a warmer and drier PBL. While the vertical and horizontal wind speeds (w, u and v) cannot be effectively updated by assimilating the PBLH, they could be indirectly improved by model dynamical adjustment when pt, qv and ph are improved. Above the PBL top, most of the above six variables cannot be effectively improved by assimilating the daytime PBLH. In contrast, at night, only u and v within the PBL could be directly updated by the low nocturnal PBLH. In this study, the simplest and most idealized schemes are selected based on idealized experiments; nevertheless, the results lay a foundation for later vertical and horizontal localization research and for the study of LiDAR‐retrieved PBLH assimilation in the future, which is the ultimate goal of this series of works.

The effect of BC on aerosol–boundary layer feedback: potential implications for urban pollution episodes

Abstract. Beijing suffers from poor air quality, particularly during wintertime haze episodes when concentrations of PM2.5 (particulate matter with a diameter &lt; 2.5 µm) can peak at &gt; 400 µg m−3. Black carbon (BC), an aerosol which strongly absorbs solar radiation, can make up to 10 % of PM2.5 in Beijing. BC is of interest due to its climatic and health impacts. BC has also been found to impact planetary boundary layer (PBL) meteorology. Through interacting with radiation and altering the thermal profile of the lower atmosphere, BC can either suppress or enhance PBL development depending on the properties and altitude of the BC layer. Previous research assessing the impact of BC on PBL meteorology has been investigated through the use of regional models, which are limited both by resolution and the chosen boundary layer schemes. In this work, we apply a high-resolution model (UCLALES-SALSA) that couples an aerosol and radiative transfer model with large-eddy simulation (LES) to quantify the impact of BC at different altitudes on PBL dynamics using conditions from a specific haze episode which occurred from 1–4 December 2016 in Beijing. Results presented in this paper quantify the heating rate of BC at various altitudes to be between 0.01 and 0.016 K/h per µg/m3 of BC, increasing with altitude but decreasing around PBL top. Through utilising a high-resolution model which explicitly calculates turbulent dynamics, this paper showcases the impact of BC on PBL dynamics both within and above the PBL. These results show that BC within the PBL increases maximum PBL height by 0.4 % but that the same loading of BC above the PBL can suppress PBL height by 6.5 %. Furthermore, when BC is present throughout the column, the impact of BC suppressing PBL development is further maximised, with BC causing a 17 % decrease in maximum PBL height compared to only scattering aerosols. Assessing the impact of these opposite effects, in this paper, we present a mechanism through which BC may play a prominent role in the intensity and longevity of Beijing's pollution episodes.

Reduced volatility of aerosols from surface emissions to the top of the planetary boundary layer

Abstract. Aerosols from surface emission can be transported upwards through convective mixing in the planetary boundary layer (PBL), which subsequently interact with clouds, serving as important sources to nucleate droplets or ice particles. However, the evolution of aerosol composition during this vertical transport has yet to be explicitly understood. In this study, simultaneous measurements of detailed aerosol compositions were conducted at two sites, namely urban Beijing (50 m above sea level – a.s.l.) and Haituo mountain (1344 m a.s.l.) during wintertime, representing the anthropogenically polluted surface environment and the top of the PBL, respectively. The pollutants from surface emissions were observed to reach the mountain site on daily basis through daytime PBL convective mixing. From the surface to the top of PBL, we found efficient transport or formation of lower-volatility species (black carbon, sulfate, and low-volatile organic aerosol, OA); however, a notable reduction in semivolatile substances, such as the fractions of nitrate and semivolatile OA reduced by 74 % and 76 %, respectively, during the upward transport. This implies that the mass loss of these semivolatile species was driven by the evaporation process, which repartitioned the condensed semivolatile substances to the gas phase when aerosols were transported and exposed to a cleaner environment. In combination with the oxidation processes, these led to an enhanced oxidation state of OA at the top of the PBL compared to surface environment, with an increase of oxygen to carbon atomic ratio by 0.2. Such a reduction in aerosol volatility during vertical transport may be important in modifying its viscosity, nucleation activity, and atmospheric lifetime.

