Spin-imbalanced Fermi Gases Research Articles

Stable nonequilibrium Fulde-Ferrell-Larkin-Ovchinnikov state in a spin-imbalanced driven-dissipative Fermi gas loaded on a three-dimensional cubic optical lattice

Stable nonequilibrium Fulde-Ferrell-Larkin-Ovchinnikov state in a spin-imbalanced driven-dissipative Fermi gas loaded on a three-dimensional cubic optical lattice

Disordered structures in ultracold spin-imbalanced Fermi gas

We investigate properties of spin-imbalanced ultracold Fermi gas in a large range of spin polarizations at low temperatures. We present results of microscopic calculations based on mean-field and density functional theory approaches, with no symmetry constraints. At low polarization values we predict the structure of the system as consisting of several spin-polarized droplets. As the polarization increases, the system self-organizes into a disordered structures similar to liquid crystals, and energetically they can compete with ordered structures such as grid-like domain walls. At higher polarizations the system starts to develop regularities that, in principle, can be called supersolid, where periodic density modulation and pairing correlations coexist. The robustness of the results has been checked with respect to temperature effects, dimensionality, and the presence of a trapping potential. Dynamical stability has also been investigated.

Feasibility of a Fulde-Ferrell-Larkin-Ovchinnikov superfluid Fermi atomic gas

We theoretically explore a promising route to achieve the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state in a spin-imbalanced ultracold Fermi gas. In the current stage of cold atom physics, search for this exotic Fermi superfluid is facing two serious difficulties: One is the desperate destruction of the FFLO long-range order by FFLO pairing fluctuations, which precludes entering the phase through a second-order transition, even in three dimension. The other is the fierce competition with the phase separation into the BCS (Bardeen-Cooper-Schrieffer) state and the spin-polarized normal state. Including strong FFLO pairing fluctuations within the framework of the strong-coupling theory developed by Nozi\`eres and Schmitt-Rink, we show that the anisotropy of Fermi surface introduced by an optical lattice makes the FFLO state stable against the paring fluctuations. This stabilized FFLO state is also found to be able to overcome the competition with the phase separation under a certain condition. Since the realization of unconventional Fermi superfluids is one of the most exciting challenges in cold atom physics, our results would contribute to the further development of this field.

Coexistence of topological and nontopological Fermi-superfluid phases

The two-dimensional spin-imbalanced Fermi gas subject to s-wave pairing and spin-orbit coupling is considered a promising platform for realizing a topological chiral-p-wave superfluid. In the BCS limit of s-wave pairing, i.e., when Cooper pairs are only weakly bound, the system enters the topological phase via a second-order transition driven by increasing the Zeeman spin-splitting energy. Stronger attractive two-particle interactions cause the system to undergo the BCS-BEC crossover, in the course of which the topological transition becomes first-order. As a result, topological and nontopological superfluids coexist in spatially separated domains in an extended region of phase space spanned by the strength of s-wave interactions and the Zeeman energy. Here we investigate this phase-coexistence region theoretically using a zero-temperature mean-field approach. Exact numerical results are presented to illustrate basic physical characteristics of the coexisting phases and to validate an approximate analytical description derived for weak spin-orbit coupling. Besides extending our current understanding of spin-imbalanced superfluid Fermi systems, the present approach also provides a platform for future studies of unconventional Majorana excitations that, according to topology, should be present at the internal interface between coexisting topological and nontopological superfluid parts of the system.

Vortex lattice in spin-imbalanced unitary Fermi gas

We investigate the properties of a spin-imbalanced and rotating unitary Fermi gas. Using a density functional theory (DFT), we provide insight into states that emerge as a result of a competition between Abrikosov lattice formation, spatial phase separation and the emergence of Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state. A confrontation of the experimental data [M. Zwierlein et al., Science 311, 492 (2006)] with theoretical predictions provides a remarkable qualitative agreement. In case of gas confined in a harmonic trap, the phase separation into a superfluid core populated by the Abrikosov lattice and a spin-polarized corona is the dominant process. Changing confinement to a box-like trap, reverts the spatial location of the component: gas being in the normal state is surrounded by superfluid threaded by quantum vortices. The vortex lattice no longer exhibits the triangular symmetry, and emergence of exotic geometries may be an indirect signature of the FFLO-like state formation in the system.

