The use of carbon fiber-reinforced polymer (CFRP) as an alternative to steel tendons in prestressed concrete is increasingly favored due to its non-corrosive properties. A critical aspect of this substitution is the bond strength required to effectively transfer pre-stressing force. This study investigates the bond strengths of CFRP rods, CFRP strands, and steel strands following ISO 10406 standards. The research comprehensively explores the influence of cable type, cable surface roughness, and concrete strength on bond-slip behavior. Experimental results were augmented using a data augmentation method to enrich the dataset, which facilitated the development of a robust random forest (RF)-based prediction model for bond strength. The RF model achieved strong performance metrics, including a mean absolute percentage error (MAE) of 17.9 % and an R-value of 0.97, underscoring its efficacy in predicting bond strength. Notably, the model highlighted the significant impact of cable surface roughness on bond strength relative to other parameters studied based on the feature importance analysis. This study contributes to advancing the understanding of CFRP's applicability as a steel tendon replacement in prestressed concrete structures. The findings emphasize the importance of surface characteristics in optimizing bond strength, providing valuable insights for structural engineers and material scientists.