Spin Phase Research Articles

Magnon Supercurrent and the Phase Slippage in an Yttrium Iron Garnet Film

Exactly forty years ago, the spin superfluidity and Bose–Einstein condensation of magnons in superfluid antiferromagnetic 3He-B were discovered. In this work, the existence of spin superfluidity and phase slippage in an yttrium iron garnet film at room temperature is demonstrated using the optical Faraday effect. The s-patial distribution of the phase and amplitude of the spin precession under the conditions of magnon Bose‒Einstein condensation are studied by varying the pump phase difference between two strip lines exciting magnons.

Unusual Quasiparticles and Tunneling Conductance in Quantum Point Contacts in ν=2/3 Fractional Quantum Hall Systems.

Understanding topological matter in the fractional quantum Hall (FQH) effect requires identifying the nature of edge state quasiparticles. FQH edge state at the filling factor ν=2/3 in the spin-polarized and unpolarized phases is represented by the two modes of composite fermions (CF) with the parallel or opposite spins described by the chiral Luttinger liquids. Tunneling through a quantum point contact (QPC) between different or similar spin phases is solved exactly. With the increase of the applied voltage, the QPC conductance grows from zero and saturates at e^{2}/2h while a weak electron tunneling between the edge modes with the same spin transforms into a backscattering carried by the charge q=e/2 quasiparticles. These unusual quasiparticles and conductance plateau emerge when one or two CF spin-polarized modes in the QPC tunnel into a single mode. We propose experiments on the applied voltage and temperature dependence of the QPC conductance and noise that can shed light on the nature of edge states and FQH transport.

Anomalous Landau Level Gaps Near Magnetic Transitions in Monolayer WSe2

First-order phase transitions produce abrupt changes to the character of both ground and excited electronic states. Here we conduct electronic compressibility measurements to map the spin phase diagram and Landau level (LL) energies of monolayer WSe2 in a magnetic field. We resolve a sequence of first-order phase transitions between completely spin-polarized LLs and states with LLs of both spins. Unexpectedly, the LL gaps are roughly constant over a wide range of magnetic fields below the transitions, which we show reflects spin-polarized ground states with opposite spin excitations. These transitions also extend into compressible regimes, with a sawtooth boundary between full and partial spin polarization. We link these observations to the important influence of LL filling on the exchange energy beyond a smooth density-dependent contribution. Our results show that WSe2 realizes a unique hierarchy of energy scales where such effects induce reentrant magnetic phase transitions tuned by density and magnetic field. Published by the American Physical Society 2024

Magnetic relaxation between ferromagnetic and helix spin configurations in holmium films

Multiple noncollinear spin structures and transitions between them initiated by field and temperature have attracted attention due to the extraordinary coexistence of complicated spin phases in Ho. We explore the magnetic relaxation dynamics within thin films undergoing transitions between ferromagnetic (FM) and helix states. When measuring susceptibility in a relatively high frequency range (∼100–1500 Hz) and magnetic viscosity at lower frequency (∼0.01 Hz), we focus on 400 nm thick Ho film. Notably, sharp variations in the real and imaginary components of magnetic susceptibility are discerned during the FM – Helix transition, occurring at temperatures between 15 and 30 K. Hysteresis effects in the magnetic susceptibility components are identified during cyclic variations in the external field, indicating a relatively rapid process with a timescale of approximately 10 ms accompanying the FM – Helix transition. The slow relaxation process is also found to exhibit sensitivity to this transition. Furthermore, the field dependence of magnetic viscosity displays a marked decline at the FM – Helix transition. The research methodologies proposed for the investigation of relaxation processes in materials with multiphase spin structures are deemed universally applicable and offer insights into transitions between spin states in materials manifesting non collinear spin structures.