Thermodynamic signatures of the polaron-molecule transition in a Fermi gas

We consider the highly spin-imbalanced limit of a two-component Fermi gas, where there is a small density of $\downarrow$ impurities attractively interacting with a sea of $\uparrow$ fermions. In the single-impurity limit at zero temperature, there exists the so-called polaron-molecule transition, where the impurity sharply changes its character by binding a $\uparrow$ fermion at sufficiently strong attraction. Using a recently developed variational approach, we calculate the thermodynamic properties of the impurity, and we show that the transition becomes a smooth crossover at finite temperature due to the thermal occupation of excited states in the impurity spectral function. However, remnants of the single-impurity transition are apparent in the momentum-resolved spectral function, which can in principle be probed with Raman spectroscopy. We furthermore show that the Tan contact exhibits a characteristic non-monotonic dependence on temperature that provides a signature of the zero-temperature polaron-molecule transition. For a finite impurity density, we argue that descriptions purely based on the behavior of the Fermi polaron are invalid near the polaron-molecule transition, since correlations between impurities cannot be ignored. In particular, we show that the spin-imbalanced system undergoes phase separation at low temperatures due to the strong attraction between $\uparrow\downarrow$ molecules induced by the Fermi sea. Thus, we find that the impurity spectrum and the induced impurity-impurity interactions are key to understanding the phase diagram of the spin-imbalanced Fermi gas.

Observation of a Smooth Polaron-Molecule Transition in a Degenerate Fermi Gas

Understanding the behavior of an impurity strongly interacting with a Fermi sea is a long-standing challenge in many-body physics. When the interactions are short-ranged, two vastly different ground states exist: a polaron quasiparticle and a molecule dressed by the majority atoms. In the single-impurity limit, it is predicted that at a critical interaction strength, a first-order transition occurs between these two states. Experiments, however, are always conducted in the finite temperature and impurity density regime. The fate of the polaron-to-molecule transition under these conditions, where the statistics of quantum impurities and thermal effects become relevant, is still unknown. Here, we address this question experimentally and theoretically. Our experiments are performed with a spin-imbalanced ultracold Fermi gas with tunable interactions. Utilizing a novel Raman spectroscopy combined with a high-sensitivity fluorescence detection technique, we isolate the quasiparticle contribution and extract the polaron energy, spectral weight, and the contact parameter. As the interaction strength is increased, we observe a continuous variation of all observables, in particular a smooth reduction of the quasiparticle weight as it goes to zero beyond the transition point. Our observation is in good agreement with a theoretical model where polaron and molecule quasiparticle states are thermally occupied according to their quantum statistics. At the experimental conditions, polaron states are hence populated even at interactions where the molecule is the ground state and vice versa. The emerging physical picture is thus that of a smooth transition between polarons and molecules and a coexistence of both in the region around the expected transition.

Spin-imbalanced ultracold Fermi gases in a two-dimensional array of tubes

Motivated by a recent experiment [Revelle et al. Phys. Rev. Lett. 117, 235301 (2016)] that characterized the one- to three-dimensional crossover in a spin-imbalanced ultracold gas of $^6$Li atoms trapped in a two-dimensional array of tunnel-coupled tubes, we calculate the phase diagram for this system using Hartree-Fock Bogoliubov-de Gennes mean-field theory, and compare the results with experimental data. Mean-field theory predicts fully spin-polarized normal, partially spin-polarized normal, spin-polarized superfluid, and spin-balanced superfluid phases in a homogeneous system. We use the local density approximation to obtain density profiles of the gas in a harmonic trap. We compare these calculations with experimental measurements in Revelle {\em et al.} as well as previously unpublished data. Our calculations qualitatively agree with experimentally-measured densities and coordinates of the phase boundaries in the trap, and quantitatively agree with experimental measurements at moderate-to-large polarizations. Our calculations also reproduce the experimentally-observed universal scaling of the phase boundaries for different scattering lengths at a fixed value of scaled inter-tube tunneling. However, our calculations have quantitative differences with experimental measurements at low polarization, and fail to capture important features of the one- to three-dimensional crossover observed in experiments. These suggest the important role of physics beyond-mean-field theory in the experiments. We expect that our numerical results will aid future experiments in narrowing the search for the FFLO phase.

Application of the renormalized random-phase approximation to polarized Fermi gases

We consider a spin imbalanced Fermi gas at zero temperature in the normal phase on the BCS side of the BCS-BEC crossover and around unitarity. We compute the critical polarization for pairing, the correlated occupation numbers and the contact in an extension of particle-particle RPA (also called non self-consistent \textit{T}-matrix approach or ladder approximation). The so-called renormalized RPA consists in computing the \textit{T} matrix with self-consistently determined occupation numbers. The occupation numbers are determined either by keeping the self-energy only to first order or by resumming the Dyson equation. In this way, the result for the critical polarization, strongly overestimated in standard RPA, is clearly improved. We also discuss some problems of this approach.

