Time-reversible Dynamics Research Articles

Time-reversible dynamics in a system of two coupled active rotators

We study two coupled active rotators with Kuramoto-type coupling and focus our attention to specific transitional regimes where the coupling is neither attractive nor repulsive. We show that certain such situations at the edge of synchronization can be characterized by the existence of a time-reversal symmetry of the system. We identify two different cases with such a time-reversal symmetry. The first case is characterized by a non-reciprocal attractive/repulsive coupling. The second case is a reciprocal coupling exactly at the edge between attraction and repulsion. We give a detailed description of possible different types of dynamics and bifurcations for both cases. In particular, we show how the time-reversible coupling can induce both oscillation death and oscillation birth to the active rotators. Moreover, we analyse the coexistence of conservative and dissipative regions in phase space, which is a typical feature of systems with a time-reversal symmetry. We show also, how perturbations breaking the time-reversal symmetry and destroying the conservative regions can lead to complicated types of dissipative dynamics such as the emergence of long-period cycles showing a bursting-like behaviour.

Additive eigenvectors as optimal reaction coordinates, conditioned trajectories, and time-reversible description of stochastic processes.

A fundamental way to analyze complex multidimensional stochastic dynamics is to describe it as diffusion on a free energy landscape-free energy as a function of reaction coordinates (RCs). For such a description to be quantitatively accurate, the RC should be chosen in an optimal way. The committor function is a primary example of an optimal RC for the description of equilibrium reaction dynamics between two states. Here, additive eigenvectors (addevs) are considered as optimal RCs to address the limitations of the committor. An addev master equation for a Markov chain is derived. A stationary solution of the equation describes a sub-ensemble of trajectories conditioned on having the same optimal RC for the forward and time-reversed dynamics in the sub-ensemble. A collection of such sub-ensembles of trajectories, called stochastic eigenmodes, can be used to describe/approximate the stochastic dynamics. A non-stationary solution describes the evolution of the probability distribution. However, in contrast to the standard master equation, it provides a time-reversible description of stochastic dynamics. It can be integrated forward and backward in time. The developed framework is illustrated on two model systems-unidirectional random walk and diffusion.

Quantum fluctuation theorem for dissipative processes

We present a general quantum fluctuation theorem for the entropy production of an open quantum system coupled to multiple environments, not necessarily at equilibrium. Such a general theorem, when restricted to the weak-coupling and Markovian regime, holds for both local and global master equations, corroborating the thermodynamic consistency of local quantum master equations. The theorem is genuinely quantum, as it can be expressed in terms of conservation of a Hermitian operator, describing the dynamics of the system state operator and of the entropy change in the baths. The integral fluctuation theorem follows from the properties of such an operator. Furthermore, it is also valid when the system is described by a time-dependent Hamiltonian. As such, the quantum Jarzynski equality is a particular case of the general result presented here. Moreover, our result can be extended to nonthermal baths, as long as microreversibility is preserved. We present some numerical examples to showcase the exact results previously obtained. We finally generalize the fluctuation theorem to the case where the interaction between the system and the bath is explicitly taken into account. We show that the fluctuation theorem amounts to a relation between time-reversed dynamics of the global density matrix and a two-time correlation function along the forward dynamics involving the baths' entropy alone.

Non-Markovian Feedback Control and Acausality: An Experimental Study

Causality is an important assumption underlying nonequilibrium generalizations of the second law of thermodynamics known as fluctuation relations. We here experimentally study the nonequilibrium statistical properties of the work and of the entropy production for an optically trapped, underdamped nanoparticle continuously subjected to a time-delayed feedback control. Whereas the non-Markovian feedback depends on the past position of the particle for a forward trajectory, it depends on its future position for a time-reversed path, and is therefore acausal. In the steady-state regime, we show that the corresponding fluctuation relations in the long-time limit exhibit a clear signature of this acausality, even though the time-reversed dynamics is not physically realizable.

Fokker–Planck equations with terminal condition and related McKean probabilistic representation

Usually Fokker–Planck type partial differential equations (PDEs) are well-posed if the initial condition is specified. In this paper, alternatively, we consider the inverse problem which consists in prescribing final data: in particular we give sufficient conditions for uniqueness. In the second part of the paper we provide a probabilistic representation of those PDEs in the form of a solution of a McKean type equation corresponding to the time-reversal dynamics of a diffusion process.

