Parametric Down-conversion Research Articles

Hybrid III-V/Silicon Quantum Photonic Device Generating Broadband Entangled Photon Pairs

The demand for integrated photonic chips combining the generation and manipulation of quantum states of light is steadily increasing, driven by the need for compact and scalable platforms for quantum information technologies. While photonic circuits with diverse functionalities are being developed in different single material platforms, it has become crucial to realize hybrid photonic circuits that harness the advantages of multiple materials while mitigating their respective weaknesses, resulting in enhanced capabilities. Here, we demonstrate a hybrid III-V/silicon quantum photonic device combining the strong second-order nonlinearity and direct band gap of the III-V semiconductor platform with the high maturity and CMOS compatibility of the silicon photonic platform. Our device embeds the spontaneous parametric down-conversion (SPDC) of photon pairs into an AlGaAs source and their vertical routing to an adhesively bonded silicon-on-insulator circuitry, within an evanescent coupling scheme managing both polarization states. This enables the on-chip generation of broadband (>40 nm) telecom photons by type-0 and type-2 SPDC from the hybrid device, at room temperature and with internal pair generation rates exceeding 105s−1 for both types, while the pump beam is strongly rejected. Two-photon interference with 92% visibility (and up to 99% upon 5-nm spectral filtering) proves the high energy-time entanglement quality of the produced quantum state, thereby enabling a wide range of quantum information applications on chip, within a hybrid architecture compliant with electrical pumping and merging the assets of two mature and highly complementary platforms in view of out-of-the-lab deployment of quantum technologies. Published by the American Physical Society 2024

Multimode squeezed state for reconfigurable quantum networks at telecommunication wavelengths

Continuous variable encoding of quantum information requires the deterministic generation of highly correlated quantum states of light in the form of quantum networks, which, in turn, necessitates the controlled generation of a large number of squeezed modes. In this paper, we present an experimental source of multimode squeezed states of light at telecommunication wavelengths. Generation at such wavelengths is especially important as it can enable quantum information processing, communication, and sensing beyond the laboratory scale. We use a single-pass spontaneous parametric down-conversion process in a nonlinear waveguide pumped with the second harmonic of a femtosecond laser. Our measurements reveal significant squeezing in more than 21 frequency modes, with a maximum squeezing value exceeding 2.5 dB. We demonstrate multiparty entanglement by measuring the state's covariance matrix. Finally, we show the source reconfigurability by preparing few-node cluster states and measure their nullifier squeezing level. These results pave the way for a scalable implementation of continuous variable quantum information protocols at telecommunication wavelengths, particularly for multiparty, entanglement-based quantum communications. Moreover, the source is compatible with additional pulse-by-pulse multiplexing, which can be utilized to construct the necessary three-dimensional entangled structures for quantum computing protocols. Published by the American Physical Society 2024

Simple but efficient polarization-entangled photon sources

We report on the design and characterization of polarization-entangled photon sources at NIR and telecom wavelengths, based on spontaneous parametric downconversion in a linear interferometric arrangement with beam displacers. The sources demonstrate state-of-the-art performance with respect to detected brightness, heralding efficiency, and entanglement visibility. Featuring a stable and compact profile with simple alignment, they hold great promise for future development of field- and space-ready prototypes, alongside serving as a practical guide for researchers interested in designing efficient entangled photon sources.

Chirality-controlled second-order nonlinear frequency conversion in lithium niobate film metasurfaces.

The high-quality factor resonant metasurfaces have extensive applications in enhancing nonlinear frequency conversion efficiency at the subwavelength scale. However, methods for actively modulating the frequency conversion process are limited. We design a chiral lithium niobate film metasurface and investigate the photonic spin as a new degree of freedom to dynamically control the second-order nonlinear frequency conversion, without reconfiguring the structure by using external stimuli. The chiral resonance with circular dichroism (CD) of 0.62 gives rise to a high nonlinear CD of 0.84 in second-harmonic generation efficiency. Interestingly, combining the chiral resonance and an achiral quasi-bound state in the continuum enables us to investigate the photonic-spin-controlled sum-frequency generation and the photon pair generation from the spontaneous parametric downconversion process. Owing to the ultrahigh quality factor exceeding 103 both for two resonances, the second-order nonlinear frequency conversion occurs at a wavelength region of 0.2 nm, suggesting good monochromaticity. Our work opens new, to our knowledge, avenues for practical implementation of dynamically controlled nonlinear optical devices and will find utility in holography, switchable light sources, and information processing.