Spatiotemporal changes in aerosol properties by hygroscopic growth and impacts on radiative forcing and heating rates during DISCOVER-AQ 2011

Abstract. This work focuses on the characterization of vertically resolved aerosol hygroscopicity properties and their direct radiative effects through a unique combination of ground-based and airborne remote sensing measurements during the Column and Vertically Resolved Observations Relevant to Air Quality (DISCOVER-AQ) 2011 field campaign in the Baltimore–Washington DC metropolitan area. To that end, we combined aerosol measurements from a multiwavelength Raman lidar located at NASA Goddard Space Flight Center and the airborne NASA Langley High Spectral Resolution Lidar-1 (HSRL-1) lidar system. In situ measurements aboard the P-3B airplane and ground-based Aerosol Robotic Network – Distributed Regional Aerosol Gridded Observational Network (AERONET-DRAGON) served to validate and complement quantifications of aerosol hygroscopicity from lidar measurements and also to extend the study both temporally and spatially. The focus here is on 22 and 29 July 2011, which were very humid days and characterized by a stable atmosphere and increasing relative humidity with height in the planetary boundary layer (PBL). Combined lidar and radiosonde (temperature and water vapor mixing ratio) measurements allowed the retrieval of the Hänel hygroscopic growth factor which agreed with that obtained from airborne in situ measurements and also explained the significant increase of extinction and backscattering with height. Airborne measurements also confirmed aerosol hygroscopicity throughout the entire day in the PBL and identified sulfates and water-soluble organic carbon as the main species of aerosol particles. The combined Raman and HSRL-1 measurements permitted the inversion for aerosol microphysical properties revealing an increase of particle radius with altitude consistent with hygroscopic growth. Aerosol hygroscopicity pattern served as a possible explanation of aerosol optical depth increases during the day, particularly for fine-mode particles. Lidar measurements were used as input to the libRadtran radiative transfer code to obtain vertically resolved aerosol radiative effects and heating rates under dry and humid conditions, and the results reveal that aerosol hygroscopicity is responsible for larger cooling effects in the shortwave range (7–10 W m−2 depending on aerosol load) near the ground, while heating rates produced a warming of 0.12 K d−1 near the top of PBL where aerosol hygroscopic growth was highest.

Understanding the Roles of Convective Trigger Functions in the Diurnal Cycle of Precipitation in the NCAR CAM5

AbstractThe wrong diurnal cycle of precipitation is a common weakness of current global climate models (GCMs). To improve the simulation of the diurnal cycle of precipitation and understand what physical processes control it, we test a convective trigger function described in Xie et al. with additional optimizations in the NCAR Community Atmosphere Model version 5 (CAM5). The revised trigger function consists of three modifications: 1) replacing the convective available potential energy (CAPE) trigger with a dynamic CAPE (dCAPE) trigger, 2) allowing convection to originate above the top of planetary boundary layer [i.e., the unrestricted air parcel launch level (ULL)], and 3) optimizing the entrainment rate and threshold value of the dynamic CAPE generation rate for convection onset based on observations. Results from 1° resolution simulations show that the revised trigger can alleviate the long-standing GCM problem of too early maximum precipitation during the day and missing the nocturnal precipitation peak that is observed in many regions, including the U.S. southern Great Plains (SGP). The revised trigger also improves the simulation of the propagation of precipitation systems downstream of the Rockies and the Amazon region. A further composite analysis over the SGP unravels the mechanisms through which the revised trigger affects convection. Additional sensitivity tests show that both the peak time and the amplitude of the diurnal cycle of precipitation are sensitive to the entrainment rate and dCAPE threshold values.

Optical and hygroscopic properties of black carbon influenced by particle microphysics at the top of the anthropogenically polluted boundary layer

Abstract. Aerosols at the top of the planetary boundary layer (PBL) could modify its atmospheric dynamics by redistributing the solar radiation and start to be activated to form low-level cloud at this layer. Black carbon (BC), as an aerosol component efficiently absorbing solar radiation, can introduce heating and positive radiative effects at this sensitive layer, especially in the polluted PBL over the continent. This study presents continuous measurements of detailed BC properties at a mountain site located at the top of the polluted PBL over the North China Plain, during seasons (3 and 4 weeks of data during winter and summer, respectively) with contrasting emission structure and meteorology. The pollution level was persistently influenced by local surface anthropogenic emission on a daily basis through daytime convective mixing, but the concentration was also enhanced or diluted depending on air mass direction, defined as a neutral, polluted and diluted PBL, respectively. Winter was observed to have a higher BC mass fraction (4 %–8 %) than summer (2 %–7 %). By resolving the detailed particle size-resolved mixing state of BC in optical and hygroscopic models, we found an enhanced BC mass absorption cross section (MACBC) for the polluted PBL (up to 13 m2 g−1 at λ = 550 nm), which was 5 % higher during summer than winter due to a smaller BC core size. The higher BC mass fraction in winter corresponded to a lower single-scattering albedo by 0.03–0.09 than summer, especially the lowest for the diluted winter PBL (0.86 ± 0.02). The water supersaturation (SS) required to activate half the number of BC decreased from 0.21 % ± 0.08 % to 0.1 % ± 0.03 % for the winter diluted and polluted PBL and from 0.22 % ± 0.06 % to 0.17 % ± 0.05 % for summer. Notably, at the top of the anthropogenically polluted PBL in both seasons, the enlarged BC with enhanced absorption capacity could also be efficiently droplet activated; e.g. winter (summer) BC with an MAC of 9.84 ± 1.2 (10.7 ± 1) m2 g−1 could be half activated at SS = 0.13 % ± 0.06 % (0.18 % ± 0.05 %). This BC at the top of the PBL can more directly interact with the free troposphere and be transported to a wider region, exerting important direct and indirect radiative impacts.