Nonlinear interferometry beyond classical limit enabled by cyclic dynamics

Time-reversed evolution has substantial implications in physics, including prominent applications in refocusing of classical waves or spins and fundamental researches such as quantum information scrambling. In quantum metrology, nonlinear interferometry based on time reversal protocols supports entanglement-enhanced measurements without requiring low-noise detection. Despite the broad interest in time reversal, it remains challenging to reverse the quantum dynamics of an interacting many-body system as is typically realized by an (effective) sign-flip of the system's Hamiltonian. Here, we present an approach that is broadly applicable to cyclic systems for implementing nonlinear interferometry without invoking time reversal. Inspired by the observation that the time-reversed dynamics drives a system back to its starting point, we propose to accomplish the same by slaving the system to travel along a 'closed-loop' instead of explicitly tracing back its antecedent path. Utilizing the quasi-periodic spin mixing dynamics in a three-mode $^{87}$Rb atom spinor condensate, we implement such a 'closed-loop' nonlinear interferometer and achieve a metrological gain of $3.87_{-0.95}^{+0.91}$ decibels over the classical limit for a total of 26500 atoms. Our approach unlocks the high potential of nonlinear interferometry by allowing the dynamics to penetrate into deep nonlinear regime, which gives rise to highly entangled non-Gaussian state. The idea of bypassing time reversal may open up new opportunities in the experimental investigation of researches that are typically studied by using time reversal protocols.

Continuous time reversal and equality in the thermodynamic uncertainty relation

We introduce a continuous time-reversal operation which connects the time-forward and time-reversed trajectories in the steady state of an irreversible Markovian dynamics via a continuous family of stochastic dynamics. This continuous time-reversal allows us to derive a tighter version of the thermodynamic uncertainty relation (TUR) involving observables evaluated relative to their local mean value. Moreover, the family of dynamics realizing the continuous time-reversal contains an equilibrium dynamics halfway between the time-forward and time-reversed dynamics. We show that this equilibrium dynamics, together with an appropriate choice of the observable, turns the inequality in the TUR into an equality. We demonstrate our findings for the example of a particle diffusing in a tilted periodic potential.

Stochastic dynamics, large deviation principle, and nonequilibrium thermodynamics.

By examining the deterministic limit of a general ε-dependent generator for Markovian dynamics, which includes the continuous Fokker-Planck equations and discrete chemical master equations as two special cases, the intrinsic connections among mesoscopic stochastic dynamics, deterministic ordinary differential equations or partial differential equations, large deviation rate functions, and macroscopic thermodynamic potentials are established. Our result not only solves the long-lasting question of the origin of the entropy function in classical irreversible thermodynamics, but also reveals an emergent feature that arises automatically during the deterministic limit, through its large deviation rate function, with both time-reversible dynamics equipped with a Hamiltonian function and time-irreversible dynamics equipped with an entropy function.

Time-reversal odd transport in bilayer graphene: Hall conductivity and Hall viscosity

We consider the time-reversal odd dynamics of the bilayer graphene at low energies in the quantum Hall regime. A generating functional for the effective action that captures the electromagnetic response to all orders in momentum and frequency is presented and evaluated to the third order in the space-time gradient $\mathcal O(\partial^3)$. In addition, we calculate the Hall viscosity and derive an explicit relationship with the $q^2$ coefficient of the Hall conductivity. It is reminiscent of the Hoyos--Son relation in the Galilean invariant systems, which can be recovered in the limit of large filling factor $N$.

