Thermofield Dynamics Approach Research Articles

Finite-Temperature Hole-Magnon Dynamics in an Antiferromagnet.

Employing the numerically accurate multiple Davydov Ansatz in combination with the thermo-field dynamics approach, we delve into the interplay of the finite-temperature dynamics of holes and magnons in an antiferromagnet, which allows for scrutinizing previous predictions from the self-consistent Born approximation while offering, for the first time, accurate finite-temperature computation of detailed magnon dynamics as a response and a facilitator to the hole motion. The study also uncovers a pronounced temperature dependence of the magnon and hole populations, pointing to the feasibility of potential thermal manipulation and control of hole dynamics. Our methodology can be applied not only to the calculation of steady-state angular-resolved photoemission spectra but also to the simulation of femtosecond terahertz pump-probe and other nonlinear signals for the characterization of antiferromagnetic materials.

Soft theorems and memory effects at finite temperatures

We study the soft theorems for photons and gravitons at finite temperatures using the thermofield dynamics approach. The soft factors lose universality at finite temperatures as the soft amplitudes depend on the nature (or spin) of the particles participating in the scattering processes. However, at low temperatures, a universal behavior is observed in the cross-section of the soft processes. Further, we obtain the thermal contribution to the electromagnetic and gravitational memory effects and show that they are related to the soft factors consistently. The expected zero temperature results are obtained from the soft factors and memories. The thermal effects in soft theorems and memories seem to be sensitive to the spin of the particles involved in scattering.

Thermodynamics and tachyon condensation of the dressed-dynamical unstable Dp-branes

Using the boundary state formalism and thermo field dynamics approach, we study a Dp-brane at finite temperature in which the background Kalb–Ramond field, a U(1) gauge potential, and tachyon field are turned on together with a general tangential dynamics. The thermal entropy of the brane will be studied. In addition, the behavior of the entropy after the tachyon condensation process will be investigated and some thermodynamic interpretations will be extracted.

Thermo-Field Dynamics Approach to Photo-induced Electronic Transitions Driven by Incoherent Thermal Radiation.

The effects of thermal light-matter interaction on the dynamics of photo-induced electronic transitions in molecules are investigated using a novel first principles approach based on the thermo-field dynamics description of both the molecular vibrational modes and of the radiation field. The developed approach permits numerically accurate simulations of quantum dynamics of electronic/excitonic systems coupled to nuclear and photonic baths kept at different temperatures. The baths can be described by arbitrary spectral densities and can have any system-bath coupling strengths. In agreement with the results obtained previously by less rigorous methods, we show that the excitation process obtained by the continuous interaction with the suddenly turned-on thermal radiation field creates a mixed ensemble having a nonnegligible component consisting of a superposition of vibronic eigenstates which can sustain coherent oscillations for relatively long times. The results become especially relevant for the dynamics of electronic transitions upon sunlight excitation. Analytical results based on time-dependent perturbation theory support the numerical simulations and provide a simple interpretation of the time evolution of quantum observables.

Vacuum Cherenkov radiation at finite temperature

In this paper we examine the thermal effects of the vacuum Cherenkov radiation in a Lorentz- and CPT-violating electrodynamics. We compute the thermal contribution to the Cherenkov radiation rate within the Thermofield Dynamics approach. Since the model under consideration possesses a consistent canonical quantization and also fulfills the physical constraints in order to this vacuum process to happen, it is a perfect candidate to implement the study at finite temperature. We evaluate in details the instantaneous rate of energy loss for a charge, and show that the radiation rate is significantly modified at very high temperatures. Intriguingly, we further observe that when the temperature goes to infinity the radiation rate goes to zero even if the process is kinematically allowed.