Relationship between summertime concurring PM2.5 and O3 pollution and boundary layer height differs between Beijing and Shanghai, China.

The rapid development in the economy during past decades has caused serious air pollution issues in China with high concentrations of PM2.5 and O3, particularly in the densely populous cities. To integrate PM2.5 and O3 controls, it is necessary to understand the impacts of meteorology on both pollutants. Thereby, the complex linkages between planetary boundary layer (PBL), synoptic forcing, regional transport, and heavy pollution in Beijing and Shanghai during summer were investigated using long-term measurements, simulations, and reanalysis. Influenced by the unfavorable meteorological conditions, PM2.5 pollution and O3 pollution often simultaneously occurred. In Beijing, the heavy concurring pollutions usually happened on the days with shallow afternoon PBL and southerly/southwesterly prevailing winds. Within the PBL, the pollutants emitted from the southern plains can be transported to Beijing and accumulated on the windward side of the mountains. At the top of PBL, the synoptic southerly warm advections can strengthen the elevated thermal inversion layer and suppress the development of PBL, leading to worse pollution. Contrarily, the heavy pollutions in Shanghai usually occurred on the days with deep afternoon PBL and southwesterly warm advections within the PBL. Although the warm advections were more favorable to the PBL development than the movements of cool marine air mass, the input of pollutants from the southwest can overweigh this advantage, resulting in poor air quality in Shanghai. The occurrence of heavy pollution or clean condition in Shanghai was primarily determined by the synoptic forcing rather than the local PBL structure. This comparative study indicates that the relationship between PBL height and pollution level is changeable and complicated, which needs to be elucidated from the synoptic perspective.

Black Carbon Emission and Wet Scavenging From Surface to the Top of Boundary Layer Over Beijing Region

AbstractThe heating impacts caused by black carbon (BC) may modify the atmospheric dynamics of planetary boundary layer (PBL), essentially determined by its vertical distribution. In this study we performed simultaneous measurements of detailed BC properties at both surface (50 m) and mountain sites (1,344 m) over Beijing region. The latter represents the top of PBL and was influenced by surface anthropogenic emissions, particularly around midday when PBL was developed, allowing continuous investigations on the evolution of BC during vertical transport in the PBL. Experiments in cold and warm seasons were performed to reflect seasonal difference in emission and meteorology: Winter had additional emission of residential heating and dry air; summer had moist air with more precipitation. The net ratio of BC/CO relative to background (ΔBC/ΔCO) is used to indicate the emission signature and scavenging of BC. At surface, both seasons peaked at similar ΔBC/ΔCO, however showed contrast shifts between both sites. In winter, mountain showed slightly higher ΔBC/ΔCO than surface due to receiving sources from wider area, whereas in summer, a refractory black carbon (rBC) mass scavenging efficiency of 35–62% was derived from the significantly lowered ΔBC/ΔCO on mountain. This scavenging process could incorporate BC into the summer moist air or low‐level clouds on a daily basis, exerting potential indirect effects. The resultant BC after scavenging exhibited smaller core size and increased coatings, leading to higher absorption efficiency by 45%. These factors should improve the representation of boundary layer processing of BC in evaluating its direct and indirect radiative impacts over the anthropogenically influenced region.

