Time-dependent Quantum System Research Articles

Origins of Electromagnetic Radiation from Spintronic Terahertz Emitters: A Time-Dependent Density Functional Theory plus Jefimenko Equations Approach.

Microscopic origins of charge currents and electromagnetic (EM) radiation generated by them in spintronic THz emitters-such as, femtosecond laser pulse-driven single magnetic layer or its heterostructures with a nonmagnetic layer hosting strong spin-orbit coupling (SOC)-remain poorly understood despite nearly three decades since the discovery of ultrafast demagnetization. We introduce a first-principles method to compute these quantities, where the dynamics of charge and current densities is obtained from real-time time-dependent density functional theory, which are then fed into the Jefimenko equations for properly retarded electric and magnetic field solutions of the Maxwell equations. By Fourier transforming different time-dependent terms in the Jefimenko equations, we unravel that in the 0.1-30THz range the electric field of far-field EM radiation by the Ni layer, chosen as an example, is dominated by charge current pumped by demagnetization, while often invoked magnetic dipole radiation from the time-dependent magnetization of a single magnetic layer is a negligible effect. Such an effect of charge current pumping by a time-dependent quantum system, whose magnetization is shrinking while its vector does not rotate, does not require any spin-to-charge conversion via SOC effects. In the Ni/Pt bilayer, EM radiation remains dominated by the charge current within the Ni layer, whose magnitude is larger than in the case of a single Ni layer due to faster demagnetization, while often invoked spin-to-charge conversion within the Pt layer provides an additional but smaller contribution. By using the Poynting vector and its flux, we also quantify the efficiency of conversion of light into emitted EM radiation, and its angular distribution.

Study of uncertainty, average energy, and thermodynamic quantities of the time dependent quantum system

Study of uncertainty, average energy, and thermodynamic quantities of the time dependent quantum system

Adiabatic Lindbladian Evolution with Small Dissipators

We consider a time-dependent small quantum system weakly coupled to an environment, whose effective dynamics we address by means of a Lindblad equation. We assume the Hamiltonian part of the Lindbladian is slowly varying in time and the dissipator part has small amplitude. We study the properties of the evolved state of the small system as the adiabatic parameter and coupling constant both go to zero, in various asymptotic regimes. In particular, we analyse the deviations of the transition probabilities of the small system between the instantaneous eigenspaces of the Hamiltonian with respect to their values in the purely Hamiltonian adiabatic setup, as a function of both parameters.

Average energy and quantum similarity of a time dependent quantum system subject to Pöschl–Teller potential

Average energy and quantum similarity of a time dependent quantum system subject to Pöschl–Teller potential

Nonadiabatic evolution and thermodynamics of a time-dependent open quantum system

We investigate the dynamic evolution and thermodynamic process of a driven quantum system immersed in a finite-temperature heat bath. A Born-Markovian quantum master equation is formally derived for the time-dependent system with discrete energy levels. This quantum master equation can be applied to situations with a broad range of driving speeds and bath temperatures and thus be used to study the finite-time quantum thermodynamics even when nonadiabatic transition and dissipation coexist. The dissipative Landau-Zener model is analyzed as an example. The population evolution and transition probability of the model reveal the importance of the competition between driving and dissipation beyond the adiabatic regime. Moreover, local maximums of irreversible entropy production occur at intermediate sweep velocity and finite temperature, which the low-dissipation model cannot describe.

Effect of a deformed cavity on a time-dependent quantum system containing an entangled two modes.

In this manuscript, the phenomenon of time dependence is treated using the integral property of a model consisting of interaction of an atom with a cavity in which a bi-mode field of an amplifier type. The exact solution is obtained through the Schrodinger equation, followed by the wave function characteristic of the proposed system. The effect of both the deformed pair coherent states and the time dependence on some statistical quantities are studied. The phenomena of revival and collapse are studied by computing the atomic inversion. Moreover, the entanglement between the parts of the quantum system is studied, and the periods of squeezing are determined by entropy squeezing and variance squeezing. The results are also compared and statistical quantities linked together.