Quantum Dynamics of Electron–Hole Separation in Stacked Perylene Diimide-Based Self-Assembled Nanostructures

We report on high-dimensional quantum dynamical simulations of electron–hole separation in self-assembled mesomorphic nanostructures composed of donor–acceptor conjugated co-oligomers. The latter are based on perylene diimide (PDI) acceptor units combined with fluorene-thiophene-benzothiadiazole donor units, which form highly ordered, stacked structural motifs upon self-assembly. Simulations are shown for a first-principles parametrized model lattice of 25 stacked PDI units under the effects of an applied external field and temperature. The simulations are carried out with the multilayer multiconfiguration time-dependent Hartree (ML-MCTDH) method with nearly 900 vibrational degrees of freedom and 25 electronic states. Temperature effects are included using the thermofield dynamics approach. A transition between a short-time coherent dynamics and a kinetic regime is highlighted. From a flux-over-population analysis, electron–hole dissociation rates are obtained in the range of 5–20 ns–1 in the absence of static disorder, exhibiting a moderate field and temperature dependence. These results for electron–hole separation rates can be employed as a benchmark to calibrate the parametrization of kinetic Monte Carlo simulations applied to much larger lattice sizes.

Simulation of Time- and Frequency-Resolved Four-Wave-Mixing Signals at Finite Temperatures: A Thermo-Field Dynamics Approach

We propose a new approach to simulate four-wave-mixing signals of molecular systems at finite temperatures by combining the multiconfigurational Ehrenfest method with the thermo-field dynamics theory. In our approach, the four-time correlation functions at finite temperatures are mapped onto those at zero temperature in an enlarged Hilbert space with twice the vibrational degrees of freedom. As an illustration, we have simulated three multidimensional spectroscopic signals, time- and frequency-resolved fluorescence spectra, transient-absorption pump-probe spectra, and electronic two-dimensional (2D) spectra at finite temperatures, for a conical intersection-mediated singlet fission model of a rubrene crystal. It is shown that a detailed dynamical picture of the singlet fission process can be extracted from the three spectroscopic signals. An increasing temperature leads to lower intensities of the signals and broadened vibrational peaks, which can be attributed to faster singlet-triplet population transfer and stronger bath-induced electronic dephasing at higher temperatures.

Finite-Temperature, Anharmonicity, and Duschinsky Effects on the Two-Dimensional Electronic Spectra from Ab Initio Thermo-Field Gaussian Wavepacket Dynamics.

Accurate description of finite-temperature vibrational dynamics is indispensable in the computation of two-dimensional electronic spectra. Such simulations are often based on the density matrix evolution, statistical averaging of initial vibrational states, or approximate classical or semiclassical limits. While many practical approaches exist, they are often of limited accuracy and difficult to interpret. Here, we use the concept of thermo-field dynamics to derive an exact finite-temperature expression that lends itself to an intuitive wavepacket-based interpretation. Furthermore, an efficient method for computing finite-temperature two-dimensional spectra is obtained by combining the exact thermo-field dynamics approach with the thawed Gaussian approximation for the wavepacket dynamics, which is exact for any displaced, distorted, and Duschinsky-rotated harmonic potential but also accounts partially for anharmonicity effects in general potentials. Using this new method, we directly relate a symmetry breaking of the two-dimensional signal to the deviation from the conventional Brownian oscillator picture.

Quantum speed limit in the thermal spin-boson system with and without tunneling term

In this paper, we study the spin-bosonic model, with and without tunneling terms, in detail. The spin-bosonic model without tunneling is studied by using the thermofield dynamics approach. Indeed, by considering temperature, we show that environmental states, while they become entangled with system, approach thermal coherent states with different phases. In addition, by considering the tunneling term, we study the interplay of the environmental cut-off frequency as well as the impacts of environmental temperature on the quantum speed limit in both cases, i.e., spin-boson system with and without tunneling term. In these studies, we indicate temperature play more important role in compare with cut-off frequency to control the quantumness of a spin system.

