Spin Ratchet Research Articles

Terahertz spin ratchet effect in magnetic metamaterials

We report on spin ratchet currents driven by terahertz radiation electric fields in a Co/Pt magnetic metamaterial formed by triangle-shaped holes forming an antidots lattice and subjected to an external magnetic field applied perpendicularly to the metal film plane. We show that for a radiation wavelength substantially larger than the period of the antidots array the radiation causes a polarization-independent spin-polarized ratchet current. The current is generated by the periodic asymmetric radiation intensity distribution caused by the near-field diffraction at the edges of the antidots, which induces spatially inhomogeneous periodic electron gas heating, and a phase-shifted periodic asymmetric electrostatic force. The developed microscopic theory shows that the magnetization of the Co/Pt film results in a spin ratchet current caused by both the anomalous Hall and the anomalous Nernst effects. Additionally, we observed a polarization-dependent trigonal spin photocurrent, which is caused by the scattering of electrons at the antidot boundaries resulting in a spin-polarized current due to the magnetization. Microscopic theory of these effects reveals that the trigonal photocurrent is generated at the boundaries of the triangle antidots, whereas the spin ratchet is generated due to the spatially periodic temperature gradient over the whole film. This difference causes substantially different hysteresis widths of these two currents.

Rapidly Enhanced Spin-Polarization Injection in an Optically Pumped Spin Ratchet

Rapid injection of spin polarization into an ensemble of nuclear spins is a problem of broad interest, spanning dynamic nuclear polarization (DNP) to quantum information science. We report on a strategy to boost the spin-injection rate by exploiting electrons that can be rapidly polarized via high-power optical pumping. We demonstrate this in a model system of nitrogen-vacancy center electrons injecting polarization into a bath of ${}^{13}\mathrm{C}$ nuclei in diamond. We deliver $>20$ W of continuous, nearly isotropic, optical power to the sample, constituting a substantially higher power than in previous experiments. Through a spin-ratchet polarization transfer mechanism, we show boosts in spin-injection rates by over 2 orders of magnitude. Our experiments elucidate bottlenecks in the DNP process caused by rates of electron polarization, polarization transfer to proximal nuclei, and spin diffusion. This work demonstrates opportunities for rapid spin injection employing nonthermally generated electron polarization, and has relevance to a broad class of experimental systems, including in DNP, quantum sensing, and spin-based MASERs (microwave amplification by stimulated emission of radiation).

Reciprocity in diffusive spin-current circuits

Similarly to their purely electric counterparts, spintronic circuits may be presented as networks of lumped elements. Due to interplay between spin and charge currents, each element is described by a matrix conductance. We establish reciprocity relations between the entries of the conductance matrix of a multi-terminal linear device, comprising normal metallic and strong ferromagnetic elements with spin-inactive interfaces between them. In particular, reciprocity equates the spin transmissions through a two-terminal element in the opposite directions. When applied to "geometric spin ratchets", reciprocity shows that certain effects, announced for such devices, are, in fact, impossible. Finally, we discuss the relation between our work and the spintronic circuit theory formalism.

Two-Electron-Spin Ratchets as a Platform for Microwave-Free Dynamic Nuclear Polarization of Arbitrary Material Targets.

Optically pumped color centers in semiconductor powders can potentially induce high levels of nuclear spin polarization in surrounding solids or fluids at or near ambient conditions, but complications stemming from the random orientation of the particles and the presence of unpolarized paramagnetic defects hinder the flow of polarization beyond the defect's host material. Here, we theoretically study the spin dynamics of interacting nitrogen-vacancy (NV) and substitutional nitrogen (P1) centers in diamond to show that outside protons spin-polarize efficiently upon a magnetic field sweep across the NV-P1 level anticrossing. The process can be interpreted in terms of an NV-P1 spin ratchet, whose handedness, and hence the sign of the resulting nuclear polarization, depends on the relative timing of the optical excitation pulse. Further, we find that the polarization transfer mechanism is robust to NV misalignment relative to the external magnetic field, and efficient over a broad range of electron-electron and electron-nuclear spin couplings, even if proxy spins feature short coherence or spin-lattice relaxation times. Therefore, these results pave the route toward the dynamic nuclear polarization of arbitrary spin targets brought in proximity with a diamond powder under ambient conditions.

Tuning magnetic ordering in a dipolar square-kite tessellation

The potential application of artificial spin ice in magnetic nanodevices provides a strong drive to investigate different lattice geometries. Here, we combine components of a recently investigated artificial spin ratchet with components of the prototypical square lattice to form a geometrically frustrated artificial spin ice system where Ising-type nanomagnets are arranged onto a two-dimensional square-kite lattice. Using synchrotron-based photoemission electron microscopy, we explore moment configurations achieved in this lattice geometry. Following thermal annealing, we image how a variation of the relevant lattice parameter affects magnetic ordering in four-island squares and four-island vertices during cooling through the Blocking temperature. Depending on lattice spacing, both nearly uniform and disordered spin configurations are accessible in our samples. We show that the relative energies of the building blocks of the system, which are typically used to classify lattice configurations, are not predictive of the low energy states adopted by the experimental system. To understand magnetic ordering in the square-kite lattice, longer range interactions must be considered.