Effect of Scale-Aware Nonlocal Planetary Boundary Layer Scheme on Lake-Effect Precipitation at Gray-Zone Resolutions

Abstract The effects of a nonlocal planetary boundary layer (PBL) scheme that considers scale dependency in the parameterized turbulent vertical transport are investigated for a case of wintertime lake-effect precipitation over Korea at gray-zone resolutions using a mesoscale model. An experiment using the scale-aware PBL scheme is compared with that using a conventional PBL scheme, which shows that the simulated precipitation amount at a resolution of less than 1 km is smaller with the scale-aware PBL scheme. The role of turbulent processes in simulating lake-effect precipitation is understood through interaction with microphysical processes. When the scale-aware PBL scheme is used, liquid water content is increased while ice water content is reduced. The higher cloud water content is because of enhanced condensation with stronger updrafts, attributed to the suppression of parameterized turbulent mixing. This results in higher rainwater content by enhancing autoconversion and accretion from cloud water to rainwater. The cloud ice content is reduced mainly because of the suppressed deposition and enhanced sublimation centered near the PBL top, and the snow content is reduced mainly because of the enhanced sublimation below and near the PBL top and suppressed growth of cloud ice to snow. The lower ice water content is mainly due to the drier PBL, attributed to the enhanced resolved (suppressed parameterized) turbulent moisture transport and enhanced condensation. The melting of a smaller amount of snow under dominant cold rain processes is responsible for the reduced surface precipitation with the scale-aware PBL scheme.

Sources of black carbon during severe haze events in the Beijing–Tianjin–Hebei region using the adjoint method

The Beijing-Tianjin-Hebei (BTH) region in China has been frequently suffering from severe haze events (observed daily mean surface fine particulate matter PM2.5 concentrations larger than 150 μg m−3) partially caused by certain types of large-scale synoptic patterns. Black carbon (BC), as an important PM2.5 component and a primarily emitted species, is a good tracer for investigating sources and formation mechanisms leading to severe haze pollutions. We apply GEOS-Chem model and its adjoint to quantify the source contributions to BC concentrations at the surface and at the top of the planetary boundary layer (PBL) during typical types of severe haze events for April 2013–2017 in BTH. Four types of severe haze events, mainly occurred in December–January-February (DJF, 62.3%) and in September–October-November (SON, 26.3%), are classified based on the associated synoptic weather patterns using principal component analysis. Model results reasonably capture the daily variations of BC measurements at three ground sites in BTH. The adjoint method attributes BC concentrations to emissions from different source sectors and from local versus regional transport at the model spatial and temporal resolutions. By source sectors, the adjoint method attributes the daily BC concentrations during typical severe haze events (in winter heating season) in Beijing largely to residential emissions (48.1–62.0%), followed by transportation (16.8–25.9%) and industry (19.1–29.5%) sectors. In terms of regionally aggregated source influences, local emissions in Beijing (59.6–79.5%) predominate the daily surface BC concentrations, while contributions of emissions from Beijing, Hebei, and outside BTH regions are comparable to the daily BC concentrations at the top of PBL (~200–400 m). Our adjoint analyses would provide a scientific support for joint regional and targeted control policies on effectively mitigating the particulate pollutions when the dominant synoptic weather patterns are predicted.

Effects of cool roofs on turbulent coherent structures and ozone air quality in Seoul

Abstract The cool-roof strategy is an effective way of mitigating severe urban heat islands, and its impacts on urban flow and air quality deserve in-depth investigations. This study examines the effects of cool roofs on turbulent coherent structures and ozone air quality in Seoul, South Korea using the Weather Research and Forecasting-Community Multiscale Air Quality (WRF-CMAQ) model with a 50 m horizontal grid spacing. Cool roofs decrease the daily average air temperature, planetary boundary layer (PBL) height, and wind speed in the urban area of Seoul by 0.80 °C, 230 m, and 0.17 m s−1, respectively. Due to the lowered air temperature by cool roofs, the sea breeze and convective structures weaken and eddies at the PBL top appear less frequently. Since high O3 concentration air flows into Seoul by the sea breeze, the weakened sea breeze decreases the daily average O3 concentration near the surface by 3.3 ppb. Air at lower level is transported upward across the PBL top by convective structures and eddies at the PBL top. The transported air at lower level has lower O3 concentration and higher concentrations of O3 precursors than air at upper level. Therefore, the weakened convective structures and less-frequent appearance of eddies at the PBL top by cool roofs weaken the upward transport of O3 precursors at lower level across the PBL top. As a result, the chemical production of O3 and O3 concentration slightly above the PBL top are decreased. An integrated process rate analysis shows that cool roofs weaken the effects of turbulent coherent structures on O3 concentration.