Noise analysis of a quasi-phase-matched quantum frequency converter and higher-order counter-propagating SPDC

Quantum frequency conversion (QFC) will be an indispensable ingredient in future quantum technologies. For example, large-scale fibre-based quantum networks will require QFC to interconnect heterogeneous building blocks like emitters, channels, memories, and detectors. The performance of existing QFC devices – typically realized in periodically poled nonlinear crystals – is often severely limited by parasitic noise that arises when the pump wavelength lies between the inter-converted wavelengths. Here we comprehensively investigate the noise spectrum of a QFC device pumped by a CW 1064 nm laser. The converter was realized as a bulk periodically poled potassium titanyl phosphate (ppKTP) crystal quasi-phase-matched for conversion between 637 nm and 1587 nm, which was also polished and coated to resonantly enhance the pump field by a factor of 50. While Raman scattering dominates the noise background from 1140 nm to 1330 nm, at larger energy shifts (beyond 60 THz), parasitic spontaneous parametric down-conversion (SPDC) is the strongest noise source. Further, the noise spectrum was contaminated by a regular succession of narrow-band peaks, which we attribute to a heretofore unidentified higher-order counter-propagating SPDC processes – with quasi-phase-matching orders up to 44 evident in our measurements. This work provides a comprehensive overview of the limiting noise sources in QFC devices that use quasi-phase-matched crystals and will prove an invaluable resource in guiding their future development.

Cavity-enhanced induced coherence without induced emission

This paper presents a theoretical study of the enhancement of Zou-Wang-Mandel (ZWM) interferometry through cavity-enhanced spontaneous parametric down-conversion (SPDC) processes producing frequency-entangled biphotons. The ZWM interferometry shows the capability to generate interference effects between single signal photons via indistinguishability between the entangled idler photons. This paper extends the foundational principles of ZWM interferometry by integrating cavity-enhanced SPDCs, aiming to narrow photon bandwidths for improved coherence and photon pair generation efficiency, which is critical for applications in quantum information technologies, quantum encryption, and quantum imaging. This work explores the theoretical implication of employing singly resonant optical parametric oscillators within the ZWM interferometer to produce narrow-band single photons. By combining cavity-enhanced SPDCs with ZWM interferometry, this study fills a gap in current theoretical proposals, offering significant advancements in quantum cryptography and network applications that require reliable, narrow-band single photons.

Nonclassical Correlations between Photons and Phonons of Center-of-Mass Motion of a Mechanical Oscillator.

We demonstrate nonclassical correlations between phonons and photons created using opto-mechanical spontaneous parametric down-conversion in a system based on a soft-clamped ultracoherent membrane oscillator inside of a Fabry-Pérot optical resonator. Non-Gaussian quantum features are demonstrated for the center-of-mass motion of a submillimeter nanogram-scale mechanical oscillator. We show that phonons stored in the mechanical oscillator, when subsequently read out, display strong signs of quantum coherence, which we demonstrate by single-photon counting enabled by our state-of-the-art optical filtering system. We observe a violation of the classical two-time Cauchy-Schwarz inequality between a heralding write photon and a stored phonon with a confidence of >92%.

Modal phase-matching in thin-film lithium niobate waveguides for efficient generation of entangled photon pairs

Thin-film lithium niobate (TFLN) waveguides have emerged as a pivotal platform for on-chip spontaneous parametric down-conversion (SPDC), serving as a crucible for the generation of entangled photon pairs. The periodic poling of TFLN, while capable of generating high-efficiency SPDC, demands intricate fabrication processes that can be onerous in terms of scalability and manufacturability. In this work, we introduce a novel approach to the generation of entangled photon pairs via SPDC within TFLN waveguides, harnessing the principles of modal phase-matching (MPM). To address the challenge of efficiently exciting pump light typically in a higher-order mode, we have engineered a mode converter that couples two asymmetrically dimensioned waveguides. This converter adeptly transforms the fundamental mode into a higher-order mode, demonstrating a conversion loss of 1.55 dB at 785 nm with a 3 dB bandwidth exceeding 30 nm. Subsequently, we have showcased the device’s capabilities by characterizing the pair generation rate (PGR), coincidences-to-accidentals ratio (CAR), and spectral profile of the entangled photon source. Our findings present a simplified and versatile method for the on-chip generation of entangled photon sources, which may pave the way for the application in the realms of quantum information processing and communication technologies.