Emergent dynamic chirality in a thermally driven artificial spin ratchet.

Modern nanofabrication techniques have opened the possibility to create novel functional materials, whose properties transcend those of their constituent elements. In particular, tuning the magnetostatic interactions in geometrically frustrated arrangements of nanoelements called artificial spin ice can lead to specific collective behaviour, including emergent magnetic monopoles, charge screening and transport, as well as magnonic response. Here, we demonstrate a spin-ice-based active material in which energy is converted into unidirectional dynamics. Using X-ray photoemission electron microscopy we show that the collective rotation of the average magnetization proceeds in a unique sense during thermal relaxation. Our simulations demonstrate that this emergent chiral behaviour is driven by the topology of the magnetostatic field at the edges of the nanomagnet array, resulting in an asymmetric energy landscape. In addition, a bias field can be used to modify the sense of rotation of the average magnetization. This opens the possibility of implementing a magnetic Brownian ratchet, which may find applications in novel nanoscale devices, such as magnetic nanomotors, actuators, sensors or memory cells.

Spin–orbit based coherent spin ratchets

The concept of ratchets, driven asymmetric periodic structures giving rise to directed particle flow, has recently been generalized to a quantum ratchet mechanism for spin currents mediated through spin–orbit interaction. Here we consider such systems in the coherent mesoscopic regime and generalize the proposal of a minimal spin ratchet model based on a non-interacting clean quantum wire with two transverse channels by including disorder and by self-consistently treating the charge redistribution in the nonlinear (adiabatic) ac-driving regime. Our Keldysh–Green function based quantum transport simulations show that the spin ratchet mechanism is robust and prevails for disordered, though non-diffusive, mesoscopic structures. Extending the two-channel to the multi-channel case does not increase the net ratchet spin current efficiency but, remarkably, yields a dc spin transmission increasing linearly with channel number.

Interplay between quantum dissipation and an in-plane magnetic field in the spin ratchet effect

We investigate the existence of the pure spin ratchet effect in a dissipative quasi-one-dimensional system with Rashba spin-orbit interaction. The system is additionally placed into a transverse uniform stationary in-plane magnetic field. It is shown that the effect exists at low temperatures and pure spin currents can be generated by applying an unbiased ac driving to the system. An analytical expression for the ratchet spin current is derived. From this expression it follows that the spin ratchet effect appears as a result of the simultaneous presence of the spin-orbit interaction, coupling between the orbital degrees of freedom and spatial asymmetry. In this paper we consider the case of a broken spatial symmetry by virtue of asymmetric periodic potentials. It turns out that an external magnetic field does not have any impact on the existence of the spin ratchet effect but it influences its efficiency, enhancing or reducing the magnitude of the spin current.

Quantum Dissipative Rashba Spin Ratchets

We predict the possibility to generate a finite stationary spin current by applying an unbiased ac driving to a quasi-one-dimensional asymmetric periodic structure with Rashba spin-orbit interaction and strong dissipation. We show that under a finite coupling strength between the orbital degrees of freedom the electron dynamics at low temperatures exhibits a pure spin ratchet behavior, i.e., a finite spin current and the absence of charge transport in spatially asymmetric structures. It is also found that the equilibrium spin currents are not destroyed by the presence of strong dissipation.

Coherent spin ratchets: A spin-orbit based quantum ratchet mechanism for spin-polarized currents in ballistic conductors

We demonstrate that the combined effect of a spatially periodic potential, lateral confinement, and spin-orbit interaction gives rise to a quantum ratchet mechanism for spin-polarized currents in two-dimensional coherent conductors. Upon adiabatic ac driving, in the absence of a net static bias, the system generates a directed spin current while the total charge current is zero. We analyze the underlying mechanism by employing symmetry properties of the scattering matrix and numerically verify the effect for different setups of ballistic conductors. The spin current direction can be changed upon tuning the Fermi energy or the strength of the Rashba spin-orbit coupling.

Zeeman ratchets: pure spin current generation in mesoscopic conductors with non-uniform magnetic fields

We consider the possibility to employ a quantum wire realized in a two-dimensional electron gas (2DEG) as a spin ratchet. We show that a net spin current without accompanying net charge transport can be induced in the nonlinear regime by an unbiased external driving via an ac voltage applied between the contacts at the ends of the quantum wire. To achieve this, we make use of the coupling of the electron spin to inhomogeneous magnetic fields created by ferromagnetic stripes patterned on the semiconductor heterostructure that harbors the 2DEG. Using recursive Green function techniques, we numerically study two different set-ups, consisting of one and two ferromagnetic stripes, respectively.