Diffusion Monte Carlo study of a spin-imbalanced two-dimensional Fermi gas with attractive interactions

We probe the superconducting gap in the zero temperature ground state of an attractively interacting spin-imbalanced two-dimensional Fermi gas with Diffusion Monte Carlo. A condensate fraction at nonzero pair momentum evidences a spatially non-uniform superconducting order parameter. Comparison with exact diagonalisation studies confirms that the nonzero condensate fraction across a range of nonzero fermion pair momenta is consistent with non-exclusive pairing between majority and minority fermions, an extension beyond FFLO theory.

Communal pairing in spin-imbalanced Fermi gases

A spin-imbalanced Fermi gas with an attractive contact interaction forms a superconducting state whose underlying components are superpositions of Cooper pairs that share minority-spin fermions. This superconducting state includes correlations between all available fermions, making it energetically favorable to the Fulde--Ferrell--Larkin--Ovchinnikov superconducting state. The ratio of the number of up- and down-spin fermions in the instability is set by the ratio of the up- and down-spin density of states in momentum at the Fermi surfaces, to fully utilize the accessible fermions. We present analytical and complementary Diffusion Monte Carlo results for the state.

Atomtronics with a spin: Statistics of spin transport and nonequilibrium orthogonality catastrophe in cold quantum gases

We propose to investigate the full counting statistics of nonequilibrium spin transport with an ultracold atomic quantum gas. The setup makes use of the spin control available in atomic systems to generate spin transport induced by an impurity atom immersed in a spin-imbalanced two-component Fermi gas. In contrast to solid-state realizations, in ultracold atoms spin relaxation and the decoherence from external sources is largely suppressed. As a consequence, once the spin current is turned off by manipulating the internal spin degrees of freedom of the Fermi system, the nonequilibrium spin population remains constant. Thus one can directly count the number of spins in each reservoir to investigate the full counting statistics of spin flips, which is notoriously challenging in solid state devices. Moreover, using Ramsey interferometry, the dynamical impurity response can be measured. Since the impurity interacts with a many-body environment that is out of equilibrium, our setup provides a way to realize the non-equilibrium orthogonality catastrophe. Here, even for spin reservoirs initially prepared in a zero-temperature state, the Ramsey response exhibits an exponential decay, which is in contrast to the conventional power-law decay of Anderson's orthogonality catastrophe. By mapping our system to a multi-step Fermi sea, we are able to derive analytical expressions for the impurity response at late times. This allows us to reveal an intimate connection of the decay rate of the Ramsey contrast and the full counting statistics of spin flips.

Thermal crossover, transition, and coexistence in Fermi polaronic spectroscopies

We investigate thermal evolution of radio-frequency (RF) spectra of a spin-imbalanced Fermi gas near a Feshbach resonance in which degenerate Fermi-polaron and classical Boltzmann-gas regimes emerge in the low-temperature and high-temperature limits, respectively. By using a self-consistent framework of strong-coupling diagrammatic approaches, both of the ejection and reserve RF spectra available in cold-atom experiments are analyzed. We find a variety of transfers from Fermi polarons to Boltzmann gas such that a thermal crossover expected in the weak-coupling regime is shifted to a sharp transition near unitarity and to double-peak coexistence of attractive and repulsive branches in the strong-coupling regime. Our theory provides semiquantitative descriptions for a recent experiment on the ejection RF spectroscopy at unitarity [Z. Yan {\it et al}., arXiv:1811.00481v1] and demonstrate that the RF spectroscopy is an essential probe to examine effects of strong correlations and finite temperature.

Communal pairing in spin-imbalanced Fermi gases

A spin-imbalanced Fermi gas with an attractive contact interaction forms a superconducting state whose underlying components are superpositions of Cooper pairs that share minority-spin fermions. This superconducting state includes correlations between all available fermions, making it energetically favorable to the Fulde-Ferrell-Larkin-Ovchinnikov superconducting state. The ratio of the number of up- and down-spin fermions in the instability is set by the ratio of the up- and down-spin density of states in momentum at the Fermi surfaces, to fully utilize the accessible fermions. We present analytical and complementary Diffusion Monte Carlo results for the state.

