The appearance of ultra-low-frequency oscillations in the grid at the sending end, after asynchronous grid interconnection, poses a significant threat to the stable operation of the system. For post-asynchronous interconnection in a multi-DC transmission system, an investigation is conducted to analyze the causes of ultra-low-frequency oscillations and the utilization of a Frequency Limit Controller (FLC) which aims to suppress these oscillations. Furthermore, a method is developed to rank DC sensitivity, considering the hydroelectric distribution in the sending-end grid, by combining the DC FLC impact factor and DC control sensitivity. Subsequently, a novel approach for ultra-low-frequency oscillation suppression is proposed. This approach employs the stochastic subspace method for parameter estimation and the NSGA-II optimization algorithm to convert the multi-DC optimization challenge into multiple sequential cyclic optimization problems, each focusing on a single DC, ensuring a more effective suppression of ultra-low-frequency oscillations. The proposed scheme’s effectiveness is validated through simulations using a specific locations’ interconnected power grid.