Relating relative Rényi entropies and Wigner-Yanase-Dyson skew information to generalized multiple quantum coherences

Quantum coherence is a crucial resource for quantum information processing. By employing the language of coherence orders largely applied in NMR systems, quantum coherence has been currently addressed in terms of multiple quantum coherences (MQCs). Here we investigate the $\alpha$-MQCs, a novel class of multiple quantum coherences which is based on $\alpha$-relative purity, an information-theoretic quantifier analogous to quantum fidelity and closely related to R\'{e}nyi relative entropy of order $\alpha$. Our framework enables linking $\alpha$-MQCs to Wigner-Yanase-Dyson skew information (WYDSI), an asymmetry monotone finding applications in quantum thermodynamics and quantum metrology. Furthermore, we derive a family of bounds on $\alpha$-MQCs, particularly showing that $\alpha$-MQC define a lower bound to quantum Fisher information (QFI). We illustrate these ideas for quantum systems described by single-qubit states, two-qubit Bell-diagonal states, and a wide class of multiparticle mixed states. Finally, we investigate the time evolution of the $\alpha$-MQC spectrum and the overall signal of relative purity, by simulating the time reversal dynamics of a many-body all-to-all Ising Hamiltonian and comment on applications to physical platforms such as NMR systems, trapped ions, and ultracold atoms.

Recovery of Damaged Information and the Out-of-Time-Ordered Correlators

The evolution with a complex Hamiltonian generally leads to information scrambling. A time-reversed dynamics unwinds this scrambling and thus leads to the original information recovery. We show that if the scrambled information is, in addition, partially damaged by a local measurement, then such a damage can still be treated by application of the time-reversed protocol. This information recovery is described by the long-time saturation value of a certain out-of-time-ordered correlator of local variables. We also propose a simple test that distinguishes between quantum and reversible classical chaotic information scrambling.

Otherwise identical particles with differing, fixed speeds demix under time-reversible dynamics.

In recent years situations where elsewise identical particles demix when different degrees of freedom do not thermalize have become a research focus in nonequilibrium statistical mechanics. The majority of these models are formulated in the context of active particles, but the phenomenon also occurs for particles without driving. All the models studied so far share the property that they do not obey microscopic reversibility, and it may be thought that this is a necessary condition for such demixing to occur. We show here that such a demixing transition also occurs in a mixture of otherwise identical particles moving at two fixed but different speeds according to a time-reversible quasi-Newtonian dynamics. The mechanical instability underlying this behavior is generated by the lack of thermalization between the two subsystems, which is shared by all systems showing this behavior.

Metastable transitions in inertial Langevin systems: What can be different from the overdamped case?

Metastable transitions in Langevin dynamics can exhibit rich behaviours that are markedly different from its overdamped limit. In addition to local alterations of the transition path geometry, more fundamental global changes may exist. For instance, when the dissipation is weak, heteroclinic connections that exist in the overdamped limit do not necessarily have a counterpart in the Langevin system, potentially leading to different transition rates. Furthermore, when the friction coefficient depends on the velocity, the overdamped limit no longer exists, but it is still possible to efficiently find instantons. The approach, we employed for these discoveries, was based on (i) a simple rewriting of the Freidlin–Wentzell action in terms of time-reversed dynamics and (ii) an adaptation of the string method, which was originally designed for gradient systems, to this specific non-gradient system.

Hidden entropy production and work fluctuations in an ideal active gas.

Collections of self-propelled particles that move persistently by continuously consuming free energy are a paradigmatic example of active matter. In these systems, unlike Brownian "hot colloids," the breakdown of detailed balance yields a continuous production of entropy at steady state, even for an ideal active gas. We quantify the irreversibility for a noninteracting active particle in two dimensions by treating both conjugated and time-reversed dynamics. By starting with underdamped dynamics, we identify a hidden rate of entropy production required to maintain persistence and prevent the rapidly relaxing momenta from thermalizing, even in the limit of very large friction. Additionally, comparing two popular models of self-propulsion with identical dissipation on average, we find that the fluctuations and large deviations in work done are markedly different, providing thermodynamic insight into the varying extents to which macroscopically similar active matter systems may depart from equilibrium.

Equivalence of nonequilibrium ensembles in turbulence models.

Understanding under what conditions it is possible to construct equivalent ensembles is key to advancing our ability to connect microscopic and macroscopic properties of nonequilibrium statistical mechanics. In the case of fluid dynamical systems, one issue is to test whether different models for viscosity lead to the same macroscopic properties of the fluid systems in different regimes. Such models include, besides the standard choice of constant viscosity, cases where the time symmetry of the evolution equations is exactly preserved, as it must be in the corresponding microscopic systems, when available. Here a time-reversible dynamics is obtained by imposing the conservation of global observables. We test the equivalence of reversible and irreversible ensembles for the case of a multiscale shell model of turbulence. We verify that the equivalence is obeyed for the mean values of macroscopic observables, up to an error that vanishes as the system becomes more and more chaotic.