Multiparticle instability in a spin-imbalanced Fermi gas

Weak attractive interactions in a spin-imbalanced Fermi gas induce a multi-particle instability, binding multiple fermions together. The maximum binding energy per particle is achieved when the ratio of the number of up- and down-spin particles in the instability is equal to the ratio of the up- and down-spin densities of states in momentum at the Fermi surfaces, to utilize the variational freedom of all available momentum states. We derive this result using an analytical approach, and verify it using exact diagonalization. The multi-particle instability extends the Cooper pairing instability of balanced Fermi gases to the imbalanced case, and could form the basis of a many-body state, analogously to the construction of the Bardeen-Cooper-Schrieffer theory of superconductivity out of Cooper pairs.

Low-energy modes of spin-imbalanced Fermi gases in BCS phase

The low-energy modes of a spin-imbalanced superfluid Fermi gas in the Bardeen-Cooper-Schrieffer (BCS) side are studied. The gas is assumed to be sufficiently dilute so that the pairing of atoms can be considered effective only in s-wave between fermions of different internal state. The order parameter at equilibrium is determined by the mean-field approximation, while the properties of the collective modes are calculated within a Gaussian approximation for the fluctuations of the order parameter. In particular we investigate the effects of asymmetry between the populations of the two different components and of temperature on the frequency and damping of collective modes. It is found that the temperature does not much affect the frequency and the damping of the modes, whereas an increase of the imbalance shifts the frequency toward lower values and enhances the damping sensitively. Besides the Bogoliubov-Anderson phonons, we observe modes at zero frequency for finite values of the wave-number. These modes indicate that an instability develops driving the system toward two separate phases, normal and superfluid.

Core filling and snaking instability of dark solitons in spin-imbalanced superfluid Fermi gases

We use the time-dependent Bogoliubov de Gennes equations to study dark solitons in three-dimensional spin-imbalanced superfluid Fermi gases. We explore how the shape and dynamics of dark solitons are altered by the presence of excess unpaired spins which fill their low-density core. The unpaired particles broaden the solitons and suppress the transverse snake instability. We discuss ways of observing these phenomena in cold atom experiments.

Larkin-Ovchinnikov superfluidity in a two-dimensional imbalanced atomic Fermi gas

We present an extensive study of two-dimensional Larkin-Ovchinnikov (LO) superfluidity in a spin-imbalanced two-component atomic Fermi gas. In the context of Fulde-Ferrell-Larkin- Ovchinnikov (FFLO) phase, we explore a wide and generic class of pairing gap functions with ex- plicit spatial dependency. The mean-field theory of such phases is applied through the Bogoliubov-de Gennes equations in which the pairing gap can be determined self-consistently. In order to systemat- ically explore the configuration space we consider both the canonical and grand canonical ensembles where we control the polarization or chemical potentials of the system, respectively. The mean-field calculations enable us to understand the nature of the phase transitions in the fully paired Bardeen- Cooper-Schrieffer (BCS) state, exotic LO phase, and partially polarized free Fermi gas. The order of the phase transitions has been examined and in particular we find a weak first-order phase transition between the exotic inhomogeneous LO phase and the BCS phase. In comparison to the three-dimensional case, where the phase diagram is dominated by a generic separation phase, we predict a broader parameter space for the spatially inhomogeneous LO phase. By computing the superfluid density of the LO phase at different polarization, we show how the superfluidity of the system is suppressed with increasing spin polarization.

Dimensional crossover in a spin-imbalanced Fermi gas

We model the one-dimension (1D) to three-dimension (3D) crossover in a cylindrically trapped Fermi gas with attractive interactions and spin-imbalance. We calculate the mean-field phase diagram, and study the relative stability of exotic superfluid phases as a function of interaction strength and temperature. For weak interactions and low density, we find 1D-like behavior, which repeats as a function of the chemical potential as new channels open. For strong interactions, mixing of single-particle levels gives 3D-like behavior at all densities. Furthermore, we map the system to an effective 1D model, finding significant density dependence of the effective 1D scattering length.

1D to 3D Crossover of a Spin-Imbalanced Fermi Gas.

We have characterized the one-dimensional (1D) to three-dimensional (3D) crossover of a two-component spin-imbalanced Fermi gas of ^{6}Li atoms in a 2D optical lattice by varying the lattice tunneling and the interactions. The gas phase separates, and we detect the phase boundaries using insitu imaging of the inhomogeneous density profiles. The locations of the phases are inverted in 1D as compared to 3D, thus providing a clear signature of the crossover. By scaling the tunneling rate t with respect to the pair binding energy ε_{B}, we observe a collapse of the data to a universal crossover point at a scaled tunneling value of t[over ˜]_{c}=0.025(7).