Variational principle for time-periodic quantum systems

Abstract A variational principle enabling one to compute individual Floquet states of a periodically time-dependent quantum system is formulated, and successfully tested against the benchmark system provided by the analytically solvable model of a linearly driven harmonic oscillator. The principle is particularly well suited for tracing individual Floquet states through parameter space, and may allow one to obtain Floquet states even for very high-dimensional systems which cannot be treated by the known standard numerical methods.

Adiabatic Transitions in a Two-Level System Coupled to a Free Boson Reservoir

We consider a time-dependent two-level quantum system interacting with a free Boson reservoir. The coupling is energy conserving and depends slowly on time, as does the system Hamiltonian, with a common adiabatic parameter \(\varepsilon \). Assuming that the system and reservoir are initially decoupled, with the reservoir in equilibrium at temperature \(T\ge 0\), we compute the transition probability from one eigenstate of the two-level system to the other eigenstate as a function of time, in the regime of small \(\varepsilon \) and small coupling constant \(\lambda \). We analyse the deviation from the adiabatic transition probability obtained in the absence of the reservoir.

Distinct Bound of the Quantum Speed Limit via the Gauge Invariant Distance.

We derive a distinct bound of the quantum speed limit for a non-Hermitian quantum system by employing the gauge invariant and geometric natures of quantum mechanics. The bound is of geometric properties since it relates to the geometric phase of the quantum system, and it is tighter than the Mandelstam-Tamm and Margolus-Levitin bounds in some cases. Also, by making the geodesic assumption, the analog of the Margolus-Levitin bound is derived for the time-dependent (non-)Hermitian quantum system. These two bounds reflect the impacts of the transmission modes of the state vectors on the evolution path in the manifold.

The upper bound function of nonadiabatic dynamics in parametric driving quantum systems**Project supported by the National Natural Science Foundation of China (Emergency Project, Grant Nos. 11447025 and 11847308).

The adiabatic control is a powerful technique for many practical applications in quantum state engineering, light-driven chemical reactions and geometrical quantum computations. This paper reveals a speed limit of nonadiabatic transition in a general time-dependent parametric quantum system that leads to an upper bound function which lays down an optimal criteria for the adiabatic controls. The upper bound function of transition rate between instantaneous eigenstates of a time-dependent system is determined by the power fluctuations of the system relative to the minimum gap between the instantaneous levels. In a parametric Hilbert space, the driving power corresponds to the quantum work done by the parametric force multiplying the parametric velocity along the parametric driving path. The general two-state time-dependent models are investigated as examples to calculate the bound functions in some general driving schemes with one and two driving parameters. The calculations show that the upper bound function provides a tighter real-time estimation of nonadiabatic transition and is closely dependent on the driving frequencies and the energy gap of the system. The deviations of the real phase from Berry phase on different closed paths are induced by the nonadiabatic transitions and can be efficiently controlled by the upper bound functions. When the upper bound is adiabatically controlled, the Berry phases of the electronic spin exhibit nonlinear step-like behaviors and it is closely related to topological structures of the complicated parametric paths on Bloch sphere.

Steering random spin systems to speed up the quantum adiabatic algorithm

A general time-dependent quantum system can be driven fast from its initial ground state to its final ground state without generating transitions by adding a steering term to the Hamiltonian. We show how this technique can be modified to improve on the standard quantum adiabatic algorithm by making a single-particle and cluster approximation to the steering term. The method is applied to a one-dimensional Ising model in a random field. For the limit of strong disorder, the correction terms significantly enhance the probability for the whole system to remain in the ground state for the proposed non-stoquastic annealing protocol. We demonstrate that even when transitions occur for stronger interaction between qubits, the most probable quantum state is one of the lower energy states of the final Hamiltonian. Since the method can be applied to any model, and more sophisticated approximations to the steering term are possible, the new technique opens up an avenue for the improvement of the quantum adiabatic algorithm.