Unveiling quantum correlations of SPDC biphoton spatial modes using spatial light modulator

Abstract We experimentally demonstrate the quantum entanglement in various spatial modes of the correlated photons generated via spontaneous parametric down-conversion (SPDC) in a type-II phase-matched periodicallypoled KTP (ppKTP) crystal. The two-fold coincidence measurement reveals the spatial entanglement between the photon pairs by projecting one of the correlated photons onto a Gaussian mode while scanning the spatial mode of its partner photon through selective projection (Gaussian, Laguerre-Gaussian, Bessel-Gaussian, and Airy-Gaussian) using a spatial light modulator (SLM). We also show the spatially-resolved detection of the orbital angular momentum (OAM) non-conservation via modal decomposition of the correlated photon in Laguerre-Gaussian and Bessel-Gaussian bases.

Single and entangled photon pair generation using atomic vapors for quantum communication applications

Significant progress has been achieved in leveraging atomic systems for the effective operation of quantum networks, which are essential for secure and long-distance quantum communication protocols. The key elements of such networks are quantum nodes that can store or generate both single and entangled photon pairs. The primary mechanisms leading to the production of single and entangled photon pairs revolve around established techniques such as parametric down-conversion, four-wave mixing, and stimulated Raman scattering. In contrast to solid-state platforms, atomic platforms offer a more controlled approach to the generation of single and entangled photon pairs, owing to the progress made in atom manipulation techniques such as trapping, cooling, and precise excitation schemes facilitated by the use of lasers. This review article delves into the techniques implemented for generating single and entangled photon pairs in atomic platforms, starting with a detailed discussion of the fundamental concepts associated with single and entangled photons and their characterization techniques. The aim is to evaluate the strengths and limitations of these methodologies and offer insights into potential applications. Additionally, the article will review the extent to which these atomic-based systems have been integrated into operational quantum communication networks.

Phase analysis of biphoton joint spectra by interference between different SPDC sources

In spontaneous parametric down-conversion, the spectral correlations between the signal and the idler are expressed by the joint spectral amplitude (JSA) function. However, in the standard coincidence measurements, the phase information of the JSA is lost, and only the square of the absolute value of the JSA is recorded, thus preventing full characterization of the biphoton state. Here, we present an experimental technique to investigate the interference of biphoton joint spectral amplitudes, unlocking new avenues in quantum photonics research. Our method explores phase-dependent phenomena within entangled biphoton spectra. This is achieved by simultaneously pumping two structured nonlinear photonic crystals and observing their interference, which reveals previously inaccessible effects with direct intensity measurements. We demonstrate the versatility of our technique by analyzing two types of joint spectra: one exhibiting a two-lobe shape and the other a three-lobe shape. Additionally, we reconstruct the joint spectral amplitudes for both scenarios and observe good agreement with theoretical predictions. These results pave the way for developing advanced quantum communication and information processing technologies using biphoton spectra.

Orchestrating time and color: a programmable source of high-dimensional entanglement

High-dimensional encodings based on temporal modes (TMs) of photonic quantum states provide the foundations for a highly versatile and efficient quantum information science (QIS) framework. Here, we demonstrate a crucial building block for any QIS applications based on TMs: a programmable source of maximally entangled high-dimensional TM states. Our source is based on a parametric downconversion process driven by a spectrally shaped pump pulse, which facilitates the generation of maximally entangled TM states with a well-defined dimensionality that can be chosen programmatically. We characterize the effective dimensionality of the generated states via measurements of second-order correlation functions and joint spectral intensities, demonstrating the generation of bi-photon TM states with a controlled dimensionality in up to 20 dimensions.

Watt-level single-frequency optical parametric oscillator around 2 µm.

A single-frequency optical parametric oscillator (OPO) operating in the wavelength range around 2 µm is reported. The OPO comprises a periodically poled LiNbO3 (PPLN) crystal for quasi-phase matching and a four-mirror ring-cavity resonant to the signal. The OPO signal and idler are tuned from 1.89 to 2.05 µm and from 2.21 to 2.42 µm, respectively, by changing the crystal temperature. Output powers in excess of 2 W are demonstrated at a pump power of 9 W for both the signal and idler over all of the respective tuning ranges. A detailed characterization of the intensity and frequency noise is presented. The OPO exhibits an integrated intensity noise below 0.1% and a linewidth of ∼58 kHz for an observation time of 1 ms. The reported performance makes this source an ideal candidate for the generation of squeezed light around 2 µm via cascaded second-harmonic generation (SHG) and parametric downconversion (PDC).