Predictions for Sparse Photometry of Jupiter-family Comet Nuclei in the LSST Era

The Legacy Survey of Space and Time (LSST) at Vera C. Rubin Observatory will deliver high-quality, temporally sparse observations of millions of solar system objects on an unprecedented scale. Such data sets will likely enable the precise estimation of small-body properties on a population-wide basis. In this work, we consider the possible applications of photometric data points from LSST to the characterization of Jupiter-family comet (JFC) nuclei. We simulate sparse-in-time lightcurve points with an LSST-like cadence for the orbit of a JFC between 2024 and 2033. Convex lightcurve inversion is used to assess whether the simulation input parameters can be accurately reproduced for a sample of nucleus rotation periods, pole orientations, activity onsets, shapes, and sizes. We find that the rotation period and pole direction can be reliably constrained across all nucleus variants tested, and that the convex shape models, while limited in their ability to describe complex or bilobed nuclei, are effective for correcting sparse photometry for rotational modulation to improve estimates of nucleus phase functions. Based on this analysis, we anticipate that LSST photometry will significantly enhance our present understanding of the spin state and phase function distributions of JFC nuclei.

Combined spin orientation and phase function of asteroids

Context. Large sky surveys provide numerous non-targeted observations of small bodies of the Solar System. The upcoming LSST of the Vera C. Rubin Observatory will be the largest source of small body photometry in the next decade. With non-coordinated epochs of observation, colors – and therefore taxonomy and composition – can only be computed by comparing absolute magnitudes obtained in each filter by solving the phase function (evolution of brightness of the small body against the solar phase angle). Current models in use in the community (HG, HG12*, and HG1G2), however, fail to reproduce the long-term photometry of many targets due to the change in the aspect angle between apparitions. Aims. We aim to derive a generic yet simple phase function model accounting for the variable geometry of the small bodies over multiple apparitions. Methods. As a spinoff of the HG1 G2 model, we propose the sHG1G2 phase function model in which we introduce a term describing the brightness changes due to spin orientation and polar oblateness. We applied this new model to 13 245 908 observations of 122 675 Solar System objects (SSOs). These observations were acquired in the g and r filters with the Zwicky Transient Facility between November 1, 2019 and December 1, 2023. We retrieved them and implemented the new sHG1G2 model in FINK, a broker of alerts designed for the LSST. Results. The sHG1G2 model leads to smaller residuals than other phase function models, providing a better description of the photometry of asteroids. We determined the absolute magnitude, H, and phase function coefficients (G1, G2) in each filter, the spin orientation (α0, δ0), and the polar-to-equatorial oblateness, R, for 95 593 SSOs, which constitutes about a tenfold increase in the number of characterized objects compared to the current census. Conclusions. The application of the sHG1 G2 model to ZTF alert data using the FINK broker shows that the model is appropriate for extracting physical properties of asteroids from multi-band and sparse photometry, such as the forthcoming LSST survey.

Sym4state.jl: An efficient computation package for magnetic materials

Exploring magnetic configurations of magnets often involves utilizing the four-state method to obtain the magnetic interaction matrix, and Monte Carlo method to simulate spin textures and phase transition processes. However, computing the interaction matrix between magnetic atoms using the four-state method requires plenty of individual calculations. Despite manual simplifying the number of individual calculations based on material's symmetry is possible, there remains a necessity for an automated approach to streamline the process for high-throughput screening of magnetic materials. Meanwhile, the traditional sequential Monte Carlo simulation encounters challenges of low efficiency and long time consuming in dealing with large systems. Furthermore, the prior parallelism in the Heisenberg model was limited to parallel computation of the system's energy or run several replicas in parallel. Hence, in our pursuit of comprehensive parallelization for the Heisenberg model, we have introduced a novel adaptation of the checkerboard algorithm, enabling a fully parallelizable simulation of the Heisenberg model. To address these problems, we have developed Sym4state.jl, a program specifically designed to simplify the computation of magnetic interaction matrix and simulate spin textures under various environmental conditions. This program, available as a Julia package, can be freely accessed at https://github.com/A-LOST-WAPITI/Sym4state.jl. Program summaryProgram title: Sym4state.jlCPC Library link to program files:https://doi.org/10.17632/s6dkmgrjfw.1Developer's repository link:https://github.com/A-LOST-WAPITI/Sym4state.jlLicensing provisions: MITProgramming language: JuliaNature of problem: Employing the four-state method to calculate magnetic interaction matrix for magnetic materials can be simplified based on material symmetry, however, there is a lack of automated approach to streamline the simplification. Additionally, the commonly used Metropolis method for simulating magnetic texture can only make parallel computation of the system's energy or run several replicas in parallel, which could hardly boost the performance when simulating the large-scale magnetic textures.Solution method: We simplify the four-state method calculations by utilizing the principles of energy invariance under symmetry operations and time reversal operations. To enhance the efficiency of the Metropolis algorithm, we have designed a strategy to divide the entire 2D lattice into multiple domains. We then execute the Metropolis algorithm in parallel for each individual domain, thereby improving the overall computational efficiency.Additional comments including restrictions and unusual features: While the methods aimed at simplifying the four-state method and parallelizing the Metropolis algorithm are applicable to both 2D and 3D systems, the current program is specifically designed for the calculation and simulation of magnetism in 2D materials. As a result, compatibility with 3D systems has not yet been implemented.