Exotic dynamical evolution in a secant-pulse-driven quantum system

We investigate an explicitly time-dependent quantum system driven by a secant-pulse external field. By solving the Schr\"odinger equation exactly, we elucidate exotic properties of the system with respect to its dynamical evolution: On the one hand, the system is shown to be essentially nonadiabatic, which prohibits an adiabatic approximation for its dynamics; on the other hand, the loop evolution of the model can induce a geometric phase which, analogous to the Berry phase of the cyclic adiabatic evolution, is in direct proportion to the solid angle subtended by the path of the state vector. Moreover, we extend the model and show that the described properties coincide in a special family of secant-pulse-driven models.

Solvable two-dimensional time-dependent non-Hermitian quantum systems with infinite dimensional Hilbert space in the broken PT-regime

We provide exact analytical solutions for a two-dimensional explicitly time-dependent non-Hermitian quantum system. While the time-independent variant of the model studied is in the broken PT-symmetric phase for the entire range of the model parameters, and has therefore a partially complex energy eigenspectrum, its time-dependent version has real energy expectation values at all times. In our solution procedure we compare the two equivalent approaches of directly solving the time-dependent Dyson equation with one employing the Lewis–Riesenfeld method of invariants. We conclude that the latter approach simplifies the solution procedure due to the fact that the invariants of the non-Hermitian and Hermitian system are related to each other in a pseudo-Hermitian fashion, which in turn does not hold for their corresponding time-dependent Hamiltonians. Thus constructing invariants and subsequently using the pseudo-Hermiticity relation between them allows to compute the Dyson map and to solve the Dyson equation indirectly. In this way one can bypass to solve nonlinear differential equations, such as the dissipative Ermakov–Pinney equation emerging in our and many other systems.

Quantum parameter estimation with the Landau-Zener transition

We investigate the fundamental limits in precision allowed by quantum mechanics from Landau-Zener transitions, concerning Hamiltonian parameters. While the Landau-Zener transition probabilities depend sensitively on the system parameters, much more precision may be obtained using the acquired phase, quantified by the quantum Fisher information. This information scales with a power of the elapsed time for the quantum case, whereas it is time-independent if the transition probabilities alone are used. We add coherent control to the system, and increase the permitted maximum precision in this time-dependent quantum system. The case of multiple passes before measurement, "Landau-Zener-Stueckelberg interferometry", is considered, and we demonstrate that proper quantum control can cause the quantum Fisher information about the oscillation frequency to scale as $T^4$, where $T$ is the elapsed time.

Effect of Poisson noise on adiabatic quantum control

We present a detailed derivation of the master equation describing a general time-dependent quantum system with classical Poisson white noise and outline its various properties. We discuss the limiting cases of Poisson white noise and provide approximations for the different noise strength regimes. We show that using the eigenstates of the noise superoperator as a basis can be a useful way of expressing the master equation. Using this we simulate various settings to illustrate different effects of Poisson noise. In particular, we show a dip in the fidelity as a function of noise strength where high fidelity can occur in the strong noise regime for some cases. We also investigate recent claims [Jing et al., Phys. Rev. A 89 032110 (2014)] that this type of noise may improve rather than destroy adiabaticity.

The Rigorous Derivation of the 2D Cubic Focusing NLS from Quantum Many-Body Evolution

We consider a 2D time-dependent quantum system of $N$-bosons with harmonic external confining and \emph{attractive} interparticle interaction in the Gross-Pitaevskii scaling. We derive stability of matter type estimates showing that the $k$-th power of the energy controls the $H^{1}$ Sobolev norm of the solution over $k$-particles. This estimate is new and more difficult for attractive interactions than repulsive interactions. For the proof, we use a version of the finite-dimensional quantum di Finetti theorem from [49]. A high particle-number averaging effect is at play in the proof, which is not needed for the corresponding estimate in the repulsive case. This a priori bound allows us to prove that the corresponding BBGKY hierarchy converges to the GP limit as was done in many previous works treating the case of repulsive interactions. As a result, we obtain that the \emph{focusing} nonlinear Schr\"{o}dinger equation is the mean-field limit of the 2D time-dependent quantum many-body system with attractive interatomic interaction and asymptotically factorized initial data. An assumption on the size of the $L^{1}$-norm of the interatomic interaction potential is needed that corresponds to the sharp constant in the 2D Gagliardo-Nirenberg inequality though the inequality is not directly relevant because we are dealing with a trace instead of a power.