Spontaneous parametric downconversion in a laser-poled lithium niobate nonlinear photonic crystal with nanoscale resolution.

Based on quasi-phase-matching (QPM) theory, nonlinear photonic crystals (NPCs) are capable of realizing efficient spontaneous parametric downconversion (SPDC) for the generation of photonic entangled states. However, the traditional electric field poling techniques employed in NPC fabrication often result in non-negligible processing errors of a few hundred nanometers, thus impeding the production of quantum photon pairs as intended. In this work, we investigate the SPDC photon pairs generated in a laser-poled lithium niobate (LN) NPC. By using the recently developed laser poling technique, the processing error of the NPC is substantially reduced to approximately 15 nm. Consequently, the coincidence counts of the generated photon pairs in the experiment reach 83.6% of the designed value. Our result paves the way for on-demand production of high-quality quantum sources, which has potential applications in quantum communications and quantum computations.

Entanglement source and quantum memory analysis for zero-added-loss multiplexing

High-rate, high-fidelity entanglement distribution is essential to the creation of a quantum internet, but recent achievements in fiber (248 km at a 9-s−1 rate) and satellite-based (1200 km at a 1.1-s−1 rate) entanglement distribution fall far short of what is needed. Chen . [Phys. Rev. Appl. , 054209 (2023)] proposed a means for dramatically increasing entanglement-distribution rates via a scheme they called zero-added-loss multiplexing (ZALM). ZALM’s quantum transmitter employs a pair of Sagnac-configured spontaneous parametric down-converters (SPDCs), channelization via dense wavelength-division multiplexing (DWDM) filtering, and partial Bell-state measurements (BSMs) to realize a heralded source of frequency-multiplexed polarization-entangled biphotons. Each biphoton is transmitted to Alice and Bob along with a classical message identifying its frequency channel and whether a ψ− singlet or a ψ+ triplet was heralded. Alice’s and Bob’s quantum receivers then use DWDM filtering and temporal-mode conversion to interface their received biphotons to intracavity color-center quantum memories. This paper delves deeply into ZALM’s SPDCs, partial BSMs, and Duan-Kimble loading of Alice’s and Bob’s quantum memories. Its principal results—the density operators for the SPDC sources and the quantum memories—allow heralding probability, heralding efficiency, and fidelity to be evaluated for both the polarization-entangled biphotons and the loaded quantum memories, thus enabling exploration of the parameter space for optimizing ZALM’s performance. Even without a comprehensive optimization analysis, the paper’s examples already demonstrate two critical features of the ZALM architecture: (1) the necessity of achieving a near-separable channelized biphoton wave function to ensure that the biphoton sent to Alice and Bob is of high purity; and (2) the premium placed on Alice’s and Bob’s temporal-mode converters enabling narrowband push-pull memory loading to ensure that the arriving biphoton’s state is faithfully transferred to the intracavity color centers. Published by the American Physical Society 2024

Efficient photon-pair generation in layer-poled lithium niobate nanophotonic waveguides

Integrated photon-pair sources are crucial for scalable photonic quantum systems. Thin-film lithium niobate is a promising platform for on-chip photon-pair generation through spontaneous parametric down-conversion (SPDC). However, the device implementation faces practical challenges. Periodically poled lithium niobate (PPLN), despite enabling flexible quasi-phase matching, suffers from poor fabrication reliability and device repeatability, while conventional modal phase matching (MPM) methods yield limited efficiencies due to inadequate mode overlaps. Here, we introduce a layer-poled lithium niobate (LPLN) nanophotonic waveguide for efficient photon-pair generation. It leverages layer-wise polarity inversion through electrical poling to break spatial symmetry and significantly enhance nonlinear interactions for MPM, achieving a notable normalized second-harmonic generation (SHG) conversion efficiency of 4615% W−1cm−2. Through a cascaded SHG and SPDC process, we demonstrate photon-pair generation with a normalized brightness of 3.1 × 106 Hz nm−1 mW−2 in a 3.3 mm long LPLN waveguide, surpassing existing on-chip sources under similar operating configurations. Crucially, our LPLN waveguides offer enhanced fabrication reliability and reduced sensitivity to geometric variations and temperature fluctuations compared to PPLN devices. We expect LPLN to become a promising solution for on-chip nonlinear wavelength conversion and non-classical light generation, with immediate applications in quantum communication, networking, and on-chip photonic quantum information processing.