Quantum control and Berry phase of electron spins in rotating levitated diamonds in high vacuum

Levitated diamond particles in high vacuum with internal spin qubits have been proposed for exploring macroscopic quantum mechanics, quantum gravity, and precision measurements. The coupling between spins and particle rotation can be utilized to study quantum geometric phase, create gyroscopes and rotational matter-wave interferometers. However, previous efforts in levitated diamonds struggled with vacuum level or spin state readouts. To address these gaps, we fabricate an integrated surface ion trap with multiple stabilization electrodes. This facilitates on-chip levitation and, for the first time, optically detected magnetic resonance measurements of a nanodiamond levitated in high vacuum. The internal temperature of our levitated nanodiamond remains moderate at pressures below 10−5 Torr. We have driven a nanodiamond to rotate up to 20 MHz (1.2 × 109 rpm), surpassing typical nitrogen-vacancy (NV) center electron spin dephasing rates. Using these NV spins, we observe the effect of the Berry phase arising from particle rotation. In addition, we demonstrate quantum control of spins in a rotating nanodiamond. These results mark an important development in interfacing mechanical rotation with spin qubits, expanding our capacity to study quantum phenomena.

An antiferromagnetic spin phase change memory

The electrical outputs of single-layer antiferromagnetic memory devices relying on the anisotropic magnetoresistance effect are typically rather small at room temperature. Here we report a new type of antiferromagnetic memory based on the spin phase change in a Mn-Ir binary intermetallic thin film at a composition within the phase boundary between its collinear and noncollinear phases. Via a small piezoelectric strain, the spin structure of this composition-boundary metal is reversibly interconverted, leading to a large nonvolatile room-temperature resistance modulation that is two orders of magnitude greater than the anisotropic magnetoresistance effect for a metal, mimicking the well-established phase change memory from a quantum spin degree of freedom. In addition, this antiferromagnetic spin phase change memory exhibits remarkable time and temperature stabilities, and is robust in a magnetic field high up to 60 T.

Stochastic quantum trajectories demonstrate the quantum Zeno effect in open spin 1/2, spin 1 and spin 3/2 systems

We investigate the quantum Zeno effect (QZE) in spin 1/2, spin 1 and spin 3/2 open quantum systems undergoing Rabi oscillations, revealing unexplored features for the spin 1 and spin 3/2 systems. The systems interact with an environment designed to perform continuous measurements of an observable, driving the systems stochastically towards one of the eigenstates of the corresponding operator. The system-environment coupling constant represents the strength of the measurement. Stochastic quantum trajectories are generated by unravelling a Markovian Lindblad master equation using the quantum state diffusion formalism. These are regarded as a more appropriate representation of system behaviour than consideration of the averaged evolution since the latter can mask the effect of measurement. Complete positivity is maintained and thus the trajectories can be considered as physically meaningful. The QZE is investigated over a range of measurement strengths. Increasing the strength leads to greater system dwell in the vicinity of the eigenstates of the measured observable and lengthens the time taken by the system to return to that eigenstate, thus the QZE emerges. For very strong measurement, the Rabi oscillations resemble randomly occurring near-instantaneous jumps between eigenstates. The trajectories followed by the quantum system are heavily dependent on the measurement strength which other than slowing down and adding noise to the Rabi oscillations, changes the paths taken in spin phase space from a circular precession into elaborate figures-of-eight. For spin 1 and spin 3/2 systems, the measurement strength determines which eigenstates are explored and the QZE is stronger when the system dwells in the vicinity of certain eigenstates compared to others.