Finite temperature dynamics of a Holstein polaron: The thermo-field dynamics approach

Combining the multiple Davydov D2 Ansatz with the method of thermo-field dynamics, we study finite temperature dynamics of a Holstein polaron on a lattice. It has been demonstrated, using the hierarchy equations of motion method as a benchmark, that our approach provides an efficient, robust description of finite temperature dynamics of the Holstein polaron in the simultaneous presence of diagonal and off-diagonal exciton-phonon coupling. The method of thermo-field dynamics handles temperature effects in the Hilbert space with key numerical advantages over other treatments of finite-temperature dynamics based on quantum master equations in the Liouville space or wave function propagation with Monte Carlo importance sampling. While for weak to moderate diagonal coupling temperature increases inhibit polaron mobility, it is found that off-diagonal coupling induces phonon-assisted transport that dominates at high temperatures. Results on the mean square displacements show that band-like transport features dominate the diagonal coupling cases, and there exists a crossover from band-like to hopping transport with increasing temperature when including off-diagonal coupling. As a proof of concept, our theory provides a unified treatment of coherent and incoherent transport in molecular crystals and is applicable to any temperature.

Lie algebras and generalized thermal coherent states

In this paper, we developed an algebraic formulation for the generalized thermal coherent states with a thermofield dynamics approach for multi-modes, based on coset space of Lie groups. In particular, we applied our construction on SU(2) and SU(1,[Formula: see text]1) symmetries and we obtain their thermal coherent states and density operator. We also calculate their thermal quantum Fidelity and thermal Wigner function.

Quantum electron-vibrational dynamics at finite temperature: Thermo field dynamics approach.

Quantum electron-vibrational dynamics in molecular systems at finite temperature is described using an approach based on the thermo field dynamics theory. This formulation treats temperature effects in the Hilbert space without introducing the Liouville space. A comparison with the theoretically equivalent density matrix formulation shows the key numerical advantages of the present approach. The solution of thermo field dynamics equations with a novel technique for the propagation of tensor trains (matrix product states) is discussed. Numerical applications to model spin-boson systems show that the present approach is a promising tool for the description of quantum dynamics of complex molecular systems at finite temperature.

Bulk from bi-locals in Thermo field CFT

We study the Large $N$ dynamics of the $O(N)$ field theory in the Thermo field dynamics approach. The question of recovering the high temperature phase and the corresponding $O(N)$ gauging is clarified. Through the associated bi-local representation we discuss the emergent bulk space-time and construction of (Higher spin) fields. We note the presence of `evanescent' modes in this construction and also the mixing of spins at finite temperature.

QUANTUM INFORMATION, THERMOFIELD DYNAMICS AND THERMALIZED BOSONIC OSCILLATOR

We show through Thermofield Dynamics approach that the action of the thermalized quantum logic gate on the thermalized state is equivalent to thermalization of the state that arise from the application of the nonthermalized quantum logic gate. In particular, we study the effect of temperature on a mixed state associated to a system capable of implementing a controlled-NOT (CNOT) quantum logic gate. According to a proposal in the literature, a way of implementing such a logic gate is by using a representation of the qubit states as elements of the Fock space of a bosonic system. We consider such a proposal and use the Thermofield Dynamics to determine the thermalized qubit states. The temperature acts as a quantum noise on pure states, making them a statistical mixture. In this context, we analyze the fidelity as a function of the temperature and using the Mandel parameter, we determine temperature ranges for which the statistics of the system becomes subpoissonian, poissonian and superpoissonian. Finally, we calculate the Wigner function, allowing an analysis of the thermal state in phase space, and we obtain that the increase of temperature decreases nonclassical properties of the system. The temperature range where one has a subpoissonian statistics and high fidelity is determined.