Turbulence effects mitigation for twin-photons generated by high order transverse modes

Turbulence presents challenges for free-space light-based protocols. In this work, we investigated the effect of turbulence on the correlations of twin photons prepared in Spontaneous Parametric Down Conversion (SPDC) by a pump beam with different transverse modes. We demonstrate that the strategy of coordinate inversion for mitigating turbulence-induced distortions on transverse coincidence profiles is effective for twin photons generated by HG/LG modes. The conservation of orbital angular momentum in SPDC enables us to encode information in the transverse degrees of freedom of the down-converted photon pairs. This information can have its correlation protected by the coordinate inversion technique against weak turbulence effects in free-space links.

Fabrication of hydrothermal PPKTP and its spontaneous parametric down-conversion characteristics

High-voltage electric field polarization, selective corrosion, current monitoring, and other methods are used to develop hydrothermal PPKTP. It is found that the reversal domain nucleation of hydrothermal-grown KTP crystals has four kinds of microscopic morphology, namely, strip shape, spindle shape, bullet shape and irregular shape, in the process of high voltage electric field polarization. Compared with the leakage current in the process of polarization of flux-grown KTP crystals, the hydrothermal-grown KTP crystals only exist when the applied electric field is much larger than the coercive field. The leakage current can be suppressed by multiple loading of short pulses, and the PPKTP with a poled period of 10 μm and 46 μm were fabricated, respectively. Subsequently, based on the fabricated PPKTP, the SPDC characteristics are studied. To the PPKTP with a poled period of 10 μm, the quantum entanglement source whose brightness exceeds 2.1 kHz @ 810 nm is prepared by the SPDC technique. Otherwise, the PPKTP with a poled period of 46 μm is used for SPDC, and the brightness of entangled photon pairs in channel 1 and channel 2 are 3.21 kHz @ 1560 nm and 5.31 kHz @ 1560 nm, respectively.

Frequency stabilization of self-sustained oscillations in a sideband-driven electromechanical resonator

We present a method to stabilize the frequency of self-sustained vibrations in micromechanical and nanomechanical resonators. The method refers to a two-mode system with the vibrations at significantly different frequencies. The signal from one mode is used to control the other mode. In the experiment, self-sustained oscillations of micromechanical modes are excited by pumping at the blue-detuned sideband of the higher-frequency mode. Phase fluctuations of the two modes show near-perfect anticorrelation. They can be compensated in either of the modes by a stepwise change of the pump phase. The phase change of the controlled mode is proportional to the pump phase change, with the proportionality constant independent of the pump amplitude and frequency. This finding allows us to stabilize the phase of one mode against phase diffusion using the measured phase of the other mode. We demonstrate that phase fluctuations of either the high-frequency mode or the low-frequency mode can be significantly reduced. The results open new opportunities in generating stable vibrations in a broad frequency range via parametric down-conversion in nonlinear resonators. Published by the American Physical Society 2024

Quantum ghost imaging microscopy depth-of-field study

Quantum ghost imaging approaches have been proposed to enhance biological microscopy, for example, using 2D visible detectors to provide IR images or providing additional dimensions of spatial or spectral information. Toward the goal of making such imaging schemes practical, we compare image quality and depth-of-field between traditional images and ghost images at the same excitation levels. We measure how image quality and depth-of-field depend on the parameters of the entangled light produced using type-I spontaneous parametric down-conversion (SPDC). We use a pair of time-synchronized, photon-timing single-photon avalanche diode (SPAD) array detectors to capture two distinct microscope imaging paths simultaneously on a photon-pair-by-photon-pair basis: one in a traditional imaging pathway and the other a quantum ghost imaging pathway. We calculate the depth-of-field, resolution, contrast, and signal-to-noise ratio (SNR) through the parameter space of a β-Barium Borate (BBO) type-I bulk non-linear crystal length and angle. Our results provide a basis for choosing parameters for quantum ghost imaging with type-I SPDC sources.