Using carbon-negative biochar is promising for the carbon footprints reduction of construction materials; however, directly utilizing biochar in concrete would negatively influence its mechanical properties, particularly when the utilizing volume exceeds a certain threshold. By designing as a core-shell structure through cold-bonding method, a novel carbon-negative core-shell aggregate (CSA) with a biochar core and a cementitious shell was developed in this study. The aggregate was characterized by strength, density, and water absorption measurements, meanwhile, analyzed by hydration heat, XRD, TGA, SEM/BSE, and X-CT. The results showed that the developed MG80 biochar-CSA attained a loose bulk density of 789 kg/m3. It exhibited a crushing strength of 6.84 MPa, a water absorption value of 19.4 %, and a significantly superior strength efficiency of 8669 Pa·m3/kg compared to commercially sintered artificial lightweight aggregates and other cold-bonded aggregates documented in literature. The carbon emission assessment indicated that producing one ton of MG80 biochar-CSA emitted −69 kg CO2, which was much lower than the commercial sintered aggregates. Concrete developed by replacing natural aggregate with 90 % MG80 biochar-CSA exhibited a compressive strength of 42.2 MPa while maintaining lightweight with density of 1866 kg/m3, which conforms to the standard-classified structural lightweight aggregate concrete.