String in AdS black hole: A thermo field dynamic approach

Based on Maldacena's description of an eternal AdS-black hole, we reassess the Thermo Field Dynamics (TFD) formalism in the context of the AdS/CFT correspondence. The model studied here involves the maximally extended AdS-Schwarschild solution and two (non-interacting) copies of the CFT associated to the global AdS spacetime, along with an extension of the string by imposing natural gluing conditions in the horizon. We show that the gluing conditions in the horizon define a string boundary state which is identified with the TFD thermal vacuum, globally defined in the Kruskal extension of the AdS black hole. We emphasize the connection of this picture with unitary SU(1,1) TFD formulation and we show that information about the bulk and the conformal boundary is present in the SU(1,1) parameters. Using the unitary SU(1,1) TFD formulation, a canonical prescription for calculating the worldsheet real time thermal Green's function is made and the entropy associated with the entanglement of the two CFT's is calculated.

Thermal magnetized D-branes on in the generalized thermo-field dynamics approach

We construct the D-brane states at finite temperature in thermal equilibrium in the spacetime in the presence of cold (unthermalized) Kalb–Ramond (KR) and U(1) gauge potential background. To this end, we first generalize the thermo-field dynamics to wrapped closed strings. This generalization is consistent with the spatial translation invariance on the string world-sheet. Next, we determine the thermal string vacuum and define the entropy operator. From these data we calculate the entropy of the closed string and the free energy. Finally, we define the thermal D-brane states in in the presence of a cold constant KR field and U(1) gauge potential as the boundary states of the thermal closed string and compute their entropy.

Finite-temperature nonlinear dynamics in cavity QED: A thermofield dynamics approach

Heath-bath effects in the dynamics of atom + cavity system are studied. The temperature effects are explored using thermofield dynamics formalism. It is found that the dynamics of the system is sensitive to small changes in the temperature and the thermal effects lead to increasing instabilities by causing transitions from regular to chaotic motion.

Two-dimensional thermofield bosonization II: Massive fermions

We consider the perturbative computation of the N-point function of chiral densities of massive free fermions at finite temperature within the thermofield dynamics approach. The infinite series in the mass parameter for the N-point functions are computed in the fermionic formulation and compared with the corresponding perturbative series in the interaction parameter in the bosonized thermofield formulation. Thereby we establish in thermofield dynamics the formal equivalence of the massive free fermion theory with the sine-Gordon thermofield model for a particular value of the sine-Gordon parameter. We extend the thermofield bosonization to include the massive Thirring model.

First order semiclassical thermal string in the AdS spacetime

We formulate the finite temperature theory for the free thermal excitations of the bosonic string in the anti-de Sitter (AdS) spacetime in the Thermo Field Dynamics (TFD) approach. The spacetime metric is treated exactly while the string and the thermal reservoir are semiclassically quantized at the first order perturbation theory with respect to the dimensionless parameter $\epsilon = \a ' H^{-2}$. In the conformal $D=2+1$ black-hole AdS background the quantization is exact. The method can be extended to the arbitrary AdS spacetime only in the first order perturbation. This approximation is taken in the center of mass reference frame and it is justified by the fact that at the first order the string dynamics is determined only by the interaction between the {\em free} string oscillation modes and the {\em exact} background. The first order thermal string is obtained by thermalization of the $T = 0$ system carried on by the TFD Bogoliubov operator. We determine the free thermal string states and compute the local entropy and free energy in the center of mass reference frame.

Closed string thermal torus from thermo field dynamics

In this Letter a topological interpretation for the string thermal vacuum in the thermo field dynamics (TFD) approach is given. As a consequence, the relationship between the imaginary time and TFD formalisms is achieved when both are used to study closed strings at finite temperature. The TFD approach starts by duplicating the system's degrees of freedom, defining an auxiliary (tilde) string. In order to lead the system to finite temperature a Bogoliubov transformation is implemented. We show that the effect of this transformation is to glue together the string and the tilde string to obtain a torus. The thermal vacuum appears as the boundary state for this identification. Also, from the thermal state condition, a Kubo–Martin–Schwinger condition for the torus topology is derived.