When you think you should transfuse…don't!

A 48-year-old female presented to the emergency department with severe fatigue. Admission laboratory test results were hemoglobin 6.6 g/dL, platelet count 287,000/μL, and white blood cell count 25,200/μL. Lactate dehydrogenase was elevated at 898 U/L, haptoglobin was markedly decreased (< 31 mg/dL), indirect bilirubin was elevated (5.3 mg/dL), and the absolute reticulocyte count was low at 0.0050/μL. A sample was sent to the immunohematology reference laboratory. The direct antiglobulin test immunoglobulin G was negative; C3 was 1+. All cells were reactive at immediate spin phase, indirect antiglobulin testing (IAT) with polyethylene glycol, with low ionic strength saline, neat, prewarm, and in the solid phase. All cells were nonreactive at IAT-ficin. Additional testing included a cold antibody titer that was 1:4096 and thermal amplitude studies demonstrating reactivity of 2+ at 37°C. These results were consistent with a clinically significant anti-Pr and cold agglutinin disease (CAD). Although rituximab is effective in autoimmune hemolytic anemia, this may take weeks. The patient was treated with pegcetacoplan, a pegylated peptide that targets C3 inhibiting hemolysis. The patient was discharged on day 29 with a hemoglobin of 8 g/dL. This is a report of one of the first patients successfully treated with pegcetacoplan for CAD.

Study on microscopic origin of spin excitation in TmFeO3 by time-resolved multicolor optical pump-probe spectroscopy

Spin dynamics of TmFeO3, mainly induced by two different mechanisms, were investigated by time-resolved multicolor pump-probe spectroscopy using femtosecond laser pulses. The spin dynamics, caused either by spin-reorientation phase transition or optical polarization-dependent effect, were distinguished by investigating their dependencies on external magnetic field and optical polarization. Spectral-dependent magneto-optic studies of the spin phase transition-induced spin dynamics revealed that laser-induced nonthermal exchange interaction between the electron states of iron (Fe3+) and thulium (Tm3+) ions is crucial for subsequent spin dynamics. This exchange interaction is influenced by the population change of the 4f electron states of Tm3+ ions, making the spin wave generation highly dependent on crystal temperature. However, spectroscopic studies of the polarization-dependent spin dynamics show that they are only related to the 3d electrons of Fe3+ ions, therefore, the spin dynamics appear to be a universal effect over a wide temperature range. Our observation can be further applied to study extended orthoferrite systems with other rare earth atoms.

NMR diffusion in restricted environment approached by a fractional Langevin model

The diffusion motion of spin-bearing molecules is considerably affected in confined environments. In Nuclear Magnetic Resonance (NMR) experiments, under the presence of magnetic field gradients, this movement can be encoded in spin phase and the NMR signal attenuation due to diffusion can be evaluated. This paper considered this effect in both normal and anomalous diffusion by means of the Langevin stochastic model within the Gaussian phase approximation (GPA) for a constant gradient temporal profile. The phenomenological approach illustrates the emergence of fractional order exponential decay in the NMR signal and retrieves the classical result from Hanh echo.