Time irreversibility from symplectic non-squeezing

The issue of how time reversible microscopic dynamics gives rise to macroscopic irreversible processes has been a recurrent issue in Physics since the time of Boltzmann whose ideas shaped, and essentially resolved, such an apparent contradiction. Following Boltzmann’s spirit and ideas, but employing Gibbs’s approach, we advance the view that macroscopic irreversibility of Hamiltonian systems of many degrees of freedom can be also seen as a result of the symplectic non-squeezing theorem.

Effective time reversal and echo dynamics in the transverse field Ising model

The question of thermalisation in closed quantum many-body systems has received a lot of attention in the past few years. An intimately related question is whether a closed quantum system shows irreversible dynamics. However, irreversibility and what we actually mean by this in a quantum many-body system with unitary dynamics has been explored very little. In this work we investigate the dynamics of the Ising model in a transverse magnetic field involving an imperfect effective time reversal. We propose a definition of irreversibility based on the echo peak decay of observables. Inducing the effective time reversal by different protocols we find an algebraic decay of the echo peak heights or an ever persisting echo peak indicating that the dynamics in this model is well reversible.

Quantum-Enhanced Sensing Based on Time Reversal of Nonlinear Dynamics

We experimentally demonstrate a nonlinear detection scheme exploiting time-reversal dynamics that disentangles continuous variable entangled states for feasible readout. Spin-exchange dynamics of Bose-Einstein condensates is used as the nonlinear mechanism which not only generates entangled states but can also be time reversed by controlled phase imprinting. For demonstration of a quantum-enhanced measurement we construct an active atom SU(1,1) interferometer, where entangled state preparation and nonlinear readout both consist of parametric amplification. This scheme is capable of exhausting the quantum resource by detecting solely mean atom numbers. Controlled nonlinear transformations widen the spectrum of useful entangled states for applied quantum technologies.

An efficient and stable hybrid extended Lagrangian/self-consistent field scheme for solving classical mutual induction.

We have adapted a hybrid extended Lagrangian self-consistent field (EL/SCF) approach, developed for time reversible Born Oppenheimer molecular dynamics for quantum electronic degrees of freedom, to the problem of classical polarization. In this context, the initial guess for the mutual induction calculation is treated by auxiliary induced dipole variables evolved via a time-reversible velocity Verlet scheme. However, we find numerical instability, which is manifested as an accumulation in the auxiliary velocity variables, that in turn results in an unacceptable increase in the number of SCF cycles to meet even loose convergence tolerances for the real induced dipoles over the course of a 1 ns trajectory of the AMOEBA14 water model. By diagnosing the numerical instability as a problem of resonances that corrupt the dynamics, we introduce a simple thermostating scheme, illustrated using Berendsen weak coupling and Nose-Hoover chain thermostats, applied to the auxiliary dipole velocities. We find that the inertial EL/SCF (iEL/SCF) method provides superior energy conservation with less stringent convergence thresholds and a correspondingly small number of SCF cycles, to reproduce all properties of the polarization model in the NVT and NVE ensembles accurately. Our iEL/SCF approach is a clear improvement over standard SCF approaches to classical mutual induction calculations and would be worth investigating for application to ab initio molecular dynamics as well.

On surface hopping and time-reversal.

While individual Tully-style fewest switches surface hopping (FSSH) trajectories are stochastic and cannot be inverted in time, it is possible to reverse in time the dynamics of a swarm of FSSH trajectories. Here we show exactly how to invert such dynamics, and we investigate the stability of such time-reversed surface hopping dynamics. We demonstrate that FSSH trajectories can be inverted successfully for short time periods, but the time-reversed dynamics become unstable for long times with multiple hopping events. We argue that this instability of FSSH going backward in time can be correlated with the stability of the FSSH algorithm going forward in time.