Supercooled liquid water cloud observed, analysed, and modelled at the top of the planetary boundary layer above Dome C, Antarctica

Abstract. A comprehensive analysis of the water budget over the Dome C (Concordia, Antarctica) station has been performed during the austral summer 2018–2019 as part of the Year of Polar Prediction (YOPP) international campaign. Thin (∼100 m deep) supercooled liquid water (SLW) clouds have been detected and analysed using remotely sensed observations at the station (tropospheric depolarization lidar, the H2O Antarctica Microwave Stratospheric and Tropospheric Radiometer (HAMSTRAD), net surface radiation from the Baseline Surface Radiation Network (BSRN)), radiosondes, and satellite observations (CALIOP, Cloud-Aerosol LIdar with Orthogonal Polarization/CALIPSO, Cloud Aerosol Lidar and Infrared Pathfinder Satellite Observations) combined with a specific configuration of the numerical weather prediction model: ARPEGE-SH (Action de Recherche Petite Echelle Grande Echelle – Southern Hemisphere). The analysis shows that SLW clouds were present from November to March, with the greatest frequency occurring in December and January when ∼50 % of the days in summer time exhibited SLW clouds for at least 1 h. Two case studies are used to illustrate this phenomenon. On 24 December 2018, the atmospheric planetary boundary layer (PBL) evolved following a typical diurnal variation, which is to say with a warm and dry mixing layer at local noon thicker than the cold and dry stable layer at local midnight. Our study showed that the SLW clouds were observed at Dome C within the entrainment and the capping inversion zones at the top of the PBL. ARPEGE-SH was not able to correctly estimate the ratio between liquid and solid water inside the clouds with the liquid water path (LWP) strongly underestimated by a factor of 1000 compared to observations. The lack of simulated SLW in the model impacted the net surface radiation that was 20–30 W m−2 higher in the BSRN observations than in the ARPEGE-SH calculations, mainly attributable to the BSRN longwave downward surface radiation being 50 W m−2 greater than that of ARPEGE-SH. The second case study took place on 20 December 2018, when a warm and wet episode impacted the PBL with no clear diurnal cycle of the PBL top. SLW cloud appearance within the entrainment and capping inversion zones coincided with the warm and wet event. The amount of liquid water measured by HAMSTRAD was ∼20 times greater in this perturbed PBL than in the typical PBL. Since ARPEGE-SH was not able to accurately reproduce these SLW clouds, the discrepancy between the observed and calculated net surface radiation was even greater than in the typical PBL case, reaching +50 W m−2, mainly attributable to the downwelling longwave surface radiation from BSRN being 100 W m−2 greater than that of ARPEGE-SH. The model was then run with a new partition function favouring liquid water for temperatures below −20 down to −40 ∘C. In this test mode, ARPEGE-SH has been able to generate SLW clouds with modelled LWP and net surface radiation consistent with observations during the typical case, whereas, during the perturbed case, the modelled LWP was 10 times less than the observations and the modelled net surface radiation remained lower than the observations by ∼50 W m−2. Accurately modelling the presence of SLW clouds appears crucial to correctly simulate the surface energy budget over the Antarctic Plateau.

On-flight intercomparison of three miniature aerosol absorption sensors using unmanned aerial systems (UASs)

Abstract. The present study investigates and compares the ground and in-flight performance of three miniaturized aerosol absorption sensors integrated on board small-sized Unmanned Aerial Systems (UASs). These sensors were evaluated during two contrasted field campaigns performed at an urban site, impacted mainly by local traffic and domestic wood burning sources (Athens, Greece), and at a remote regional background site, impacted by long-range transported sources including dust (Cyprus Atmospheric Observatory, Agia Marina Xyliatou, Cyprus). The miniaturized sensors were first intercompared at the ground-level against two commercially available instruments used as a reference. The measured signal of the miniaturized sensors was converted into the absorption coefficient and equivalent black carbon concentration (eBC). When applicable, signal saturation corrections were applied, following the suggestions of the manufacturers. The aerosol absorption sensors exhibited similar behavior against the reference instruments during the two campaigns, despite the diversity of the aerosol origin, chemical composition, sources, and concentration levels. The deviation from the reference during both campaigns concerning (eBC) mass was less than 8 %, while for the absorption coefficient it was at least 15 %. This indicates that those sensors that report black carbon mass are tuned and corrected to measure eBC more accurately than the absorption coefficient. The overall potential use of miniature aerosol absorption sensors on board small UASs is also illustrated. UAS-based absorption measurements were used to investigate the vertical distribution of eBC over Athens up to 1 km above sea level during January 2016, exceeding the top of the planetary boundary layer (PBL). Our results reveal a heterogeneous boundary layer concentration of absorbing aerosol within the PBL intensified in the early morning hours due to the concurrent peak traffic emissions at ground-level and the fast development of the boundary layer. After the full development of the PBL, homogenous concentrations are observed from 100 m a.g.l. to the PBL top.