Terahertz Generation In Lithium Niobate Research Articles

Nonlinear distortion and spatial dispersion of intense terahertz generation in lithium niobate via the tilted pulse front technique

We systematically investigate the influences of the input infrared spectrum, chirp, and polarization on the emitted intense terahertz spectrum and spatial dispersion in lithium niobate via optical rectification. The terahertz yield and emission spectrum depend on both the chirp and spectrum of the input pump laser pulses. We also observe slight non-uniform spatial dispersion using a knife-edge measurement, which agrees well with the original predictions. The possible mechanism is the nonlinear distortion effect caused by high-energy laser pumping. Our study is very important and useful for developing intense terahertz systems with applications in extreme terahertz sciences and nonlinear phenomena.

Optimization of highly efficient terahertz generation in lithium niobate driven by Ti:sapphire laser pulses with 30 fs pulse duration

We systematically study the optimization of highly efficient terahertz (THz) generation in lithium niobate (LN) crystal pumped by 800 nm laser pulses with 30 fs pulse duration. At room temperature, we obtain a record optical-to-THz energy conversion efficiency of 0.43% by chirping the pump laser pulses. Our method provides a new technique for producing millijoule THz radiation in LN via optical rectification driven by joule-level Ti:sapphire laser systems, which deliver sub-50-fs pulse durations.

Dual-mode tunable terahertz generation in lithium niobate driven by spatially shaped femtosecond laser.

A new approach for dual-mode (namely broadband mode and narrowband mode) terahertz (THz) pulses generation in a single lithium niobate (LN) crystal excited by spatially shaped tilted-pulse-front femtosecond (fs) laser pulse was proposed and experimentally demonstrated. The two THz emission modes are generated simultaneously while spatially separated. Both central frequency and bandwidth of narrowband THz emission is controllable by in situ tuning the spatial modulation period and beam size of the fs-laser, and the broadband (0.1-1.5 THz) THz emission keeps almost unchanged while tuning the narrowband emission. Further optimization achieves the narrowband THz emission with energy spectral density up to 0.27 μJ/THz and with bandwidth narrowly down to 23 GHz. Such dual-mode THz source is useful for nonlinear THz optics, such as selected resonant THz excitation with broadband THz probe spectroscopy of crystalline matters.

Terahertz generation in lithium niobate driven by Ti:sapphire laser pulses and its limitations.

We experimentally investigate the limits of 800-nm-to-terahertz (THz) energy conversion in lithium niobate at room temperature driven by amplified Ti:sapphire laser pulses with tilted pulse front. The influence of the pump central wavelength, pulse duration, and fluence on THz generation is studied. We achieved a high peak efficiency of 0.12% using transform limited 150 fs pulses and observed saturation of the optical-to-THz conversion efficiency at a fluence of 15 mJ/cm(2) for this pulse duration. We experimentally identify two main limitations for the scaling of optical-to-THz conversion efficiencies: (i) the large spectral broadening of the optical pump spectrum in combination with large angular dispersion of the tilted pulse front and (ii) free-carrier absorption of THz radiation due to multi-photon absorption of the 800 nm radiation.

Limitations to THz generation by optical rectification using tilted pulse fronts

Terahertz (THz) generation by optical rectification (OR) using tilted-pulse-fronts is studied. A one-dimensional (1-D) model which simultaneously accounts for (i) the nonlinear coupled interaction of the THz and optical radiation, (ii) angular and material dispersion, (iii) absorption, iv) self-phase modulation and (v) stimulated Raman scattering is presented. We numerically show that the large experimentally observed cascaded frequency down-shift and spectral broadening (cascading effects) of the optical pump pulse is a direct consequence of THz generation. In the presence of this large spectral broadening, the large angular dispersion associated with tilted-pulse-fronts which is ~15-times larger than material dispersion, accentuates phase mismatch and degrades THz generation. Consequently, this cascading effect in conjunction with angular dispersion is shown to be the strongest limitation to THz generation in lithium niobate for pumping at 1 µm. It is seen that the exclusion of these cascading effects in modeling OR, leads to a significant overestimation of the optical-to-THz conversion efficiency. The results are verified with calculations based on a 2-D spatial model. The simulation results are supported by experiments.