Global biasing using a hardware-based artificial Zeeman term in spinwave Ising machines

A spinwave Ising machine (SWIM) is a recently proposed type of time-multiplexed hardware solver for combinatorial optimization that employs feedback coupling and phase sensitive amplification to map an Ising Hamiltonian into phase-binarized propagating spinwave RF pulses in an Yttrium-Iron-Garnet film. In this work, we increase the mathematical complexity of the SWIM by adding a global Zeeman term to a 4-spin nearest neighbor Hamiltonian using a continuous external electrical signal with the same frequency as the spin pulses and phase locked with one of the two possible states. We are able to induce ferromagnetic ordering in both directions of the spin states despite antiferromagnetic pairwise coupling. Embedding a planar antiferromagnetic spin system in a magnetic field has been proven to increase the complexity of the graph associated with its Hamiltonian, and, thus, this straightforward implementation helps explore higher degrees of complexity in this evolving solver.

Coexistence of Quantum-Spin-Hall and Quantum-Hall-Topological-Insulating States in Graphene/hBN on SrTiO3 Substrate.

SrTiO3 (STO) substrate, a perovskite oxide material known for its high dielectric constant (ɛ), facilitates the observation of various (high-temperature) quantum phenomena. A quantum Hall topological insulating (QHTI) state, comprising two copies of QH states with antiparallel two ferromagnetic edge-spin overlap protected by the U(1) axial rotation symmetry of spin polarization, has recently been achieved in low magnetic field (B) even as high as ≈100 K in a monolayer graphene/thin hexagonal boron nitride (hBN) spacer placed on an STO substrate, thanks to the high ɛ of STO. Despite the use of the heavy STO substrate, however, proximity-induced quantum spin Hall (QSH) states in 2D TI phases, featuring a topologically protected helical edge spin phase within time-reversal-symmetry, is not confirmed. Here, with the use of a monolayer hBN spacer, it is revealed the coexistence of QSH (at B = 0T) and QHTI (at B ≠ 0) states in the same single graphene sample placed on an STO, with a crossover regime between the two at low B. It is also classified that the different symmetries of the two nontrivial helical edge spin phases in the two states lead to different interaction with electron-puddle quantum dots, caused by a local surface pocket of the STO, in the crossover regime, resulting in a spin dephasing only for the QHTI state. The results obtained using STO substrates open the doors to investigations of novel QH spin states with different symmetries and their correlations with quantum phenomena. This exploration holds value for potential applications in spintronic devices.

Soft Mesocrystal Enabled Multi‐Degree Light Modulation

AbstractMesocrystals introduce high‐level orders, such as chirality, topology, and hierarchy to the crystallography, and thus bring collective and emergent properties beyond traditional crystals. Orthogonally modulating the multiple degrees of light is highly pursued to fully explore the intrinsic multidimensional and large‐scale parallel processing capability of photon informatics. Unfortunately, it is unachievable with traditional light–matter interaction systems. Here, the multi‐degree light modulation is realized based on the hierarchical architecture of a soft mesocrystal. High‐quality monodomains of both blue phase I and blue phase II are formed via regulating the assembly of liquid crystals by photoalignment anchoring and electricity. The mapping relationship between optical freedoms (the spin, wavelength, and geometric phase of light) and hierarchical structures (the chirality of helix, lattice constant, and the azimuthal orientation of cubic lattices) is established. Omnidirectional spatial phase modulation with spin and full color selectivity is demonstrated. Based on the multi‐degree light modulation, 3D and wavelength‐selective orbital angular momentum generation as well as multichannel color holographic display are presented. This work extends the fundamental understanding of blue phase mesocrystals and provides a promising strategy for large‐scale parallel and multi‐degree light modulation that may be utilized in vital fields, such as supercomputing, optical communications, and virtual/augmented realities.

Phase transitions associated with magnetic-field induced topological orbital momenta in a non-collinear antiferromagnet

Resistivity measurements are widely exploited to uncover electronic excitations and phase transitions in metallic solids. While single crystals are preferably studied to explore crystalline anisotropies, these usually cancel out in polycrystalline materials. Here we show that in polycrystalline Mn3Zn0.5Ge0.5N with non-collinear antiferromagnetic order, changes in the diagonal and, rather unexpected, off-diagonal components of the resistivity tensor occur at low temperatures indicating subtle transitions between magnetic phases of different symmetry. This is supported by neutron scattering and explained within a phenomenological model which suggests that the phase transitions in magnetic field are associated with field induced topological orbital momenta. The fact that we observe transitions between spin phases in a polycrystal, where effects of crystalline anisotropy are cancelled suggests that they are only controlled by exchange interactions. The observation of an off-diagonal resistivity extends the possibilities for realising antiferromagnetic spintronics with polycrystalline materials.