Communication: satisfying fermionic statistics in the modeling of open time-dependent quantum systems with one-electron reduced density matrices.

For an open, time-dependent quantum system, Lindblad derived the most general modification of the quantum Liouville equation in the Markovian approximation that models environmental effects while preserving the non-negativity of the system's density matrix. While Lindblad's modification is correct for N-electron density matrices, solution of the Liouville equation with a Lindblad operator causes the one-electron reduced density matrix (1-RDM) to violate the Pauli exclusion principle. Consequently, after a short time, the 1-RDM is not representable by an ensemble N-electron density matrix (not ensemble N-representable). In this communication, we derive the necessary and sufficient constraints on the Lindbladian matrix within the Lindblad operator to ensure that the 1-RDM remains N-representable for all time. The theory is illustrated by considering the relaxation of an excitation in several molecules F2, N2, CO, and BeH2 subject to environmental noise.

The interaction between a single two-level atom and the combination of a frequency converter and the sub-harmonic generation

The problem of a time-dependent quantum system, which consists of coupled sub-harmonic generation with the parametric down conversion injected within a single cavity containing an atom, is considered. The problem is transformed into the interaction between the su(1,1) quantum system and a single two-level atom. The wave function is calculated and the expectation values for the dynamical operators are obtained. It is shown that the phenomenon of collapses and revivals are sensitive to the variation of the Bargmann index k and the Perelomov parameter η; moreover, a coherent trapping behavior is seen at the atomic coherence angle θ = π/2. The phenomena of bunching and anti-bunching are reported where the atomic angle θ and the phase angle φ as well as η are the most effective parameters. They are also effective for the variance squeezing, however the Bargmann index k increases the fluctuations and decreases the amount of squeezing. For the linear entropy we have observed that the index k has no effect, but the main effective parameters are θ, φ and η in addition to the ratio between the atomic frequency and the coupling parameter.

Density-potential mappings in quantum dynamics

In a recent letter [Europhys. Lett. 95, 13001 (2011)] the question of whether the density of a time-dependent quantum system determines its external potential was reformulated as a fixed point problem. This idea was used to generalize the existence and uniqueness theorems underlying time-dependent density functional theory. In this work we extend this proof to allow for more general norms and provide a numerical implementation of the fixed-point iteration scheme. We focus on the one-dimensional case as it allows for a more in-depth analysis using singular Sturm-Liouville theory and at the same time provides an easy visualization of the numerical applications in space and time. We give an explicit relation between the boundary conditions on the density and the convergence properties of the fixed-point procedure via the spectral properties of the associated Sturm-Liouville operator. We show precisely under which conditions discrete and continuous spectra arise and give explicit examples. These conditions are then used to show that in the most physically relevant cases the fixed point procedure converges. This is further demonstrated with an example.

Equivalence between Redfield- and master-equation approaches for a time-dependent quantum system and coherence control

We present a derivation of the Redfield formalism for treating the dissipative dynamics of a time-dependent quantum system coupled to a classical environment. We compare such a formalism with the master equation approach where the environments are treated quantum mechanically. Focusing on a time-dependent spin-1/2 system we demonstrate the equivalence between both approaches by showing that they lead to the same Bloch equations and, as a consequence, to the same characteristic times $T_{1}$ and $T_{2}$ (associated with the longitudinal and transverse relaxations, respectively). These characteristic times are shown to be related to the operator-sum representation and the equivalent phenomenological-operator approach. Finally, we present a protocol to circumvent the decoherence processes due to the loss of energy (and thus, associated with $T_{1}$). To this end, we simply associate the time-dependence of the quantum system to an easily achieved modulated frequency. A possible implementation of the protocol is also proposed in the context of nuclear magnetic resonance.