Ab Initio Predictions of Spin Relaxation, Dephasing, and Diffusion in Solids.

Spin relaxation, dephasing, and diffusion are at the heart of spin-based information technology. Accurate theoretical approaches to simulate spin lifetimes (τs), determining how fast the spin polarization and phase information will be lost, are important to the understanding of the underlying mechanism of these spin processes, and invaluable in searching for promising candidates of spintronic materials. Recently, we develop a first-principles real-time density-matrix (FPDM) approach to simulate spin dynamics for general solid-state systems. Through the complete first-principles descriptions of light-matter interaction and scattering processes including electron-phonon, electron-impurity, and electron-electron scatterings with self-consistent spin-orbit coupling, as well as ab initio Landé g-factor, our method can predict τs at various conditions as a function of carrier density and temperature, under electric and magnetic fields. By employing this method, we successfully reproduce experimental results of disparate materials and identify the key factors affecting spin relaxation, dephasing, and diffusion in different materials. Specifically, we predict that germanene has long τs (∼100 ns at 50 K), a giant spin lifetime anisotropy, and spin-valley locking effect under electric fields, making it advantageous for spin-valleytronic applications. Based on our theoretical derivations and ab initio simulations, we propose a new useful electronic quantity, named spin-flip angle θ↑↓, for the understanding of spin relaxation through intervalley spin-flip scattering processes. Our method can be further applied to other emerging materials and extended to simulate exciton spin dynamics and steady-state photocurrents due to photogalvanic effect.

Studying the variations of the cyclotron line in Cen X-3 using Insight-HXMT

We investigate the cyclotron resonant scattering features (CRSFs) of the accreting X-ray pulsar Cen X-3 and significantly detect the 29 keV cyclotron line features in the hard X-ray averaged spectroscopy studies based on the recent Insight-HXMT observations in 2022, when Cen X-3 has X-ray luminosity LX>∼5×1037 erg s−1 in the bands of 2 – 60 keV. We do not find a harmonic line in the average spectra based on different continuum models. We showed that the CRSF energies have no correlation with time or luminosity in the average spectra. In addition, by performing a pulse phase-dependent spectral analysis, we revealed the fundamental line with the centroid energy ranging from 25 to 29 keV with a high significance over the spin phases. The evolution of the cyclotron line centroid energies over pulse phase is similar to the shape of pulse profiles, illustrating a positive correlation between the energy of CRSFs and the pulse phase flux.

Nonequilibrium dynamics of the Jaynes-Cummings dimer.

We investigate the nonequilibrium dynamics of a Josephson-coupled Jaynes-Cummings dimer in the presence of Kerr nonlinearity, which can be realized in the cavity and circuit quantum electrodynamics systems. The semiclassical dynamics is analyzed systematically to chart out a variety of photonic Josephson oscillations and their regime of stability. Different types of transitions between the dynamical states lead to the self-trapping phenomenon, which results in photon population imbalance between the two cavities. We also study the dynamics quantum mechanically to identify characteristic features of different steady states and to explore fascinating quantum effects, such as spin dephasing, phase fluctuation, and revival phenomena of the photon field, as well as the entanglement of spin qubits. For a particular "self-trapped" state, the mutual information between the atomic qubits exhibits a direct correlation with the photon population imbalance, which is promising for generating photon mediated entanglement between two non interacting qubits in a controlled manner. Under a sudden quench from stable to unstable regime, the photon distribution exhibits phase space mixing with a rapid loss of coherence, resembling a thermal state. Finally, we discuss the relevance of the new results in experiments, which can have applications in quantum information processing and quantum technologies.